Critical pairing fluctuations in the normal state of a superconductor: pseudogap and quasi-particle damping
Philipp Lange, Oleksandr Tsyplyatyev, and Peter Kopietz

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Abstract
We study the effect of critical pairing fluctuations on the electronic properties in the normal state of a clean superconductor in three dimensions. Using a functional renormalization group approach to take the non-Gaussian nature of critical fluctuations into account, we show microscopically that in the BCS regime, where the inverse coherence length is much smaller than the Fermi wavevector, critical pairing fluctuations give rise to a non-analytic contribution to the quasi-particle damping of order , where the Ginzburg-Levanyuk number is a dimensionless measure for the width of the critical region. As a consequence, there is a temperature window above where the quasiparticle damping due to critical pairing fluctuations can be larger than the usual -Fermi liquid damping due to non-critical scattering processes. On the other hand, in the…
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Critical pairing fluctuations
in the normal state of a superconductor: pseudogap and quasi-particle damping
Philipp Lange, Oleksandr Tsyplyatyev, and Peter Kopietz
Institut für Theoretische Physik, Universität Frankfurt, Max-von-Laue Strasse 1, 60438 Frankfurt, Germany
(April 18, 2017)
Abstract
We study the effect of critical pairing fluctuations on the electronic properties in the normal state of a clean superconductor in three dimensions. Using a functional renormalization group approach to take the non-Gaussian nature of critical fluctuations into account, we show microscopically that in the BCS regime, where the inverse coherence length is much smaller than the Fermi wavevector, critical pairing fluctuations give rise to a non-analytic contribution to the quasi-particle damping of order , where the Ginzburg-Levanyuk number is a dimensionless measure for the width of the critical region. As a consequence, there is a temperature window above where the quasiparticle damping due to critical pairing fluctuations can be larger than the usual -Fermi liquid damping due to non-critical scattering processes. On the other hand, in the strong coupling regime where is of order unity, we find that the quasiparticle damping due to critical pairing fluctuations is proportional to the temperature. Moreover, we show that in the vicinity of the critical temperature the electronic density of states exhibits a fluctuation-induced pseudogap. We also use functional renormalization group methods to derive and classify various types of processes induced by the pairing interaction in Fermi systems close to the superconducting instability.
I Introduction
The BCS mean-field theory has been tremendously successful to explain the physical properties of superconductors, but the true critical behavior of the classical phase transition between a normal metal and a superconductor is not mean-field like but belongs to the universality class of the classical XY-model. Fortunately, in conventional superconductors the critical region where fluctuation effects are important is extremely small, so that for all practical purposes the mean-field approximation is sufficient Larkin05 . The smallness of the critical region in weakly coupled BCS superconductors is due to the fact that in these systems the zero temperature coherence length , which measures the typical size of the Cooper pairs, is many orders of magnitude larger than the lattice spacing. A dimensionless measure of the temperature range around the critical temperature where fluctuations are important is given by the Ginzburg-Levanyuk number Ginzburg60 ; Levanyuk59 , which for a clean three-dimensional superconductor can be written as Larkin05
[TABLE]
where is the Fermi energy. In the weak coupling BCS regime the value of is typically in the range between and , so that the critical region cannot be resolved experimentally. On the other hand, in strongly correlated superconductors the inverse coherence length can have the same order of magnitude as the Fermi momentum . In this case is of the order of unity and the critical regime is experimentally accessible. Another class of experimentally tunable systems where fluctuations of the superfluid order parameter cannot be neglected are the ultracold fermions with attractive interaction in the vicinity of the unitary point where the two-body scattering length diverges Bloch08 .
Although fluctuation effects in superconductors and superfluids have been studied for many decades Larkin05 , there are still some open questions. In particular, the renormalization of the electronic single-particle excitations in the normal state at or slightly above the critical temperature are not completely understood. In a seminal work by Aslamazov and LarkinAslamazov69 , the transport time and its effect on conductivity were shown to be divergent at the transition temperature within the ladder approximation. The effect of superconducting fluctuations on the density of states and the tunneling resistance has been studied within a perturbative approach to first order in the strength of the superconducting interactionDiCastro90 . This approximation is expected to break down sufficiently close to the critical temperature Larkin05 , where the non-Gaussian nature of the pairing fluctuations and the renormalization of the electronic single-particle excitations must be taken into account. The single-particle spectral function was calculated numerically in Refs. [Palestini12, ] and [Reichl15, ] using the same ladder approximation, which corresponds to treating fluctuations of the superconducting order parameter only on the Gaussian level. To the best of our knowledge, a quantitative analysis of the electronic density of states and the quasi-particle damping beyond this approximation does not exist in the literature. In the superconducting phase, the modification of the electronic density of states due to Gaussian order parameter fluctuations has been studied by Lerch et al. Lerch08 , who found an unexpected logarithmic renormalization of the BCS result. In the present work we focus on the temperature regime above the critical temperature where the system is in the normal state and hence the anomalous part of the electronic self-energy vanishes. This simplifies the calculations and enables us to include the effect of non-Gaussian critical order-parameter fluctuations on the single-particle spectrum using renormalization group methods.
Diagrammatically, retaining Gaussian fluctuations of the superconducting order parameter is equivalent to calculating the effective two-body interaction between fermions in ladder approximation, which amounts to solving the Bethe-Salpeter equation for the effective interaction in the particle-particle channel Larkin05 . Higher order interaction processes involving fluctuations with arbitrary momentum transfer give rise to non-Gaussian order parameter fluctuations. The next order effect of the pairing coupling on the critical temperature of a weakly interacting superconductor in the BCS regime has first been calculated by Gorkov and Melik-Barkhudarov (GM) Gorkov61 , who showed that even for arbitrarily weak bare interaction the fluctuations lead to a finite decrease of the critical temperature. In recent years the effects of induced interactions due to non-Gaussian pairing fluctuations have been studied for various other setups, such as systems involving more than two fermion flavors Heiselberg00 , effective models describing the crossover from a BCS superconductor to a Bose-Einstein condensate (BCS-BEC crossover) Chen05 ; Floerchinger08 ; Yu09 , and multi-band models describing the iron-based superconductors Chubukov16 . Moreover, it has been shown Lederer15 that in the vicinity of a nematic quantum critical point the induced interactions mediated by soft fluctuations associated with the nematic order parameter can enhance the critical temperature for superconductivity.
In this work we use a functional renormalization group (FRG) approach Kopietz10 ; Metzner12 to derive and classify the induced interactions responsible for the corrections to BCS theory. Our approach is based on the vertex expansion and partial bosonization in the particle-particle channel Kopietz10 ; Bartosch09 , and is therefore complementary to recent work by Tanizaki et al. Tanizaki14 , who have used a purely fermionic formulation of the FRG to calculate the correction to the BCS result for due to pairing fluctuations. Our main focus is the effect of critical pairing fluctuations on the spectrum of single-particle excitations in the normal state.
Let us give a brief overview of the rest of this work and summarize our main results. In Sec. II we derive an effective field theory describing normal fermions which are coupled to pairing fluctuations. We also show how the GM correctionGorkov61 to the critical temperature can be obtained within our approach, and that the GM result for is modified if the chemical potential (and not the density of the electrons) is held constant. Our FRG approach for this model is developed in Sec. III, where we also explain the emergence of various types of induced interaction processes due to pairing fluctuations from the renormalization group point of view.
In Sec. IV we then discuss the effect of pairing fluctuations of the superconducting order parameter on the fermionic self-energy and the density of states within the ladder approximation. We show that in this approximation the density of states exhibits a finite pseudogap but the damping of quasiparticles with momenta on the Fermi surface still diverges logarithmically as for . While the emergence of a pseudogap due to fluctuations above has been intensely investigated in the pastStajic04 ; Chien10 ; Hu10 ; Magierski11 ; Mueller17 , it is somewhat surprising that the logarithmic divergence of the quasiparticle damping in a clean three-dimensional superconductor has not been noticed in the previous literature on the subject Larkin05 . This singularity can be cured by taking into account the finite lifetime of the quasiparticles in intermediate states, or by including non-Gaussian critical pairing fluctuations which generate a finite anomalous dimension of the pairing fluctuations. In Sec. III we take both effects consistently into account using a specific implementation of the FRG. We find that the quasiparticle damping at due to critical order-parameter fluctuations has in the BCS regime the non-analytic form,
[TABLE]
where our estimate for the numerical prefactor is . Due to the rather large value of , in a sizable regime of temperatures close to the critical contribution (2) to the quasiparticle damping dominates the usual -Fermi liquid behavior due to non-critical interaction processes, as illustrated in Fig. 16 below. Moreover, we also show that in the strongly interacting superconductors, where the inverse coherence length can have the same order of magnitude as the Fermi momentum , the quasiparticle damping due to critical order-parameter fluctuations is proportional to the temperature. Finally, in Sec. V we present our conclusions and discuss possible extensions of the methods developed in this work.
Further technical details are given in five appendices. In Appendix A we discuss in detail the approximations which are necessary to derive the GM result Gorkov61 for the critical temperature from the interaction corrections to the particle-particle bubble. In Appendix B we write down exact FRG flow equations for the induced interactions in our model. The momentum-dependence of the non-interacting particle-particle bubble is derived in Appendix C, while in Appendix D we justify why in the vicinity of it is sufficient to retain only the zeroth Matsubara frequency (associated with classical fluctuations) in the bosonic correlation function. Finally, in Appendix F we improve the FRG calculation of the quasiparticle damping of Sec. IV.2 by taking into account higher order vertex corrections.
II Induced interactions in fermionic superfluids
II.1 Effective field theory for superfluid fluctuations
We consider a system of electrons with quadratic energy dispersion which are coupled by a short-range attractive two-body interaction with strength . The coupling represents some effective interaction in the spin-singlet particle-particle channel. Since we neglect long-range Coulomb interactions and do not consider the coupling to external electromagnetic fields, we do not distinguish between superfluidity and superconductivity. At finite temperature and chemical potential the Euclidean action of the system is
[TABLE]
where and are Grassmann fields labeled by momentum , Matsubara frequencies , and spin projection (we introduce collective labels and use units where and the Boltzmann constant can be set equal to unity), and the collective fields and are defined by
[TABLE]
Here represents the total (bosonic) Matsubara frequency and the total momentum of a pair of electrons with opposite spin, and the integration symbols are defined by and . Although we are eventually interested in dimensions, we will keep arbitrary before we explicitly start evaluating momentum integrals. We represent the bare interaction of our model defined in Eq. (3) by the graphical element shown in Fig. 1 (a).
The physics in the vicinity of the superfluid transition is dominated by the effective interaction in the particle-particle channel. It is then natural to decouple the two-body interaction in Eq. (3) by means of a complex bosonic Hubbard-Stratonovich field such that the composite particle-particle fields defined in Eqs. (4a) and (4b) appear in the decoupled action, which then assumes the form
[TABLE]
where we have introduced the bare fermion propagator
[TABLE]
The interaction in the last term of Eq. (5) involves three-legged (Yukawa) vertices with one bosonic and two fermionic external legs, as shown in Fig. 1 (b). We shall refer to as the order parameter field, because a finite expectation value of this field signals the existence of superfluidity in the system. In this work, we shall focus on the temperature regime above the superfluid critical temperature. In this case the exact fermionic propagator is given by
[TABLE]
where is the exact fermionic self-energy in the normal state. Similarly, the exact propagator of our order parameter field is of the form
[TABLE]
where the function can be identified with the one-interaction-line irreducible bosonic self-energy. Graphical representations of the two Dyson equations (7) and (8) are shown in Fig. 2.
Note that in lowest order perturbation theory can be identified with the particle-particle bubble with bare fermionic propagators,
[TABLE]
The transition temperature to the superfluid state can be determined from the condition that the order-parameter field for becomes gapless at , i.e.,
[TABLE]
which is equivalent with the statement that the corresponding uniform susceptibility diverges. To determine the critical temperature for superfluidity, we should calculate the function to a certain approximation and then tune the temperature such that Eq. (10) is satisfied. The corrections to the non-interacting bubble given in Eq. (9) can be expressed in terms of the induced interactions, which take scattering processes in all channels into account. Although the Hubbard-Stratonovich transformed bare action (5) does not contain two-body and higher order interaction vertices, these vertices will appear in the effective low-energy theory when we integrate out high-energy degrees of freedom. In particular, two types of fermionic two-body interaction vertices will be generated, which we denote by , and , where and the supercripts denote the field types associated with the external legs and the energy-momentum labels refer to the corresponding superscripts. Moreover, the two-body interactions between the superfluid order parameter are encoded in the bosonic interaction vertex . Finally, symmetry allows also mixed four-point vertices with two fermionic and two bosonic external legs. Graphical representations of these different types of induced interaction vertices are shown in Fig. 3.
II.2 Skeleton equations
Before calculating the fermionic and bosonic irreducible self-energies and using the FRG, it is instructive to rederive the GM result for the critical temperature using the effective field theory derived above. Therefore it is convenient to start from formally exact skeleton equations (also called Dyson-Schwinger equations), which allow us to express the self-energies in terms of the induced interaction between fermions with opposite spin. Graphically, the skeleton equations for the self-energies and and for the irreducible three-point vertices and are shown in in Fig. 4.
Formally, these equations can be derived by using the invariance of the functional integral representing the generating functional of the irreducible vertices under shift transformations of the fields ZinnJustin02 ; Kopietz10 . Explicitly, the skeleton equations relating the fermionic and bosonic self-energies to the three-point vertices are
[TABLE]
while the skeleton equations (c) and (d) in Fig. 4 relating the three-point vertex to the effective interaction between two fermions with opposite spin are
[TABLE]
Substituting these expressions into Eqs. (LABEL:eq:DysonSchwingerPhi), we obtain the skeleton equation for the bosonic self-energy shown in the second line of Fig. 4 (b),
[TABLE]
II.3 Perturbative expansion in powers of the scattering length
The GM correction to the critical temperature can now be obtained by expanding the induced interaction between electrons with opposite spin appearing in the skeleton equation (15) to second order in the scattering length. Recall that in three dimensions the -wave scattering length is defined by
[TABLE]
where the so-called -matrix in vacuum at vanishing total momentum is related to the bare interaction via
[TABLE]
and the particle-particle bubble at vanishing temperature and chemical potential is in three dimensions given by
[TABLE]
Here is an ultraviolet cutoff in momentum space and
[TABLE]
is the density of states (per spin projection) at the Fermi energy, where is the Fermi momentum. To generate an expansion in powers of , let us write the propagator of the pairing field in Gaussian approximation (where the bosonic self-energy is approximated by , see Eq. (9)) in the following form
[TABLE]
where the regularized particle-particle bubble is
[TABLE]
Due to the subtraction this expression is ultraviolet convergent so that we may take the limit . Assuming and that the relevant momenta in loop integrations are such that we may approximate
[TABLE]
The leading terms in the expansion of the fermionic self-energy and the effective interaction between fermions with opposite spin are shown in Fig. 5 (a) and (b).
Explicitly, the first order self-energy correction in Fig. 5 (a) is
[TABLE]
where is the density (per spin projection) in the non-interacting limit. The induced interaction between fermions with opposite spin to order shown in Fig. 5 (b) can be written as
[TABLE]
where
[TABLE]
is the non-interacting particle-hole bubble. Substituting these expansions into the skeleton equation (15) for the bosonic self-energy we obtain the expansion shown in Fig. 5 (c), which can be written as
[TABLE]
where the non-interacting particle-particle bubble is given in Eq. (9), the first order correction is
[TABLE]
while the leading correction due to the induced interaction is
[TABLE]
If we follow GMGorkov61 and work at constant density, the self-energy is exactly canceled by a shift in the chemical potential which is necessary to keep the density fixed; in this case we should ignore the first order correction , so that the leading interaction correction to is given by the second order term . On the other hand, at constant chemical potential the term modifies the GM result.
According to Eq. (10), the critical temperature is determined by
[TABLE]
An explicit evaluation of the three contributions on the right-hand side of this equation in the BCS regime (where ) is given in Appendix A. Here we briefly summarize the main results. First of all, for temperatures the regularized particle-particle bubble is given by
[TABLE]
where and
[TABLE]
Here is the Euler-Mascheroni constant. If we ignore the terms and on the right-hand side of Eq. (29) we obtain the mean-field critical temperature
[TABLE]
with the dimensionless interaction constant
[TABLE]
As shown in Appendix A, for the first order correction to the particle-particle bubble (27) is at low temperatures given by
[TABLE]
where
[TABLE]
and is a dimensionless ultraviolet cutoff which is necessary to regularize the relevant momentum integral. As discussed above, the contribution should be omitted if we work at constant density. The second order correction to the particle-particle bubble is
[TABLE]
with
[TABLE]
Consider first the case of constant density, where the contribution from should be omitted. Substituting Eqs. (30) and (36) into Eq. (29) we obtain the following estimate of the dimensionless critical temperature,
[TABLE]
In the asymptotic weak coupling limit we may neglect the cutoff-dependent correction and find that the induced interaction due to particle-hole fluctuations reduces the critical temperature for superfluidity by a factor of
[TABLE]
in agreement with GMGorkov61 . Note that according to Eq. (38) the cutoff-dependent correction to the GM result is of the order which depends linearly on the ultraviolet cutoff . We show in Appendix A that this linear cutoff dependence is an artifact of neglecting the momentum- and frequency dependence of the particle-hole bubble in the evaluation of Eq. (28). In a more accurate calculation taking the momentum or the frequency dependence of into account the correction depends only logarithmically on the cutoff. If the chemical potential is held constant, then the term is not canceled and we obtain
[TABLE]
which is larger than the GM result in Eq. (39). The discrepancy to the GM result for found in a recent renormalization group calculation by Tanizaki et al. Tanizaki14 seems to be due to the fact that these authors did not fix the density in their calculation.
III Induced interactions and vertex corrections from the FRG
In order to understand the origin of the GM correction from the renormalization group point of view and to set up a machinery which allows us to calculate the fermionic self-energy non-perturbatively, we develop in this section a general FRG approach for our model with bare action given by Eq. (5). To derive formally exact FRG flow equations for the irreducible vertices of our model, we introduce an additional cutoff such that for large fluctuations are suppressed while for we obtain our original model Kopietz10 . The evolution of the generating functional of the one-line irreducible vertices under changes of the cutoff is described by the Wetterich equation Wetterich93 . By expanding this equation in powers of the fields, we obtain a formally exact hierarchy of FRG flow equations for all one-line irreducible vertices of our theory. For the implementation of this procedure there is considerable freedom in the choice of the cutoff scheme. For our purpose it is most convenient to use the particle-particle version of the momentum-transfer cutoff scheme proposed in Refs. [Schuetz05, ; Schuetz06, ], which has been shown to be useful in several other contexts Kopietz10 ; Drukier12 ; Sharma16 . In this interaction-momentum cutoff scheme, we replace the inverse bare coupling of our model by the cutoff- and momentum-dependent coupling
[TABLE]
there the regulator function vanishes for and approaches some large value for , where is some large initial value of the cutoff. Below we will work with a sharp momentum cutoff which amounts to setting
[TABLE]
For , the generating functional of the cutoff-dependent one-particle irreducible vertices of our model can be expanded in powers of the fields as follows
[TABLE]
where the ellipsis represents terms involving five and more powers of the fields and all vertices are assumed to be properly symmetrized with respect to permutations of the labels associated with fields of the same type. and are the cutoff-dependent fermionic and bosonic irreducible self-energies. The corresponding cutoff-dependent inverse propagators are
[TABLE]
The last four lines in Eq. (43) represent the various induced interactions shown graphically in Fig. 3. Although these interactions do not appear in our bare action given in Eq. (5), they are generated by the FRG flow. Since we do not introduce the regulator into the fermionic sector of our model, we have to start the FRG flow at some large initial scale with a non-trivial initial condition, as explained in Refs. Kopietz10, ; Schuetz06, . Hence, apart from the initial values of the three-legged vertices which appear in the bare action (5),
[TABLE]
all purely bosonic -point vertices with incoming and outgoing boson lines are finite at the initial cutoff . Diagrammatically, these vertices can be identified with the symmetrized closed fermion loops with incoming and outgoing external bosonic legs, as shown in Fig. 6.
Specifically, the initial value of the bosonic self-energy is the non-interacting particle-particle bubble,
[TABLE]
while the bosonic four-point vertex at the initial cutoff scale is
[TABLE]
Note that this vertex is symmetric with respect to the independent exchange and . Setting all external momenta and frequencies equal to zero we obtain
[TABLE]
The contribution of the higher order bosonic vertices to the initial value of the generating functional (43) is
[TABLE]
In our approach the GM correction to is determined by the initial value of the bosonic six-point vertex, which after symmetrization can be written as
[TABLE]
All other vertices vanish at the initial scale, but all vertices which are compatible with the -symmetry of the bare action are generated by the FRG flow, in particular the induced interactions shown in Fig. 3. From the bosonic sector of our initial action it is easy to reproduce the perturbation series for the renormalized particle-particle bubble shown graphically in Fig. 5 (c). The non-interacting particle-particle bubble is contained in the Gaussian propagator , see Eq. (20). The first order corrections shown in the second line of Fig. 5 (c) can be recovered from the one-loop contraction of the four-point vertex shown in Fig. 6 (c), while the last diagram in Fig. 5 (c) which gives the GM correction is contained in the two-loop contraction of the six-point vertex shown in Fig. 6 (c).
Let us now write down exact FRG flow equations for the self-energies of our model in our interaction-momentum cutoff scheme. The derivation of these flow equations is straightforward following the general procedure outlined in Ref. [Kopietz10, ]. The cutoff-dependent fermionic self-energy satisfies
[TABLE]
while the flow of the bosonic self-energy (which can be identified with the renormalized particle-particle bubble) is given by
[TABLE]
Here is the bosonic single-scale propagator, which for our sharp interaction-momentum cutoff scheme is simply given by
[TABLE]
A graphical representation of Eqs. (52) and (53) is shown in Fig. 7.
Note that in our interaction-momentum cutoff scheme only diagrams with bosonic single-scale propagators appear in the flow equations. For this simplification we pay the price that we have to start the FRG flow with a non-trivial initial condition, as explained above.
The right-hand sides of the flow equations (52) and (53) for the self-energies depend on higher order vertices with three and four external legs for which we can derive again exact FRG flow equations. The flow equations for the three-point vertices are
[TABLE]
A graphical representation of Eqs. (55) and (56) is shown in Fig. 8.
Next, consider the bosonic four-point vertex which controls the FRG flow of the bosonic self-energy in Eq. (53). Recall that in our interaction-momentum cutoff scheme this vertex, which describes the induced interaction between fluctuations of the superfluid order parameter, has a finite initial value at given by the symmetrized fermion loop in Eq. (48). The FRG flow equation for the bosonic four-point vertex is (see Fig. 9)
[TABLE]
where we have introduced the following product rule notation,
[TABLE]
To conclude this section, let us briefly discuss the flow equations of the induced interactions which vanish at the initial cutoff scale: the mixed fermion-boson vertex and the induced fermionic interactions and which appear in the vertex expansion (43) and are represented by the symbols defined in Fig. 3 (a) and (b). The exact FRG flow equations for these vertices are rather complicated and are given in Appendix B. Because the right-hand sides of the flow equations for the mixed fermion-boson vertex and for the fermionic interaction vertex are finite even if the above four-point vertices are neglected, the FRG flow generates finite values of these induced interactions. An approximate method to take these induced interactions into account is to retain only those vertices in the FRG flow equations which are finite at the initial scale. In Ref. Sharma16, we have obtained reasonable results using a similar strategy to truncate the hierarchy of FRG flow equations for the vertices in a low-energy model for graphene. Following this strategy, we arrive to the simplified FRG flow equations for the induced interactions shown graphically in Fig. 10. Note that the induced interaction between fermions with parallel spin still vanishes within this approximation.
In Appendix E we present an approximate evaluation of the flow equation for the mixed four-point vertex shown in Fig. 10 (a) and study the effect of this vertex on the fermionic self-energy. At this point, let us make three comments on the truncated flow equations of the induced interactions shown in Fig. 10. First of all, if we replace the boson propagators in the approximate flow equation for the fermionic interaction vertex shown in Fig. 10 (b) by the -matrix and neglect all self-energy corrections to the fermionic propagators, we recover the leading term in the perturbative expansion of this interaction vertex shown in Fig. 5 (b). Note, however, that within our interaction-momentum cutoff scheme this vertex does not directly couple to the FRG flow of the bosonic self-energy. The corresponding renormalization of the critical temperature is taken into account via the bosonic six-point vertex, as explained in the text after Eq. (51).
Next, we note that for small values of the scattering matrix we can use these flow equations to calculate higher order vertex corrections to various physical quantities. For example, from the truncated flow equation for the mixed fermion-boson vertex shown in Fig. 10 (a) it is obvious that this vertex is at least of order . From the exact flow equations for the three-point vertices shown in Fig. 8 we then see that the latter are at least of order .
Finally, let us point out that the induced interactions can exhibit some rather complicated momentum- and frequency dependence. Only in cases where this can be neglected, one can try to avoid the appearance of the induced interactions by redefining the bosonic Hubbard-Stratonovich fields and . This strategy, which has been called dynamical re-bosonization Gies02 , was adopted by Floerchinger et al. Floerchinger08 who attempted to reproduce the GM correction to the critical temperature using this strategy. However, the numerical value of the GM correction is determined by the full momentum dependence of the induced interaction in (B5), so that it is not surprising that Floerchinger et al. Floerchinger08 could not reproduce the precise numerical value of the GM correction given in Eq. (39).
IV Density of states and quasiparticle damping
in the normal state close to
In this section, we shall consider the effect of superfluid fluctuations on the electronic self-energy in the normal state at and slightly above the critical temperature. This effect is usually neglected Larkin05 , which is only correct for temperatures not too close to . Surprisingly, a quantitatively accurate calculation of the electronic self-energy in this regime cannot be found in the literature. Although such a theory is currently needed in other contexts, e.g. temporal development of an order parameter following a sudden quench in the field of out-of-equilibrium dynamicsYuzbashyan06 ; Yuzbashyan09 ; Straeter12 . To begin with, we analyze this problem in Sec. IV.1 within the Gaussian approximation for the propagator of the superfluid order parameter field. However, the critical behavior of the superfluid order parameter belongs to the XY-universality class, which below four dimensions is controlled by the Wilson-Fisher fixed point. In Sec. IV.2 we shall therefore present a more accurate analysis of this problem using the FRG approach developed in Sec. III.
IV.1 Gaussian approximation
To begin with, let us calculate the electronic self-energy within the Gaussian approximation, which is equivalent to calculating the effective interaction in ladder approximation. In the normal state the self-energy is then given by
[TABLE]
where the Gaussian propagator of the pairing field is given in Eq. (20). Since we are interested in the effect of long-wavelength and low-energy order parameter fluctuations on the fermionic self-energy, we may expand the inverse Gaussian propagator to leading order in momenta and frequencies,
[TABLE]
In the BCS regime and for the dimensionless parameter can be identified with the reduced temperature
[TABLE]
while the momentum scale and the energy scale are both proportional to the temperature Larkin05
[TABLE]
Note that can be identified with the coherence length of a clean three-dimensional superconductor with isotropic Fermi surface Larkin05 . The Ginzburg-Levanyuk number introduced in Eq. (1) can be written as Larkin05
[TABLE]
On the other hand, in the strong coupling regime where is not small the coefficients in the long-wavelength expansion of have a more complicated dependence in and , as discussed in Appendix C. In particular, at the unitary point the momentum scale is of the order of while is of order . Note that the corresponding expressions given by Larkin and Varlamov Larkin05 are only valid in the BCS limit .
Let us now focus on the effect of classical long-wavelength fluctuations of the superfluid order parameter on the fermionic self-energy. Because in the vicinity of the critical temperature the dynamics of the order parameter is slow compared with the electron dynamics, it is then sufficient to retain only the contribution from the zeroth Matsubara frequency in Eq. (59). In Appendix D we present a formal justification of this approximation. The resulting critical contribution to the fermionic self-energy is
[TABLE]
where the cutoff takes into account the range of validity of our long-wavelength expansion (60). Eq. (65) can be evaluated analytically without further approximation, but the result is very complicated so that we do not present it here. In Fig. 11 we plot the corresponding renormalized density of states
[TABLE]
Obviously, for classical pairing fluctuations give rise to a pronounced pseudogap in the density of states at the Fermi energy. This has already been noticed by Di Castro et al. in Ref. [DiCastro90, ] within a perturbative approach which amounts to expanding the right-hand side of Eq. (66) to first order in the self-energy. With this approximation Di Castro et al. obtained for the density of states at the Fermi-energy DiCastro90
[TABLE]
This suppression of the density of states has been observed experimentally in the fluctuation regime above the superfluid transition of a strongly interacting Fermi gasGaebler10 . However, for the correction in Eq. (67) diverges. Clearly, this divergence is unphysical and signals the breakdown of perturbation theory for temperatures close to . In contrast to the perturbative result (67) our expression (66) obtained within the Gaussian approximation predicts a finite suppression of the density of states for all . To show this, we have evaluated Eq. (66) numerically for different temperatures. In Fig. 12. and show our numerical result for as a function of . Note that at the critical point the Gaussian approximation (66) predicts a finite suppression of the density of states at the Fermi energy.
The phenomenon that within perturbation theory superconducting fluctuations above give rise to singular corrections to various physical quantities has first been noticed by Aslamazov and Larkin Aslamazov69 , who discovered a singularity in the conductivity of normal metals due to virtually formed Cooper pairs above . Moreover, Maki Maki68 and ThompsonThompson69 have shown that Cooper pair formation along diffusive paths in a disordered conductor also lead to singularities in the the transport coefficients. Although the Maki-Thompson correction to the conductivity has generally a weaker functional dependence on the reduced temperature , in certain regimes it can be larger than the Aslamazov-Larkin correction. However, similar to the singularity in the density of states given in Eq. (67), the perturbatively generated singularities at should be regularized by some higher order process. The only systematic way of introducing a cutoff at so far is an external pair-breaking mechanism, such as magnetic impurities or electron-phonon interactions.Keller71 There were a few attempts to identify a cutoff at within the microscopic theory itself: by accounting for some subclasses of higher order diagramsPatton71 and by accounting for non-linear effects of the fluctuations through Gorkov equationLarkin72 , at least in dirty superconductors. But the results are still inconclusive. Here we focus on the singularity in the density of states and propose a new strategy to solve this long-standing problem using renormalization group methods. In fact, from Fig. 12 it is clear that the singularity in the perturbative result (67) can be removed if we do not expand the density of the states in powers of the self-energy but insert the perturbative self-energy into the Dyson equation and use Eq. (66) to calculate the density of states.
To gain a better analytical understanding of the low-energy behavior of the self-energy, let us simplify the integrand in Eq. (65) by setting and assuming . We may then approximate . We have verified numerically that this approximation correctly reproduces the main low-energy features of the self-energy. After analytic continuation () we obtain from Eq. (65) for the imaginary part for and ,
[TABLE]
To calculate the real part of the self-energy for and we first perform the angular integration in Eq. (65) and obtain
[TABLE]
In the regime we may set and move the upper limit of the - integral to infinity. Using the fact that for ,
[TABLE]
we obtain for ,
[TABLE]
In the opposite regime we may expand the logarithm for ,
[TABLE]
Then we obtain to leading order
[TABLE]
Note that in both regimes the imaginary part of the self-energy is parametrically larger than the real part, so that from now on we shall simply neglect the real part of the self-energy.
Our result (68) for the imaginary part of the self-energy due to classical fluctuations of the superfluid order parameter implies that for the damping of quasiparticles on the Fermi surface diverges as
[TABLE]
While within the Gaussian approximation the density of states is finite, the quasiparticle damping exhibits an unphysical logarithmic singularity for . In the BCS regime the logarithm is multiplied by a small prefactor , while in the vicinity of the unitary point where the prefactor is linear in the temperature, such that
[TABLE]
Comparing the above with the generic form of the quasiparticle damping in a three-dimensional Fermi liquid,
[TABLE]
where the numerical constant is usually of the order of unity Kittel66 ; Thouless77 , we conclude that for the contribution from classical superconducting fluctuations to the quasiparticle damping dominates.
It turns out, however, that the logarithmic divergence in Eq. (74) is an artifact of the Gaussian approximation. Physically, it is clear that both the damping of the intermediate states as well as the existence of an anomalous dimension of the superfluid order parameter field will smooth out this singularity. For example, to take into account the usual Fermi liquid damping (76) we should replace the free propagator in Eq. (59) by
[TABLE]
Then we obtain for instead of Eq. (74),
[TABLE]
which is proportional to in the BCS regime. A similar sub-leading non-analytic correction to the self-energy of three-dimensional Fermi liquids is also generated by short-range interactions Chubukov06 . Note, however, that Eq. (78) does not take into account that the anomalous dimension of superfluid fluctuations at the critical point. Recall that critical behavior of the superconduting transition belong to the universality class of the classical XY-model which is characterized by a finite critical exponent (anomalous dimension) in three dimensions [Pelissetto02, ]. The true static propagator of the order-parameter field at is therefore for small momenta of the form
[TABLE]
where is a dimensionless constant. If we replace the Gaussian propagator in Eq. (65) by Eq. (79) we obtain for the self-energy at the critical point,
[TABLE]
From this expression it is easy to show that
[TABLE]
Due to the small value of , the prefactor of the leading -behavior is unusually large. Of course, the above procedure is not satisfactory because it does not self-consistently take the interplay between critical fluctuations and quasiparticle damping of intermediate states into account. We shall address this problem below using the FRG. This allows us to consistently take into account the feedback of non-Gaussian critical order parameter fluctuations on the electronic properties, which provide an intrinsic cutoff of the logarithmic singularity in the quasiparticle damping encountered in Gaussian approximation, see Eq. (74).
IV.2 FRG calculation of the quasiparticle damping
The exact FRG flow equation of the fermionic self-energy is given in Eq. (52) and is shown graphically in Fig. 7 (a). This flow equation depends on the cutoff-dependent mixed fermion-boson interaction and on the three-point vertices and . In this subsection we shall neglect all vertices which vanish at the initial cutoff scale within our cutoff scheme. In particular, we set the mixed fermion-boson interaction vertex equal to zero,
[TABLE]
From the exact FRG flow equations (55, 56) for the three-point vertices shown graphically in Fig. 8 it is obvious that in our interaction-momentum cutoff scheme this truncation is consistent with approximating the three-point vertices by their initial values,
[TABLE]
see Eq. (46). In Appendix E we shall use a more elaborate truncation strategy where the RG flow of the three-point vertices , and the mixed four-point vertex is regained. However, our main result for the quasiparticle damping derived in this subsection is not qualitatively modified by the higher order vertex corrections represented by the RG flow of , , and .
Since we are interested in the effect of classical critical fluctuations, we retain only the contribution from the zeroth Matsubara frequency to the right-hand side of the flow equation (52). After analytic continuation to the real frequencies we obtain the following FRG flow equation for the fermionic self-energy,
[TABLE]
We approximate the flowing static single-scale propagator by its long wavelength limit
[TABLE]
The parameters and are determined by the FRG flow equation (53) for the bosonic self-energy shown graphically in Fig. 7 (b). Since we are only interested in classical fluctuations we may set all Matsubara frequencies equal to zero in these equations and obtain
[TABLE]
Note that the parameter is related to the scale-dependent anomalous dimension of the superfluid order parameter field as follows Kopietz10
[TABLE]
Our truncated FRG flow equation (84) therefore contains both the effect of the anomalous dimension of the superfluid order parameter and the damping of intermediate states. In fact, our evaluation of the self-energy in Gaussian approximation presented in Sec. IV.1 shows that critical fluctuations mainly renormalize the imaginary part of the self-energy. We therefore ignore the real part of the self-energy in Eq. (84) and focus on the FRG flow of its imaginary part on the Fermi surface,
[TABLE]
This quasiparticle damping is determined by the flow equation
[TABLE]
Assuming we may linearize the energy dispersion around the Fermi surface, . In three dimensions, the angular integration is then elementary and we obtain for the flow of the quasiparticle damping on the Fermi surface,
[TABLE]
where
[TABLE]
To obtain the self-consistent quasiparticle damping from Eq. (91), we need additional RG flow equations for the two parameters and . Within our classical approximation this flow is determined by Eqs. (86) and (87) which depend on the induced interaction between classical order parameter fluctuations. Note that in our interaction-momentum cutoff scheme the FRG flow of all vertices without fermionic external legs is completely decoupled from the FRG flow of the other vertices with fermionic legs so that we may use the strategy developed in Refs. [Ledowski04, ; Hasselmann04, ] to obtain a closed systems of RG flow equations for and . In a first step, we define
[TABLE]
and neglect the momentum-dependence of on the right-hand sides of the flow equations (86) and (87). In this approximation does not flow and the RG flow of is
[TABLE]
To obtain the RG flow of the interaction , we neglect again the momentum-dependence of the four-point vertices on the right-hand side of the flow equation (57) for the induced interaction between order parameter fluctuations and obtain
[TABLE]
where we have also neglected the flow of the six-point vertex. Actually, as discussed in Sec. III, within our cutoff scheme the GM correction to the critical temperature can be obtained by calculating the effect of the initial value of the six-point vertex on the bosonic self-energy to second order in the Gaussian propagator of the order parameter field, see Fig. 6 (c). In our FRG approach this contribution can be simply taken into account via the initial condition , where the value of includes the GM correction. Finally, to obtain the RG of and the associated flowing anomalous dimension from Eq. (88), we need the momentum-dependence of the induced interaction , which is determined by the exact FRG flow equation (57) shown graphically in Fig. 9. Following Refs. Ledowski04, ; Hasselmann04, , we obtain an approximate solution of this flow equation by neglecting the flowing six-point vertex as well as the momentum-dependence of the four-point vertices on the right-hand side. Moreover, since we are interested in classical order parameter fluctuations, we only need the classical component of the interaction which can be obtained by setting all external Matsubara frequencies in our exact flow equation (57) equal to zero. With these approximations we obtain for the momentum-dependent induced interaction between order parameter fluctuations,
[TABLE]
where
[TABLE]
Integrating Eq. (96) over the flow parameter we find for the induced two-body interaction between classical superfluid fluctuations
[TABLE]
Recall that in our cutoff scheme the initial value of the induced interaction is given by the symmetrized closed fermion loop defined in Eq. (48) (see also Fig. 6 (a)), which is momentum-dependent. Substituting Eq. (98) into our flow equation (87) for the coupling we find for the flowing anomalous dimension defined in Eq. (88),
[TABLE]
From the explicit expression for the initial interaction in Eq. (48) we obtain for the estimate
[TABLE]
where is a numerical constant of the order of unity and is given in Eq. (49). It is then easy to see that the first term in Eq. (LABEL:eq:etares1) cannot modify the fixed point limit of for , so that from now on we shall omit this term. The resulting system of coupled RG flow equations for the three couplings , and is then formally identical to the system discussed in Refs. Ledowski04, ; Hasselmann04, . Introducing the logarithmic flow parameter , the RG flow of the dimensionless rescaled couplings
[TABLE]
is given by
[TABLE]
The scale-dependent anomalous dimension satisfies the integral equation
[TABLE]
where the kernel can be expressed in terms of the dimensionless function
[TABLE]
as follows,
[TABLE]
Here and denote the first and the second derivative of .
At the critical temperature the rescaled couplings , , and approach finite limits for . In Fig. 13 we plot the flow of , , and for two different values of the critical temperature as an example. Within our simple truncation the fixed point values are Ledowski04 ; Hasselmann04
[TABLE]
Note that the fixed point value of the anomalous dimension is larger than the accepted value for the XY-universality class in three dimensions Pelissetto02 , this discrepancy can be significantly reduced using more sophisticated truncation strategies Hasselmann04 ; Berges02 of the FRG flow equations. For our purpose, the simple truncation strategy described above is sufficient.
Given the RG flow of the rescaled quantities , , and , we can reconstruct the flow of the dimensionful relevant coupling and of the marginal coupling
[TABLE]
which we need for calculating the quasiparticle damping from the flow equation (91).
By solving the coupled flow equations (103), (104), and (105) for various temperatures and using the result as an input for the flow equation (91) for the quasiparticle damping we obtain the quasiparticle damping as a function of the temperature. Our numerical result for the damping as a function of the critical temperature is plotted in Fig. 14.
In the weak coupling regime the quasiparticle damping due to classical critical fluctuations is described by the interpolation formula
[TABLE]
where the numerical value of the prefactor is
[TABLE]
Using Eq. (64) to express the the logarithm in Eq. (110) in terms of the Ginzburg-Levanyuk number we can express the quasiparticle damping due to critical fluctuations in the form (2) given in the introduction.
The appearance of the logarithm in Eq. (110 is related to the logarithmic divergence of the quasi-particle damping encountered in Gaussian approximation, see Eq. (74). Note that the numerical value of the prefactor is rather large. Although the precise numerical value of given above is an artifact of our truncation scheme, we show in Appendix E that a more sophisticated truncation including the RG flow of the three-point and mixed four-point vertices confirms the validity of Eq. (110) with a prefactor which is still large compared with unity.
The above results should be compared with the well known quadratic low-temperature behavior of the quasi-particle damping in a three-dimensional Fermi liquid, see Eq. (76). At the Fermi liquid damping is
[TABLE]
where the numerical value of depends on the strength of the screened interaction but is usually close to unity Kittel66 . Although for sufficiently small the Fermi liquid damping is always larger than the damping due to critical superconducting fluctuations discussed above, due to the large prefactor in Eq. (110) there is a substantial temperature regime where the damping due to critical fluctuations dominates. Note also that short-range interactions in Fermi liquids give rise to a non-analytic correction of the form (110), see Ref. [Chubukov06, ]. However, the corresponding prefactor is or order unity, so that the numerical value of the prefactor of the non-analytic -contribution to the quasi-particle damping at is dominated by classical critical fluctuations. Moreover, for for the quasi-particle damping due to classical critical fluctuations is a decreasing function of temperature, as shown in Fig. 15.
This is very different from any perturbative correction to the quasi-particle damping, which usually increases with temperature. The fact that the contribution from classical critical fluctuations to grows as the temperature is lowered is closely related to the logarithmic divergence of the damping for encountered within the Gaussian approximation, see Eq. (74). Note that, in contrast to the result for the Gaussian approximation, our FRG result for the damping approaches a finite limit for , as given in Eqs. (110). The decrease of relaxation rates with temperature as one moves away from the critical point has also been observed for disordered metals above the superconducting transitionLarkin05 . In Fig. 16 we illustrate the regime in the plane spanned by the interaction length (which we parametrize by ) and the temperature where the damping due to classical pairing fluctuations obtained from our FRG approach is larger than the Fermi liquid damping , see Eq. (76). Obviously, the colorful area where this condition is fulfilled is is sizable even for rather small values of the interaction.
Finally, let us point out that our result (110) for the quasiparticle damping due to classical critical fluctuations is not qualitatively modified by vertex corrections. In Appendix E we present an improved truncation of the FRG flow equations where we retain, in addition to the purely bosonic vertices in Eqs. (103-105) and the fermionic self-energy in Eq. (91), the three-legged vertices , , as well as the mixed four-legged vertex . From the numerical solution of the extended set of the flow equations we can confirm the validity of Eq. (110) with a modified prefactor , which is still large compared with unity.
V Summary and conclusions
In this work we have used functional renormalization group methods to study the effect of static pairing fluctuations on the electronic properties of metals in the critical (Ginzburg) region above the superconducting transition temperature. Our approach is based on partial bosonization of the electron-electron interaction in the particle-particle channel and the application of FRG methods to the resulting mixed Bose-Fermi model within a special cutoff scheme where a regulator is introduced only in the bosonic sector (interaction-momentum cutoff scheme). To illustrate the efficiency of our approach, we have re-derived in a simplified way the correction to obtained by Gorkov and Melik-BarkhudarovGorkov61 by identifying with the temperature where the gap of the inverse bosonic propagator vanishes. Moreover, we have shown, within our more streamlined approach, that this correction to is changed by a numerical factor when the chemical potential is fixed instead of the particle density. Another advantage of our approach is that it allows us to understand the emergence of various types of induced interaction vertices involving pairing fluctuations from the renormalization group point of view.
We have then used our powerful method to study the effect of critical pairing fluctuations on the electronic single-particle excitations in the normal state, especially on the electronic density of states and on the damping of quasiparticles with momenta on the Fermi surface. Within the Gaussian approximation (which corresponds to the ladder or -matrix approximation for the effective two-body interaction) we have found an (up to now unnoticed) logarithmic divergence of the quasiparticle damping for , while the density of states exhibits a finite pseudogap. At this level of approximation a finite value of can only be introduced by invoking other interaction processes, for instance inelastic electron-electron collisions within Fermi liquid theoryKittel66 that are further enhanced by disorder present in real materials due to the weak localization effectAltshuler82 ; Altshuler85 ; Altshuler85_2 . The logarithmic divergence of encountered in Gaussian approximation implies that Gaussian pairing fluctuations completely destroy the Fermi liquid behavior of the single-particle Green function at and slightly above the critical temperature. In view of the fact that in three dimensions the critical fluctuations of the pairing field are not controlled by the Gaussian fixed point this is perhaps not so surprising. Note also that for , i.e. in the superfluid phase, order parameter fluctuations are known to have a strong effect on the single-particle properties. For example, in Ref. Lerch08, it has been shown that at Gaussian fluctuations of the pairing field give rise to a logarithmic suppression of the quasiparticle residue and the density of states.
Given the fact the Gaussian approximation is not sufficient, we have used the FRG to take the non-Gaussian nature of critical pairing fluctuations into account, which is the main technical part of our work. Let us point out that this approach should also be useful for a systematic evaluation of corrections to the Gaussian approximation in other cases where the dominant scattering channel between electrons can be uniquely identified on physical grounds. It is then convenient to treat the dominant channel non-perturbatively using a suitable Hubbard-Stratonovich field, so that the Gaussian approximation for this field amounts to solving a single-channel Bethe-Salpeter equation for the effective interaction. Other scattering channels and the corresponding vertex corrections can then be taken into account approximately via the induced interaction vertices which are generated as we integrate the FRG flow equations. A similar strategy is adopted by the dynamical re-bosonization method Gies02 , which is, however, restricted to situations where the momentum- and frequency dependence of the induced interactions can be neglected.
In the fluctuation regime just above our FRG approach gives a finite relaxation rate of the fermionic quasiparticles, which increases down to the transition temperature but remains finite at the transition point, , where the numerical constant is large compared with unity. Physically, the corresponding finite lifetime of quasiparticles on the Fermi surface is due to collisions between the unpaired fermions and virtually formed Cooper pairs associated with critical pairing fluctuations. This is similar to the effect of a disorder potential on the phase coherence of quasi-particles in dirty systemsAltshuler98 ; Aleiner99 ; Narozhny02 , where limited applicability of the ergodicity hypothesis makes direct observation of some of the coherence effects harderTsyplyatyev03 ; Falko04 .
It is tempting to associate with the phase breaking time due to the Anderson’s theoremAnderson59 , which is applicable to the s-type superconductor studied in the present work. However, its manifestation in the particle-particle (fluctuation) propagator has only been studied within the ladder approximation, see Ref. [Abrikosov59, ] and a comprehensive book by Larkin and VarlamovLarkin05 . The finite quasi-particle lifetime obtained in Eq. (110) requires essentially a beyond ladder approach, i.e. renormalization of the bosonic line in the second term in Fig. 7(a) corresponds to a sum over the ladder diagrams in Eq. (4.1) but renormalization of the fermionic line accounts for more diagrams of a different type; here we refer to the analysis in Subsec. IIIB where the first term in Fig. 7(a) is neglected. Thus, the two-particle correlation function would need to be calculated using the approach developed in this paper in order to put such an interpretation on a solid ground, which could be a subject of a future work.
At higher temperatures above the Fermi liquid damping Kittel66 ; Thouless77 becomes larger, but close to the transition temperature there is a finite region where the damping in clean systems is dominated by critical fluctuations, as shown in Fig. 16. To be specific, we estimate that the effect of critical pairing fluctuations can be seen if the critical temperature is larger than . With eV this gives K, so that the contribution of critical pairing fluctuations to the quasiparticle damping should be observable in superconductors with K.
Our approach also provides a microscopic and fully consistent theory for the pseudogap in a clean electronic system originating from the superconducting fluctuations only. The density of states in Eq. (66) evaluated using the result of the FRG in Eq. (89) is significantly different from the Gaussian approximation in Eq. (65). The former result predicts a partial suppression of the density of states at the Fermi energy and a finite quasi-particle relaxation rate down to the point of the superconducting transition. Fitting the result of our numerical integration of the FRG equations in subsection APPENDIX E: FRG calculation with vertex corrections, we find for the leading order behavior for the density of states at the Fermi level in the weak coupling regime,
[TABLE]
This functional dependence of the pseudogap strength on should be observable in clean superconductors with higher , which transition temperatures exceeding our estimate for given above.
Generally, the effect of critical pairing fluctuations on the electronic spectrum is most pronounced in strongly coupled superconductors with small coherence length and broad fluctuation regimes, corresponding to Ginzburg-Levanyuk numbers of the order of unity. For instance, this regime should be relevant for the normal state of the cuprate superconductors,Dagatto94 ; Basov05 ; Devereaux07 ; Fischer07 ; Alloul09 ; Armitage10 which exhibits a pseudogap and a linear temperature dependence of the quasiparticle damping, in agreement with our prediction. Another class of fermionic superfluids where fluctuation effects can be studied experimentally are ultracold gases of fermionic atoms or molecules. In these systems the effective two-body interaction can be controlled using the Feshbach-resonance technique Bloch08 . In particular, in the vicinity of the unitary point where the scattering length diverges, fluctuation effects above are expected to be most pronounced. It should be interesting to extend the calculations for the quasi-particle damping and the pseudogap presented in this work to the unitary point and discuss the BCS-BEC crossover of these quantities.
acknowledgements
We thank Andrey Varlamov for many useful discussions and for his insightful suggestions and comments on the manuscript. We also thank Casper Drukier for his contributions at initial states of this work and acknowledge financial support by the DFG through SFB/TRR 49 and FOR 723.
APPENDIX A: Interaction corrections to the particle-particle
bubble
The self-energy of the pairing field introduced in Eq. (8) can be identified with the renormalized particle-particle bubble. In this appendix we will explicitly evaluate the regularized non-interacting bubble defined in Eq. (21) and the first two interaction corrections and given in Eqs. (27) and (28) for vanishing total momentum and energy.
Consider first the non-interacting particle-particle bubble defined in Eq. (9). After performing the Matsubara sum and setting we obtain
[TABLE]
where , is the Fermi function, and we have defined the integration symbol . The ultraviolet cutoff restricts the momentum integration to the regime . We assume that the external momentum satisfies so that the shift in the integration variable in the third line of Eq. (A1) does not affect the cutoff. At the integral in the last line of Eq. (A1) can be transformed to a dimensionless form by substituting ,
[TABLE]
where , , and is the density of states at the Fermi energy per spin projection. We focus on the BCS regime where . The asymptotic behavior of this integral for can then be extracted following the procedure outlined by GM Gorkov61 and we finally obtain
[TABLE]
with the numerical constant , see Eq. (31). If we subtract from the vacuum bubble defined in Eq. (18) the cutoff-dependent term on the right-hand side of (A3) is canceled so that we may take the limit and obtain the low-temperature asymptotics of the regularized particle-particle bubble given in Eq. (30).
Next, let us evaluate the second order correction to the particle-particle bubble arising from the induced interaction in the particle-hole channel, which according to Eq. (28) can we written as
[TABLE]
where the non-interacting particle-hole bubble is defined in Eq. (25). It turns out that this integral is still ultraviolet divergent so that we introduce again an ultraviolet cutoff as in Eq. (A1). Following GM, we simplify the integrand in Eq. (A4) as follows:
Neglect the frequency dependence of the particle hole bubble,
[TABLE] 2. 2.
Project the momentum dependence of the particle-hole bubble onto the Fermi surface,
[TABLE]
where is the point on the Fermi surface closest to .
By numerically evaluating Eq. (A4) we have explicitly verified that the above approximations do not modify the prefactor of the leading dependence of given in Eq. (36), which determines the fluctuation correction to in the weak coupling limit. With these approximations the second order correction (A4) to the particle-particle bubble reduces to
[TABLE]
The particle-hole bubble is given by
[TABLE]
At zero temperature and in the static limit this reduces to
[TABLE]
where and is the density of states at the Fermi energy. Setting
[TABLE]
where is the angle between and , we may expand in Legendre polynomials ,
[TABLE]
where
[TABLE]
Actually, the integration in Eq. (A7) projects out the component so that under the integral sign we may replace by its angular average
[TABLE]
where the numerical constant is given in Eq. (37). The second order correction to the particle-particle bubble then reduces to
[TABLE]
as given in Eq. (36) of the main text. The cutoff-dependence in Eq. (A14) is an artifact of the approximation (A6); if we do not project the momenta onto the Fermi surface, the resulting integral in Eq. (A4) depends only logarithmically on the ultraviolet cutoff, which follows from the fact that for large the static polarization vanishes as .
Finally, let us evaluate the term defined in Eq. (27), which contributes to the shift of if we fix the chemical potential instead of the density. Therefore we manipulate the right-hand side of Eq. (27) for as follows,
[TABLE]
where we have integrated by parts to express the integral in terms of the derivative of the energy-dependent density of states . Using the fact that in dimensions the density (per spin projection) can be related to the density of states at the Fermi energy as , we obtain in three dimensions to leading logarithmic order
[TABLE]
in agreement with Eq. (34).
APPENDIX B: FRG flow of induced interactions
The vertex expansion (43) of the generating functional of the irreducible vertices contains four different types of four-point vertices, which are defined graphically in Fig. 3. In our interaction-momentum cutoff scheme, only the effective two-body interaction between superfluid fluctuations shown in Fig. 3 (d) is finite at the initial scale. The exact FRG equation for this vertex is given in Eq. (57) and is shown graphically in Fig. 9. In this appendix, we give the exact FRG flow equations for the other three induced interaction vertices shown in Fig. 3.
In Fig. 17 we show a graphical representation of the exact FRG flow equation of the induced fermion-boson interaction vertex in our interaction-momentum cutoff scheme.
For our purpose, we need only a truncated version of this flow equation where all vertices which vanish at the initial scale are neglected on the right-hand side of the flow equations. In this limit we obtain the FRG flow equation shown graphically in Fig. 10 (a), which is explicitly given by
[TABLE]
Here we have used the product rule notation introduced in Eq. (58),
[TABLE]
Next, consider for completeness the FRG flow equations for the two types of purely fermionic induced interaction vertices defined in Fig. 3 (a) and (b). Since these flow equations are rather lengthy, we do not explicitly write them down here but represent them graphically in Fig. 18 and Fig. 19.
We can close the infinite hierarchy of FRG flow equations by neglecting all vertices with more than four external legs on right-hand side. Then the FRG flow equation for the induced interaction between two electrons with opposite spin reduces to
[TABLE]
while the flow of effective interaction between electrons with parallel spin is given by
[TABLE]
As a first step in an iterative solution of these flow equations, we may set all vertices which vanish at the initial scale equal to zero. Then the FRG flow equation (B3) for the effective interaction between electrons with opposite spin reduces to
[TABLE]
which is shown graphically in Fig. 10 (b). Another approximation strategy is to replace the three-point and bosonic four-point vertices on the right-hand sides of the flow equations in Fig. 10 by their initial values and . Then the FRG flow of the mixed boson-fermion interaction reduces to
[TABLE]
while the induced interaction between fermions with opposite spin determined by the truncated flow equation
[TABLE]
APPENDIX C:
Particle-particle bubble at finite momentum and frequency
To calculate the expansion of the particle-particle bubble for small momenta and frequencies, it is convenient to expand in powers of external momenta and frequencies before carrying out the Matsubara sums. Therefore we write Eq. (A1) as
[TABLE]
In the book by Larkin and Varlamov Larkin05 one can find an approximate evaluation of Eq. (C1) in the regime where the momentum integral is dominated by states with energies close to the Fermi energy. In this regime the energy dependence of the density of states can be neglected so that we may approximate under the integral. Using the -matrix regularization defined via Eq. (21) we then obtain for the regularized particle-particle bubble
[TABLE]
where for a spherical Fermi surface in dimensions the Fermi surface average in Eq. (C2) is
[TABLE]
The Digamma function has the representation
[TABLE]
where is the Euler-Mascheroni constant. The numerical constant in the argument of the logarithm in Eq. (C2) has already been introduced in Eq. (31). Note that
[TABLE]
and that for large the Digamma function has the asymptotic expansion
[TABLE]
The mean-field critical temperature is determined by
[TABLE]
which yields the well-known weak-coupling result quoted in Eq. (32). Setting
[TABLE]
we see that in the weak coupling regime and for small momenta the inverse bosonic propagator can be written as
[TABLE]
The corresponding retarded propagator can be obtained via analytic continuation, . Assuming we may expand the Digamma functions in powers of frequencies and obtain for the inverse retarded propagator
[TABLE]
where
[TABLE]
and
[TABLE]
can be identified with the square of the inverse coherence length. In particular, in the static limit the Gaussian propagator of the pairing field can be written as
[TABLE]
The above expressions are only valid in the weak coupling BCS limit at low temperatures, where , , and . On the other hand, when is of the order of unity the energy dependence of the density of states cannot be neglected, so that Eq. (C2) is not valid. Setting for simplicity (which is sufficient for our purpose because we are only interested in classical long-wavelength fluctuations) we write the static propagator of the order parameter field as
[TABLE]
In the BCS limit we obtain from Eq. (C10)
[TABLE]
More generally, for arbitrary values of the coefficients and can be obtained directly from Eq. (C1). For the parameter which measures the distance to the critical point we obtain
[TABLE]
where the energy-dependent density of states (per spin projection) is in three dimensions given by
[TABLE]
Assuming and introducing the dimensionless integration variable we obtain to leading order in the reduced temperature ,
[TABLE]
where the dimensionless function is given by
[TABLE]
In the BCS limit where we may approximate and obtain , in agreement with Eq. (C8). A graph of the function is shown in Fig. 20.
Finally, consider the coefficient in Eq. (C14), which can be written as
[TABLE]
After carrying out the Matsubara sums we obtain
[TABLE]
with
[TABLE]
Here and are defined by the following fermionic Matsubara sums,
[TABLE]
A graph of the function is shown in Fig. 20. In the BCS limit where we obtain to leading order in dimensions
[TABLE]
APPENDIX D: Justification of the classical approximation
close to
To justify the static approximation for pairing fluctuations in the evaluation of the electronic self-energy given in Eq. (65) we go back to Eq. (59), introduce the spectral representation of the Gaussian pairing propagator, and explicitly carry our the Matsubara sum. Therefore it is useful to write the Gaussian pairing propagator as
[TABLE]
Given the fact that particle-particle bubble vanishes for large as we see that the corresponding resummed bubble vanishes also for large , so that it has a spectral representation
[TABLE]
The inverse relation is
[TABLE]
From the expansion (C10) we see that for small frequencies ,
[TABLE]
where in the BCS regime and , see Eqs. (C11) and (C12). The spectral function is therefore
[TABLE]
Substituting Eqs. (D1) and (D2) into Eq. (59) we may carry out the Matsubara sum and obtain
[TABLE]
Here is the Bose function and is the Fermi function. From this expression we can now justify the static approximation for temperatures close to . In this regime, the dynamics of the boson is much slower that the dynamics of the fermions because the typical value of the boson frequency is , whereas the typical value of the fermion energy is of order . In this regime we may approximate the Bose function by its classical limit and neglect the term and the constant . In this approximation
[TABLE]
By definition the frequency integral gives
[TABLE]
For we may approximate in the numerator so that we finally arrive at Eq. (65).
APPENDIX E: FRG calculation with
vertex corrections
In the FRG calculation of the quasi-particle damping presented in Sec. IV.2 we have set the mixed fermion-boson interaction equal to zero and ignored the FRG flow of the three-point vertices and . However, if we assume the usual Fermi liquid scaling in the fermionic sector and Gaussian critical scaling in the bosonic sector, it is easy to see that the coupling
[TABLE]
is relevant at the critical point with scaling dimension in three dimensions. In the above definition of it is understood that the bosonic momenta and frequencies are set equal to zero, while the fermionic frequency is analytically continued to the real axis and then set equal to zero with an infinitesimal imaginary part as indicated. Similarly, the coupling defined by
[TABLE]
has scaling dimensions and is therefore marginal in three dimensions. Hence, for the calculation of the feedback of critical order parameter fluctuations on the electronic properties, the RG flow of these two couplings has to be taken into account. If we neglect all other (irrelevant) vertices, the RG flow of is given by the truncated flow equation shown graphically in Fig. 10 (a), which is explicitly written down in Eq. (B1). Introducing the dimensionless rescaled couplings
[TABLE]
and the rescaled damping
[TABLE]
we find that Eq. (B1) reduces to
[TABLE]
Similarly, we obtain from the FRG flow equations for the three-point vertices given in Eqs. (55, 56) which are shown graphically in Fig. 10 (b),
[TABLE]
Taking into account the couplings and , we obtain from Eq. (52) for the flow of the quasiparticle damping,
[TABLE]
In terms of the rescaled couplings introduced above this can be written as
[TABLE]
The above system of flow equations should be integrated with the following initial conditions,
[TABLE]
The finite initial value of takes into account the usual Fermi liquid contribution to the quasi-particle damping which is not related to critical pairing fluctuations, see the discussion in Sec.IV.1. For our model defined in Eq. (3) second order perturbation theory in the regularized interaction yields for the quasiparticle damping at low temperaturesAbrikosov63
[TABLE]
More generally, we may use the generic form of the quasiparticle damping of a Fermi liquid [see Eq. (76)], where the value of the numerical constant is determined by all types of interaction processes into account, including those which are not included in our effective low-energy model (3). For simplicity we choose such that the initial condition for the rescaled damping is given by .
After solving the flow equations (103–105) in the bosonic sector for various temperatures, we may substitute the result into the flow equations (E6) and (E7) for the four-legged and three-legged vertices, and into the flow equation (E9) for the quasiparticle damping. In Fig. 21 we plot the flow of the rescaled couplings and as well as the rescaled quasiparticle damping for .
From the solution for the dimensionless rescaled damping we can reconstruct the physical quasiparticle damping due classical pairing parameter fluctuations as follows,
[TABLE]
where the subtraction of the initial condition is necessary to isolate the contribution from classical pairing fluctuations. The rescaled damping is proportional to for large , so that converges against a constant value, as shown in Fig. 22.
Our final result for the contribution from classical critical fluctuations to the quasi-particle damping at the is shown in Fig. 23, where we also show the corresponding expression without vertex corrections derived in Sec. IV.2.
Comparing the two curves we can see, that in the weak coupling limit the qualitative behavior is not modified by vertex corrections, while for larger values of the interaction (corresponding to ) vertex corrections do have a significant effect. One should keep in mind, however, that in the derivation of the flow equations (E6) and (E7) we have made several simplifications (for example, we have projected all external momenta of the vertices on the Fermi surface) which can only be expected to be quantitatively accurate in the weak coupling BCS regime. Hence, quantitative accuracy of our FRG calculation including vertex corrections can only be expected for . In this regime our FRG result for the quasiparticle damping shown in Fig. 23 can be fitted by
[TABLE]
with . The above weak-coupling result including vertex corrections confirms our result of Sec. IV.2 given in Eq. (110). Note, however, that vertex corrections reduce the numerical value of the prefactor from to , which is still large compared with unity. A controlled calculation of the precise numerical value of is beyond the scope of this work; in the calculation including vertex corrections of the numerical value of is also sensitive to the choice of the numerical coefficient in the expression for the Fermi liquid damping defining the initial condition for the FRG flow equations.
Finally, let us point out that our FRG calculation predicts that at the critical point the marginal part of the mixed four-point vertex defined in Eq. (E2) diverges logarithmically for vanishing cutoff , while the relevant part of the three-legged vertex approaches a finite value in this limit. To see this, we plot these un-rescaled couplings in Fig. 24 for as function of the logarithmic flow parameter . Our numerical result for is for small (corresponding to large of the form . The logarithmic growth of the vertex correction at can be understood analytically from the flow equation (E6), which implies that for large , where is the fixed point value of the anomalous dimension. In the limit of large the flow equation (E6) therefore reduces to
[TABLE]
The analytic solution to this inhomogeneous differential equation is given by . If we scale back to the physical coupling we find for large . The logarithmic divergence of a vertex correction associated with a marginal coupling at the critical point should not be surprising. Our FRG approach automatically takes care of this divergence and its feedback to the other scale-dependent couplings in the problem. The non-analytic form of the quasiparticle damping is not modified by this divergence.
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