Frequency-dependent current noise in quantum heat transfer with full counting statistics

TL;DR

This paper develops a theory to analyze frequency-dependent current noise in quantum heat transfer, extending previous zero-frequency models and applying it to a spin-boson system with detailed results on noise behavior.

Contribution

It introduces a generalized formulation of frequency-dependent current noise for quantum heat transfer using full counting statistics and applies it to a non-equilibrium spin-boson model.

Findings

Maximal FDCN occurs in moderate coupling regimes.

FDCN exhibits Lorentzian scaling in weak coupling.

Strong coupling leads to white noise spectrum and bias suppression.

Abstract

To investigate frequency-dependent current noise (FDCN) in open quantum systems at steady states, we present a theory which combines Markovian quantum master equations with a finite time full counting statistics. Our formulation of the FDCN generalizes previous zero-frequency expressions and can be viewed as an application of MacDonald's formula for electron transport to heat transfer. As a demonstration, we consider the paradigmatic example of quantum heat transfer in the context of a non-equilibrium spin-boson model. We adopt a recently developed polaron-transformed Redfield equation which allows us to accurately investigate heat transfer with arbitrary system-reservoir coupling strength, arbitrary values of spin bias as well as temperature differences. We observe maximal values of FDCN in moderate coupling regimes, similar to the zero-frequency cases. We find the FDCN with varying coupling strengths or bias displays a universal Lorentzian-shape scaling form in the weak coupling regime, and a white noise spectrum emerges with zero bias in the strong coupling regime due to a distinctive spin dynamics. We also find the bias can suppress the FDCN in the strong coupling regime, in contrast to its zero-frequency counterpart which is insensitive to bias changes. Furthermore, we utilize the Saito-Utsumi relation as a benchmark to validate our theory and study the impact of temperature differences at finite frequencies. Together, our results provide detailed dissections of the finite time fluctuation of heat current in open quantum systems.