Granular materials flow like complex fluids

TL;DR

This study uses X-ray tomography to analyze the microscopic relaxation dynamics of granular ellipsoids under shear, revealing universal displacement distributions and power-law mean squared displacements, highlighting their complex fluid-like behavior.

Contribution

It provides the first detailed experimental characterization of particle-level relaxation in 3D granular systems, showing their dynamics differ from thermal glass-formers and resemble complex fluids.

Findings

Displacement distribution follows a time- and strain-independent Gumbel law.

Mean squared displacement exhibits power-law behavior with strain-dependent exponents.

Granular relaxation involves friction and memory effects, unlike thermal systems.

Abstract

Granular materials such as sand, powders, foams etc. are ubiquitous in our daily life, as well as in industrial and geotechnical applications. Although these disordered systems form stable structures if unperturbed, in practice they do relax because of the presence of unavoidable external influences such as tapping or shear. Often it is tacitly assumed that for granular systems this relaxation dynamics is similar to the one of thermal glass-formers, but in fact experimental difficulties have so far prevented to determine the dynamic properties of three dimensional granular systems on the particle level. This lack of experimental data, combined with the fact that in these systems the motion of the particles involves friction, makes it very challenging to come up with an accurate description of their relaxation dynamics. Here we use X-ray tomography to determine the microscopic relaxation dynamics of hard granular ellipsoids that are subject to an oscillatory shear. We find that the distribution function of the particle displacement can be described by a Gumbel law with a shape parameter that is independent of time and the strain amplitude $\gamma$. Despite this universality, the mean squared displacement of a tagged particle shows power-laws as a function of time with an exponent that depends on $\gamma$ and the time interval considered. We argue that these results are directly related to the existence of the microscopic relaxation mechanisms that involve friction and memory effects. These observations demonstrate that on the particle level the dynamical behavior of granular systems is qualitatively different from the one of thermal glass-formers and instead more similar to the one of complex fluids. Thus we conclude that granular materials can relax even when the driving is weak, an insight which impacts our understanding of the nature of granular solids.