Two-photon exchange interaction from Dicke Hamiltonian under parametric modulation
A. V. Dodonov

TL;DR
This paper demonstrates how to engineer two-photon exchange interactions in a circuit QED system with multiple qubits by using parametric modulation, providing both analytical and numerical insights for experimental realization.
Contribution
It introduces a method to generate two-photon exchange interactions in multi-qubit circuit QED systems through parametric modulation, with analytical and numerical validation.
Findings
Two-photon exchange interaction can be engineered via frequency modulation.
Analytic expressions are derived for weak atom-field coupling.
Numerical simulations confirm experimental feasibility.
Abstract
We consider the nonstationary circuit QED architecture in which a single-mode cavity interacts with N>1 identical qubits, and some system parameters undergo a weak external perturbation. It is shown that in the dispersive regime one can engineer the two-photon exchange interaction by adjusting the frequency of harmonic modulation to (approximately) , where is the average atom--field detuning. Closed analytic description is derived for the weak atom-field coupling regime, and numeric simulations indicate that the phenomenon can be observed in the present setups.
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Two-photon exchange interaction from Dicke Hamiltonian under
parametric modulation
A. V. Dodonov
Institute of Physics and International Centre for Condensed Matter Physics, University of Brasilia, 70910-900, Brasilia, Federal District, Brazil
Abstract
We consider the nonstationary circuit QED architecture in which a single-mode cavity interacts with identical qubits, and some system parameters undergo a weak external perturbation. It is shown that in the dispersive regime one can engineer the two-photon exchange interaction by adjusting the frequency of harmonic modulation to (approximately) , where is the average atom–field detuning. Closed analytic description is derived for the weak atom–field coupling regime, and numeric simulations indicate that the phenomenon can be observed in the present setups.
nonstationary circuit QED, Two-photon exchange interaction, Tavis-Cummings Hamiltonian, Dicke Hamiltonian
pacs:
42.50.Pq, 42.50.Ct, 42.50.Hz, 32.80-t, 03.65.Yz
I Introduction
The area of circuit Quantum Electrodynamics (circuit QED) has grown to embrace a plethora of architectures with different kinds of multi-level atoms and sophisticated assemblies of interconnected 3D and 1D resonators and waveguides paik ; you ; science ; rev1 ; APL ; rev2 ; nori2017 . Diverse designs incorporating up to tens of Josephson Junctions give rise to superconducting artificial atoms with distinct properties regarding the dissipation mechanisms and the structure of energy levels, however, all they share the capability of coherently coupling to the Electromagnetic (EM) field nor ; smith ; reagor ; wilson ; ofec ; wallr . Moreover, a single cavity mode can interact with several locally addressable artificial atoms 3at0 ; 3at1 ; 3at2 ; ann ; cle ; saito ; gam1 ; song or an ensemble of trapped ultracold atoms uatoms1 ; uatoms2 .
Many types of superconducting artificial atoms allow for real-time manipulation of the energy levels or the atom–field coupling strength majer ; ge ; ger ; ger1 ; v1 ; v2 ; v3 . Combined with the ability of in situ tuning the resonator’s frequency by external magnetic flux nori-n ; meta , such nonstationary circuit QED architectures give rise to a novel regime of light–matter interaction in which all the parameters in the Hamiltonian are controllable functions of time jpcs ; JPA . Using resonant perturbations one can induce creation and annihilation of photons or atomic excitations liberato9 ; roberto ; diego ; etc1 ; juan ; hoeb , generate entanglement entangles ; etc3 ; enta2 , induce new forms of light–matter interaction igor ; porras ; palermo ; tom , perform quantum simulations relativistic ; sim and study other novel effects etc2 ; processing ; ert ; ert2 . Some of the early proposals jpcs ; bla have recently been verified experimentally, such as the one-photon exchange between the qubit and the field in the dispersive regime (reliant on the ‘rotating’ terms in the interaction Hamiltonian) blais-exp ; simmonds and generation of two quanta from vacuum due to the ‘counter-rotating terms’ (CRT) schuster .
In this paper we describe another effect based on the rotating terms – the two-photon exchange interaction – that can be implemented in nonstationary circuit QED by modulating any system parameter with frequency , where is the average atom–field detuning. We illustrate the phenomenon for the case of off-resonant qubits described by the Dicke dicke ; HP or Tavis-Cummings TC1 ; TC2 Hamiltonians, however, our approach can be straightforwardly generalized to an arbitrary multilevel atom in the ladder configuration JPA . Assuming the weak atom–field coupling regime, we derive a closed analytic description of the unitary dynamics (see Sec. II) and find a good agreement with numeric data even for moderate coupling strengths (Sec. III). We also show that our proposal can be implemented in the current circuit QED setups with weak dissipation and slightly different atoms (Sec. III.1), and discuss manners to enhance the two-photon transition rate.
II Analytic results
Our system consists of a single mode of EM field interacting with qubits, as described by the quantum Dicke model dicke ; HP
[TABLE]
where the index labels the identical noninteracting atoms. We assume that the cavity frequency , the atomic transition frequency and the atom–cavity coupling strength are externally prescribed functions of time ( is considered real). and are the annihilation and creation operators and is the photon number operator. The qubit operators are , and , where and denote the ground and excited states of the -th qubit, respectively. In the absence of CRT the Hamiltonian (1) is known as Tavis-Cummings Hamiltonian TC1 ; TC2 . We stress that although our approach takes into account the CRT, the phenomenon described in this paper does not require their presence.
We consider the general case of simultaneous external modulation of all the system parameters as , where stands for , or (for the particular case of a single-parameter modulation, only one is nonzero). is the bare value, is the respective modulation depth, is the modulation frequency and is the initial phase. Moreover, we restrict our analysis to the perturbative regime when and .
To obtain closed analytical description we employ the normalized Dicke states with atomic excitations
[TABLE]
where the sum runs over all the allowed permutations of excited and non-excited qubits and . In the Dicke basis the Hamiltonian (1) reads
[TABLE]
where and .
We work in the dispersive regime, for all relevant values of , where is the bare atom–field detuning and is the total number of excitations. Following the approach described in JPA ; juan , we expand the system state as
[TABLE]
is a real oscillatory function
[TABLE]
where we defined the constant coefficients
[TABLE]
[TABLE]
[TABLE]
and assumed that for and all relevant values of , and .
is the effective eigenfrequency, where and are the -excitations eigenfrequencies and eigenstates (dressed states) of the bare Hamiltonian
[TABLE]
The index labels the different eigenvalues and eigenstates within the subspace of a given value of . is the frequency shift juan due to the counter-rotating terms in Eq. (3):
[TABLE]
[TABLE]
where we assumed . Lastly, is the slowly-varying probability amplitude for the dressed state .
Substituting (4) into the Schrödinger equation and neglecting the rapidly oscillating terms JPA , we obtain to the first order in , and
[TABLE]
where and
[TABLE]
. To obtain Eq. (12) we neglected frequency shifts smaller than , as well as the corrections of the order of for .
Under the resonant modulation frequency, , we get
[TABLE]
corresponding to the modulation-induced transition . We emphasize that, under the considered approximations, Eqs. (12) – (13) also describe the effective dynamics in the absence of CRT in the Hamiltonian (3), though in this case the frequency shift so that .
In the dispersive regime the spectrum of can be obtained from the standard perturbation theory. To the second order in one finds
[TABLE]
[TABLE]
where , , , and is the normalization constant ( is the cavity Fock state). Actually, to evaluate the two-photon transition rate one needs the eigenstates to the fourth order in , which are omitted here for brevity.
The two-photon exchange interaction chen ; alexanian ; chen2 corresponds to the transition , which represents (approximately) . To the lowest order in we obtain
[TABLE]
where . The corresponding resonant modulation frequency reads
[TABLE]
Notice that for a given value of the other states () are not affected by such modulation due to the condition , as can be seen from Eq. (12). So in the most common situation when the atoms are initially in the ground states (the Dicke state ) only the pair of states selected by the modulation frequency becomes coupled. On the other hand, if the atoms are prepared in a superposition of Dicke states, several states can become coupled by a single modulation frequency. For example, from Eq. (17) we see that to the second order in the same frequency couples the pair of states and ; we verified that for certain values of parameters this fact persists to the fourth order in as well.
III Numeric results
To check our analytic predictions we solved numerically the Schrödinger equation for the original Hamiltonian (1). In Fig. 1 we compare the exact numeric results, with and without CRT, to the approximate formulas (13) – (14). We plot the average number of photons and the average number of atomic excitations for the initial state and parameters , , , , , . As expected, the resonant modulation frequencies vary depending on whether the CRT are taken into account or not: with CRT and without CRT. The analytic and numeric results agree qualitatively, though there is a roughly difference in the analytic and actual transition rates . Such discrepancy is not surprising, since for the above parameters the required inequalities and are only barely satisfied foot1 . The apparent broad width of the curves is explained by fast low-amplitude oscillations due to the off-resonant photon exchange inherent to the dispersive regime, as inferred from the wavefunction (4) and the expression for the dressed states (II).
In Fig. 2 we consider a more realistic initial state , where stands for the cavity coherent state with [so that the initial probability of 5 photons is ]. For the sake of compactness we only present the exact numeric results in the presence of CRT. We set and consider the -modulation (with parameters , , , and ), as well as the simultaneous modulation of and with the additional parameters and (in this case ). These modulation frequencies were adjusted to promote the transition , and we defined (i. e., is the transition rate under the pure -modulation). We observe that excitations are transferred between the cavity and far-detuned atoms, and under the simultaneous - and -modulations the oscillations are roughly twice faster than under the sole -modulation, in agreement with Eq. (II).
To attest that the periodic behavior of and indeed corresponds to a two-photon exchange, in Fig. 3 we plot the probability of photons and the probability of atomic excitations under the simultaneous - and -modulations (discussed in Fig. 2). We observe that the main transition occurs between the states |\mathbf{0},5\rangle\and , although there are unwanted couplings between other states owing to the off-resonant one-photon exchange. As an example, we illustrate small oscillations between the states , inferred from the periodic oscillation of probabilities and at the same rate as the probabilities and .
III.1 Simulation under realistic conditions
The above numeric results apply to an ideal situation, namely, strictly identical atoms and dissipation-free environment. To asses the experimental feasibility of our proposal in circuit QED, we consider a realistic scenario of two slightly different artificial atoms coupled to a single-mode waveguide resonator under weak Markovian dissipation. The dynamics is now governed by the master equation
[TABLE]
[TABLE]
where is the total density operator and is the Liouvillian. To get a rough estimative we solved numerically the ‘standard’ phenomenological master equation bla for zero-temperature reservoirs foot2
[TABLE]
where is the Lindbladian superoperator. The constant parameters , and denote the cavity damping and the -th qubit’s relaxation and pure dephasing rates, respectively.
In Fig. 4 we compare the dynamics for the ideal and realistic scenarios under the -modulations and the initial cavity coherent state , where . For the realistic case we set: , , , , , , , and . For the ideal case , , and (the modulation frequencies were chosen to induce the transition ). Such parameters are compatible with the current circuit QED architectures, where typically GHz paik ; ger ; 3at0 ; 3at1 ; 3at2 ; saito ; reagor ; ofec ; schuster . We see that for initial times, s, the two-photon exchange can be proved via measurements of the average number of atomic excitations or the probabilities , and , whereas the measurement of the average photon number is of little help due to overwhelming effects of dissipation.
IV Conclusions
We showed analytically and numerically that effective two-photon exchange interaction between a single cavity mode and off-resonant qubits can be achieved by externally modulating any system parameter at frequency , where is the average atom–field detuning. This effect originates from the ‘rotating’ terms in the Dicke (or Tavis-Cummings) Hamiltonian, but the associated transition rate is quite small due to the multiplicative factor . Closed analytical description was derived under the assumption of weak atom–field coupling, and a good agreement with exact numeric results was observed even for moderate coupling strengths. For a simultaneous modulation of different parameters the transition rate can be increased by properly adjusting the initial phases. Regarding the experimental feasibility, we demonstrated that for our proposal can be implemented in the current circuit QED architectures on the timescales s, which could be further reduced through an increase in the modulation amplitudes, atom–field coupling strength or the number of qubits.
Acknowledgements.
The author acknowledges a partial support of the Brazilian agency CNPq (Conselho Nacional de Desenvolvimento Científico e Tecnológico).
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