Tracking Thermal-Induced Amorphization of a Zeolitic Imidazolate Framework via Synchrotron In Situ Far-Infrared Spectroscopy
Matthew R. Ryder, Thomas D. Bennett, Chris S. Kelley, Mark D. Frogley,, Gianfelice Cinque, Jin-Chong Tan
TL;DR
This study employs in situ far-infrared spectroscopy to investigate the thermal amorphization process of a zeolitic imidazolate framework, providing new insights into vibrational changes and the impact of temperature on its structure.
Contribution
It is the first to use in situ far-infrared spectroscopy to analyze thermal amorphization in a zeolitic imidazolate framework, revealing vibrational and structural insights.
Findings
Vibrational motion changes during amorphization
Temperature affects Zn-N tetrahedra structure
New insights into thermal amorphization process
Abstract
We present the first use of in situ far-infrared spectroscopy to analyze the thermal amorphization of a zeolitic imidazolate framework material. We explain the nature of vibrational motion changes during the amorphization process and reveal new insights into the effect that temperature has on the Zn-N tetrahedra.
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Taxonomy
TopicsAdvanced ceramic materials synthesis · Silicon Nanostructures and Photoluminescence · Nonlinear Optical Materials Research