Ultrafast near-field imaging of exciton-polariton dynamics in WSe_2 waveguides at room temperature

TL;DR

This paper introduces a novel ultrafast near-field imaging technique to directly observe the femtosecond-scale formation and propagation of exciton-polaritons in WSe2 waveguides at room temperature, revealing slow group velocities.

Contribution

It presents the first direct ultrafast imaging of exciton-polariton dynamics in vdW materials, advancing understanding of their spatio-temporal behavior at room temperature.

Findings

Observed slow exciton-polariton group velocity (~0.017c)

Demonstrated direct visualization of EP formation and propagation

Linked bandgap renormalization to light coupling near exciton transition

Abstract

Van der Waals (vdW) materials, weakly bound layered compounds, have received enormous interest as they offer a malleable playground for a wide range of physical properties in thermal, electronic and optical devices. In particular, owing to their inherent deep subwavelength light confinement, they support a variety of light-matter interactions phenomena such as plasmons, excitons and phonons conveyed as polaritonic modes. Specifically, semiconductor vdW materials such as WSe_2 are particularly attractive for photonic and quantum integrated technologies since they sustain VIS-NIR exciton-polariton modes at room temperature. In the quest to unravel the underlying physics of these intriguing phenomena, advanced subdiffraction imaging techniques such as SNOM has provided valuable insights on the nature of the EP coupling mechanism to the waveguide modes sustained in vdW materials. While most of these works focused on the steady state of the EP, the spatio-temporal dynamics of EP formation, happening in the sub-picosecond regime, remains largely unexplored. Hence, a direct imaging at the femtosecond-nanoscale of the EP evolution is critical to the understanding of these coupled light-matter states. Here we report for the first time the ultrafast and deep-subwavelength imaging of EP formation and propagation in WSe2 waveguides. Our method, based on a novel ultrafast pump-probe near-field imaging, allows to directly visualize the EP time evolution at room temperature. More specifically, and in agreement with our time dependent model, we directly observe a significantly slow EP wave packet group velocity of v_g~0.017c which is attributed to the bandgap renormalization originating in the light coupling near the exciton transition. These findings suggest that vdW materials could be used for slow light with applications in light storage for memory, enhanced optical nonlinearity, sensing and more.