Andreev levels as a quantum dissipative environment
A.V. Galaktionov, D.S. Golubev, and A.D. Zaikin

TL;DR
This paper models the quantum behavior of superconducting weak links at subgap energies using an effective Hamiltonian that includes Andreev levels as a dissipative environment, revealing different regimes of supercurrent decay.
Contribution
It introduces an exact Hamiltonian model incorporating Andreev levels as a quantum dissipative environment affecting supercurrent decay regimes.
Findings
Identification of three supercurrent decay regimes based on dissipation and capacitance
Demonstration of the environment's role in crossover between quantum and thermal decay
Quantitative analysis of Andreev levels' impact on supercurrent dynamics
Abstract
We argue that at subgap energies quantum behavior of superconducting weak links can be exactly accounted for by an effective Hamiltonian for a Josephson particle in a quantum dissipative environment formed by Andreev levels. This environment can constitute an important source for intrinsic inelastic relaxation and dephasing in highly transparent weak links. We investigate the problem of macroscopic quantum tunneling in such weak links demonstrating that -- depending on the barrier transmission -- the supercurrent decay can be described by three different regimes: () weak intrinsic dissipation, () strong intrinsic dissipation and () strong capacitance renormalization. Crossover between quantum and thermally-assisted supercurrent decay regimes can also be strongly affected by the Andreev level environment.
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Taxonomy
TopicsQuantum and electron transport phenomena · Physics of Superconductivity and Magnetism · Cold Atom Physics and Bose-Einstein Condensates
Andreev levels as a quantum dissipative environment
Artem V. Galaktionov1, Dmitry S. Golubev2 and Andrei D. Zaikin3,1
1I.E.Tamm Department of Theoretical Physics, P.N.Lebedev Physical Institute, 119991 Moscow, Russia
2Low Temperature Laboratory, Department of Applied Physics, Aalto University, Espoo, Finland
3Institute of Nanotechnology, Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe, Germany
Abstract
We argue that at subgap energies quantum behavior of superconducting weak links can be exactly accounted for by an effective Hamiltonian for a Josephson particle in a quantum dissipative environment formed by Andreev levels. This environment can constitute an important source for intrinsic inelastic relaxation and dephasing in highly transparent weak links. We investigate the problem of macroscopic quantum tunneling in such weak links demonstrating that – depending on the barrier transmission – the supercurrent decay can be described by three different regimes: () weak intrinsic dissipation, () strong intrinsic dissipation and () strong capacitance renormalization. Crossover between quantum and thermally-assisted supercurrent decay regimes can also be strongly affected by the Andreev level environment.
I Introduction
Quantum dissipation is known to occur as a result of interaction with an effective environment. Quite generally, this environment can be modeled as a set of harmonic oscillators. Tracing out the oscillator degrees of freedom one naturally arrives at the Feynman-Vernon influence functional theory FH and the Caldeira-Leggett description of quantum dissipation CL ; Weiss . Electrons in metallic conductors can also play the role of a quantum dissipative environment, as it is illustrated, e.g., by the Ambegaokar-Eckern-Schön (AES) effective action treatment of metallic tunnel junctions AES ; SZ . Further extension of the influence functional technique also allows to directly account for Fermi statistics GZ99 in the situation when electrons in a metal form an effective environment ”for themselves”.
In superconducting tunnel junctions dissipation at low enough temperatures/energies can only occur extrinsically (e.g. by attaching an Ohmic shunt resistor CL ; Weiss ; SZ ) as there exist no states with energies below the superconducting gap in such junctions. The situation changes if one goes beyond the tunneling limit. In this case subgap Andreev bound states And are formed inside superconducting weak links. For sufficiently short junctions the corresponding bound state energies are , where
[TABLE]
denote normal transmissions of conducting channels and is the superconducting phase difference across the junction. While in the tunneling limit one has for any value , at higher transmissions the energies of Andreev levels (1) can drop well below and may even tend to zero for fully open channels and .
Here we will demonstrate that Andreev bound states – along with model oscillators FH ; CL ; Weiss or electrons in a metal AES ; SZ ; GZ99 – may act as intrinsic quantum dissipative environment for the Josephson phase strongly affecting quantum properties of superconducting weak links.
II Effective Hamiltonian for a weak link
In what follows we will consider a current biased superconducting junction characterized by a geometric capacitance and an arbitrary distribution of normal transmissions among transport channels. Provided the phase does not fluctuate the junction may conduct the supercurrent KO
[TABLE]
Here and below the sum runs over all channels from to . In order to describe quantum fluctuation effects it is necessary to treat the phase as a quantum variable SZ . The generalization of the AES type-of-approach can be worked out also beyond the tunneling limit employing both Matsubara Z and Keldysh SN techniques, however the resulting effective action becomes tractable only in certain physical situations.
One of such situations is realized if phase fluctuations remain sufficiently weak we ; we2 . Splitting the phase variable into constant and fluctuating parts and assuming one can express the kernel of the Keldysh evolution operator as a double path integral
[TABLE]
where the phase variables are defined respectively on the forward and backward branches of the Keldysh contour and ] define local in time contributions
[TABLE]
Here is the effective junction capacitance which may differ from due to retardation effects we and
[TABLE]
is the effective potential where the first term is recovered by integrating the supercurrent (2) over and the second term accounts for the bias current .
The remaining – nonlocal in time – terms
[TABLE]
describe the influence functional for the phase variable. Here we denote and . Both kernels and in Eqs. (6), (7) are real functions related to each other via the fluctuation-dissipation theorem. General expressions for each of these kernels remain rather involved we and contain three different contributions originating from (i) the subgap Andreev bound states, (ii) the quasiparticle states above the gap and (iii) the interference between (i) and (ii).
Significant simplifications occur provided both temperature and typical phase fluctuation frequencies remain well in the subgap range, i.e. . Under this condition the contributions (ii) and (iii) to the kernel vanish, while the analogous contributions to the Fourier component of can be expanded in powers of up to terms which yields an effective capacitance renormalization. In the interesting for us limit and this renormalization yields
[TABLE]
What remains is to account for the Andreev terms (i) in both kernels and . Making use of the results we ; we2 , we obtain
[TABLE]
where
[TABLE]
Note that in the limit and provided the Fourier component of the kernel in Eq. (9) can also be expanded in powers of up to terms giving rise to extra renormalization of we (see below). For , however, this expansion is not justified anymore. For this reason in what follows we will keep the kernel in its exact form (9).
It is interesting to observe that the influence functional defined in Eqs. (6)-(10) is exactly equivalent to that produced by a bath of harmonic oscillators FH ; CL ; Weiss coupled linearly to the fluctuating part of the phase . In other words, our weak link can also be described by an effective low energy Hamiltonian
[TABLE]
The first and the second lines of Eq. (12) account respectively for the ”Josephson particle” and for its Andreev level environment which consists of harmonic oscillators with frequencies coupled to the ”particle coordinate” . The coupling constants are identified by the condition . It is important to emphasize that the Hamiltonian (12) follows directly from a fully microscopic effective action we without any model assumptions.
Before dwelling into further calculations it is instructive to also construct the grand partition function for our weak link . Making use of the effective Hamiltonian in Eq. (12) we can express in terms of the path integral over both and the oscillator coordinates . Integrating out all -variables we obtain
[TABLE]
where
[TABLE]
is the imaginary time effective action for our superconducting contact and
[TABLE]
Expanding the kernel (15) in the Fourier series with , we get
[TABLE]
III Andreev level bath spectrum and inelastic relaxation
To begin with, we observe that the coupling constants (11) vanish in the limit . Thus, environmental modes corresponding to fully open transport channels are totally decoupled from the phase variable and, hence, cannot influence its quantum dynamics.
On the other hand, channels with do affect the behavior of . As long as remains much smaller than the -th environmental mode may only contribute to extra capacitance renormalization. Provided the inequality is fulfilled for all we again recover the corresponding result for the renormalized capacitance we . In the opposite limit Andreev levels may already act as a quantum dissipative environment for the fluctuating phase. This is because the oscillators can get excited to higher energy states as a result of their interaction with . Note that since phase fluctuations remain small the conjugate charge variable, in contrast, fluctuates strongly implying that multiple electron charge transfer is possible through each conducting channel. Accordingly, many of such electrons can in general get excited to the higher of the two Andreev levels while passing through the -th channel. These processes translate into the excitation of harmonic oscillators to higher levels illustrating the physical reason why the effect of Andreev doublets is equivalent to that of such oscillators.
The frequency spectrum of this quantum dissipative environment depends on the particular distribution of normal transmissions . Let us introduce
[TABLE]
For a junction with large number of channels and with transmissions distributed in the interval with the probability after a simple algebra for we get
[TABLE]
and otherwise. Here we define
[TABLE]
Intrinsic dissipation due to subgap Andreev levels can be identified if we consider, e.g., the two lowest energy levels in the Josephson potential well which can also be treated as a qubit. The corresponding inelastic relaxation rate for such a qubit reads
[TABLE]
Here is the junction charging energy, is the plasma oscillation frequency and the phase is fixed by the condition .
In many cases remains of order . E.g., in diffusive junctions at and close to one finds . Only provided is close to and, in addition, there exist transmitting channels with the frequency can go well below . This situation occurs, e.g., in the problem of macroscopic quantum tunneling (MQT) to be addressed below.
IV MQT in highly transparent weak links
Provided a superconducting weak link with is biased by the current close to the zero resistance state becomes unstable and can decay into a resistive state due to quantum tunneling of the phase across the potential barrier . In the case of superconducting tunnel barriers with this MQT problem with extrinsic dissipation was thoroughly studied in the past CL ; Weiss . Here we consider the opposite limit of highly transparent weak links with in which case the critical current is reached at the phase value close to . Such weak links can now be fabricated in a controlled manner employing a variety of different materials including, e.g., atomic point contacts exp1 , graphene-based weak links exp2 ; exp3 , high transparency Al/BiTe/Al double barrier heterostructures exp4 , or InAs nanowire Josephson junctions exp5 . In some of these experiments effective channel transmissions with values very close to unity were demonstrated.
In what follows for simplicity we will assume that all the junction transmissions have the same value and, hence, , cf. Eq. (1). We also define the reflection coefficient and the parameter .
Let us evaluate the supercurrent decay rate with the exponential accuracy . At the effective potential (5) reduces to a simple form
[TABLE]
For Eq. (21) can be simplified further by expanding it in powers of around . Dropping an unimportant constant we get
[TABLE]
Observing a strong inequality below we will set . For the expansion (22) is no more sufficient, and the exact form of (21) should be employed.
Provided geometric capacitance is large it suffices to ignore both effects of capacitance renormalization (8) and of Andreev levels by formally setting and in Eq. (14). Then our MQT problem reduces to that of a quantum particle with mass which tunnels under the barrier in the potential (21). This problem is resolved easily with the result
[TABLE]
where defines the potential barrier height and .
Note that the numerical prefactor is almost two times bigger in the limit than in the opposite one . Since we conclude that for an increase of by a very small value can result in an increase of the supercurrent decay rate by orders of magnitude. This is because the potential barrier in the limit is substantially ”thinner” than that at , while the barrier height remains the same in both limits. Hence, the tunneling probability can be much bigger in the former limit, see also Fig. 1.
Let us now assume that is small and the capacitance is dominated by the last term in Eq. (8), i.e. we set . Provided the coupling constant (11) between the particle and the Andreev bath is sufficiently small. Accordingly, dissipation remains weak and can be treated perturbatively. At we find
[TABLE]
where accounts for dissipation FNA . As long as the value grows with merely due to the potential profile change (as accounted for by the parameter in Eq. (23) and also illustrated in Fig. 1) rather than due to dissipation. Hence, in the limit the function can be safely neglected.
For effective coupling of to the Andreev level bath becomes strong and the last term in Eq. (14) should be treated nonperturbatively. It is well known that quantum tunneling can be described in terms of classical dynamics of the particle propagating in the inverted potential along the so-called bounce trajectory. Identifying the bounce frequency with that of small oscillations near the bottom of this potential at and setting again , after trivial algebra we get
[TABLE]
where we introduced the function
[TABLE]
with . For the potential (22) we find
[TABLE]
This formula together with Eqs. (25) and (26) accounts for a trade-off between two different tunneling regimes. Let us define the value from the equation which yields . In the adiabatic limit (or ) Andreev oscillators are “fast” and provide strong capacitance renormalization FN
[TABLE]
The particle then becomes heavier albeit its energy remains conserved during tunneling and Eq. (27) yields
[TABLE]
In the opposite antiadiabatic limit (or ) Andreev oscillators become “slow” generating effective potential renormalization . Such oscillators can get excited to higher levels taking energy from the tunneling particle . Hence, for Eq. (27) describes a strong dissipation regime and matches smoothly with Eq. (24) at .
V Quantum-to-classical crossover
Quantum decay can only occur at low enough temperatures whereas at thermal activation takes over with . In order to analyze the crossover between these two regimes we will employ an approximate form (22) for the potential energy . At lower Eq. (22) holds for , as we already indicated above. At higher temperatures the approximation (22) applies without any further restrictions. Indeed, at such and for Eq. (2) reduces to
[TABLE]
reaching its maximum at , where now and is the Lambert W-function defined by the equation . For we can again expand the potential (5) in and reproduce Eq. (22) with .
At temperatures in the vicinity of the crossover to thermal activation quantum tunneling is described by the bounce trajectory which remains close to the local maximum of the potential (22) at . The value is formally identified Weiss ; LO83 ; GW84 as a temperature at which the bounce first reduces to meaning that at this point. This is achieved provided the corresponding eigenvalue of the operator vanishes, which yields
[TABLE]
Resolving Eq. (31) one determines the crossover temperature . If the geometric capacitance is large, it suffices to set and in Eq. (31). Then we immediately recover the standard result Affleck , where is defined below Eq. (23). This result holds for . In the limit Eq. (31) cannot be applied anymore. In this case reaches the value in Eq. (23) at .
Perhaps the most interesting situation occurs if geometric capacitance is small and is dominated by the last term in Eq. (8). Substituting together with Eq. (16) into Eq. (31) and resolving the latter with respect to we obtain
[TABLE]
In the limit we have and Eq. (32) reduces to . In particular, at small enough we get . For Eq. (32) approaches the -independent result . The function (32) is displayed in Figs. 2 and 3 (inset) for different values of .
Note that for very small the function becomes multivalued for some values of . This behavior, however, does not imply the presence of several crossover temperatures for a given bias because the critical current also depends on temperature and, hence, . For each value the crossover temperature should be obtained from the equation , as it is also illustrated in Fig. 2. As a result, we arrive at the bias current value at which quantum-to-classical crossover occurs at a given temperature. The function is plotted in Fig. 3 for together with . With decreasing classical activation region shrinks and rapidly approaches .
In summary, we demonstrated that subgap Andreev bound states in superconducting weak links form an intrinsic quantum dissipative environment for the Josephson phase and derived a microscopic low energy Hamiltonian for such weak links. Effective coupling between and Andreev oscillators depends on transport channel transmissions and vanishes for fully open channels with . In the case of highly transparent weak links we analyzed both quantum and thermally-assisted decay of the supercurrent and identified the MQT regimes of weak intrinsic dissipation, strong intrinsic dissipation and strong capacitance renormalization. Our predictions can be directly tested by routinely measuring the statistics of switching currents (see, e.g., recent experiment Ustinov ) in highly transparent superconducting weak links in combination with Andreev level spectroscopy Urbina .
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