Two-color pump-probe interferometry of ultra-fast light-matter interaction

TL;DR

This paper introduces a two-color pump-probe interferometry technique that achieves high spatial and temporal resolution for observing ultra-fast light-matter interactions, revealing charge dynamics and electron removal processes.

Contribution

It presents a novel two-color side-view probing method with holographic digital focusing for high-resolution imaging of ultra-fast plasma dynamics.

Findings

Resolved electron removal with ~150 fs time constant

Achieved ~0.9 μm spatial and ~20 fs temporal resolution

Demonstrated potential for deep-sub-wavelength optical control

Abstract

Two-color side-view probing of light-matter interaction from minute focal volume of a tightly focused fs-laser pump pulse reveals charge dynamics with high 0.9 micrometers optical resolution and approximately ~20 fs temporal resolution in coincidence between pump and probe pulses. Use of two colors is advantageous for probing optically excited plasma regions with different density. Holographical digital focusing and spatial filtering were implemented to obtain the same resolution images for subsequent Fourier analysis. Fast electron removal with time constant ~150 fs was resolved and is consistent with self-trapping. Potential applications of an optical control over a light-induced defect placement with deep-sub-wavelength resolution is discussed.