Magnetic ground state and magnon-phonon interaction in multiferroic h-YMnO$_3$

TL;DR

This study investigates the magneto-elastic excitations in multiferroic h-YMnO3 using neutron scattering, revealing magnon-phonon hybridization, field-induced effects, and providing a comprehensive theoretical model that clarifies the magnetic ground state.

Contribution

It presents a detailed experimental and theoretical analysis of magnon-phonon interactions in h-YMnO3, establishing a quantitative model that explains hybridized modes and magnetic ground state symmetry.

Findings

Identification of avoided crossing between magnon and phonon modes.

Observation of field-induced splitting of spin wave branches.

Development of a Heisenberg model that reproduces experimental dispersion.

Abstract

Inelastic neutron scattering has been used to study the magneto-elastic excitations in the multiferroic manganite hexagonal YMnO$_3$. An avoided crossing is found between magnon and phonon modes close to the Brillouin zone boundary in the $(a,b)$-plane. Neutron polarization analysis reveals that this mode has mixed magnon-phonon character. An external magnetic field along the $c$-axis is observed to cause a linear field-induced splitting of one of the spin wave branches. A theoretical description is performed, using a Heisenberg model of localized spins, acoustic phonon modes and a magneto-elastic coupling via the single-ion magnetostriction. The model quantitatively reproduces the dispersion and intensities of all modes in the full Brillouin zone, describes the observed magnon-phonon hybridized modes, and quantifies the magneto-elastic coupling. The combined information, including the field-induced magnon splitting, allows us to exclude several of the earlier proposed models and point to the correct magnetic ground state symmetry, and provides an effective dynamic model relevant for the multiferroic hexagonal manganites.