Quantum versus classical dynamics in the optical centrifuge

TL;DR

This paper compares quantum and classical dynamics in the optical centrifuge, identifying two resonance mechanisms and analyzing their effects on rotational excitation efficiency through theoretical and numerical methods.

Contribution

It introduces a quantum mechanical formalism for the optical centrifuge and distinguishes between classical autoresonance and quantum ladder-climbing mechanisms.

Findings

Good agreement between numerical simulations and theory

Identification of two distinct resonant excitation mechanisms

Analysis relevant to current experimental setups

Abstract

The interplay between classical and quantum mechanical evolution in the optical centrifuge (OC) is discussed. The analysis is based on the quantum mechanical formalism starting from either the ground state or a thermal ensemble. Two resonant mechanisms are identified, i.e. the classical autoresonance and the quantum mechanical ladder-climbing, yielding different dynamics and rotational excitation efficiencies. The rotating wave approximation is used to analyze the two resonant regimes in the associated dimensionless two-parameter space and calculate the OC excitation efficiency. The results show good agreement between numerical simulations and theory and are relevant to existing experimental setups.