# High Photovoltaic Quantum Efficiency in Ultrathin van der Waals   Heterostructures

**Authors:** Joeson Wong, Deep Jariwala, Giulia Tagliabue, Kevin Tat, Artur R., Davoyan, Michelle C. Sherrott, Harry A. Atwater

arXiv: 1706.02700 · 2017-06-09

## TL;DR

This paper demonstrates ultrathin van der Waals heterostructures with high external quantum efficiencies over 50% and internal collection efficiencies above 70%, achieved through experimental and simulation methods.

## Contribution

It presents the first experimental demonstration of ultrathin heterostructures with over 50% external quantum efficiency and high internal collection efficiency.

## Key findings

- External quantum efficiency exceeds 50%.
- Absorbance surpasses 90%.
- Internal collection efficiency exceeds 70%.

## Abstract

We report experimental measurements for ultrathin (< 15 nm) van der Waals heterostructures exhibiting external quantum efficiencies exceeding 50%, and show that these structures can achieve experimental absorbance > 90%. By coupling electromagnetic simulations and experimental measurements, we show that pn WSe2/MoS2 heterojunctions with vertical carrier collection can have internal photocarrier collection efficiencies exceeding 70%.

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Source: https://tomesphere.com/paper/1706.02700