Simple spin-orbit based devices for electron spin polarization
Y. Avishai, Y. B. Band

TL;DR
This paper introduces simple quantum devices utilizing spin-orbit coupling without magnetic materials to achieve high electron spin polarization, with potential enhancement from structural curvature like in DNA.
Contribution
It presents a novel device model based on coupled 1D chains with Rashba spin-orbit interaction, analyzing polarization effects and the influence of structural curvature and disorder.
Findings
High polarization predicted in the proposed device model.
Curvature, such as in DNA-like structures, enhances polarization.
Disorder leads to a broad distribution of polarization, with potential for high polarization in specific realizations.
Abstract
We propose quantum devices having spin-orbit coupling (but no magnetic fields or magnetic materials) that, when attached to leads, yield a high degree of transmitted electron polarization. An example of such a simple device is treated within a tight binding model composed of two 1D chains coupled by several consecutive rungs (i.e., a ladder) and subject to a gate voltage. The ensuing scattering problem (with Rashba spin-orbit coupling) is solved, and a sizable polarization is predicted. When the ladder is twisted into a helix (as in DNA), the curvature energy augments the polarization. For a system with random spin-orbit coupling, the distribution of polarization is broad, hence a high degree of polarization can be obtained in a measurement of a given disorder-realization. When disorder occurs in a double helix structure then, depending on scattering energy, the variance of the…
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Spin-orbit based devices for electron spin polarization
Y. Avishai1,3,4
Y. B. Band2,3,
1Department of Physics, and the Ilse Katz Center for Nano-Science,
2Department of Chemistry, Department of Physics, Department of Electro-Optics, and the Ilse Katz Center for Nano-Science,
Ben-Gurion University, Beer-Sheva 84105, Israel,
3New York University and the NYU-ECNU Institute of Physics at NYU Shanghai, 3663 Zhongshan Road North, Shanghai, 200062, China
4 Yukawa Institute for Theoretical Physics, Kyoto University, Kyoto 606-8502, Japan
Abstract
We propose quantum devices having spin-orbit coupling (but no magnetic fields or magnetic materials) that, when attached to leads, yield a high degree of transmitted electron polarization. An example of such a simple device is treated within a tight binding model composed of two 1D chains coupled by several consecutive rungs (i.e., a ladder) and subject to a gate voltage. The ensuing scattering problem (with Rashba spin-orbit coupling) is solved, and a sizable polarization is predicted. When the ladder is twisted into a helix (as in DNA), the curvature energy augments the polarization. For a system with random spin-orbit coupling, the distribution of polarization is broad, hence a high degree of polarization can be obtained in a measurement of a given disorder-realization. When disorder occurs in a double helix structure then, depending on scattering energy, the variance of the polarization distribution can increase even further due to helix curvature.
I Introduction.
Considerable interest has recently been focused on spintronic devices that give rise to spin polarization Sanvito_11 ; Urdampilleta_11 ; Charles_13 . Of particular importance for spintronics are devices that do not resort to external magnetic fields or magnetic materials Awschalom_09 , in contrast with those that do Upadhyay_99 . A major advantage of semiconductor spintronic devices requiring only electric fields for manipulating spins is the lack of design complexities associated with incorporating local magnetic fields Awschalom_09 . Interest in such devices was heightened following the measurement of spin-selective transmission of electrons through double-stranded DNA with spin polarizations exceeding 60% at room temperature (the spin polarization efficiency depends on the length of the DNA and its organization) Gohler_11 ; Naaman_15 . Here we propose a simple structure that yields outgoing polarized electrons given an incident beam of unpolarized electrons. It has a ladder-type structure (see Fig. 1) made of materials in which only spin-orbit (SO) is active (no magnetic fields). For simplicity and elegance, the SO is introduced as a non-Abelian gauge Frohlich .
This paper is arranged as follows. The description of the tight-binding model is presented in Sec. II and is used is Sec. III to study electron polarization in a few mesoscopic systems: (1) a clean planar and (2) a clean twisted two-chain ladder, in subsections III.1 and III.2 respectively. (3) In subsection III.3 we argue that a twisted disordered ladder emulates, in some sense, a DNA system and we evaluate the distribution of polarization for such system. Our main results are summarized in Sec. IV, where we suggest the following: (a) For clean systems with the geometry of a planar ladder, one can achieve a high degree of electron polarization that is due solely to SO coupling. (b) The effect of twisting the ladder into double helical strands with links is reflected by a negative curvature energy that enhances the polarization dramatically when the Fermi energy is close to the band center. (c) For a twisted disordered system (reminiscent of DNA, in a sense to be discussed below), the distribution of polarization has zero mean, but it is broad enough to expect a sizable degree of polarization measured on a given disorder-realization. Moreover, the effect of curvature augments the variance of the distribution even further. Some relevant topics are clarified in the appendices, including the transfer matrix solution to the scattering problem, the definition of the Aharonov-Casher phase, a proof that in a system respecting time reversal symmetry with a single source and a single drain leads such that both leads are strictly one dimensional, there is no polarization, and a discussion of spin density, spin-current, spin-torque, and a useful relation between spin flux and spin-torque.
II Tight binding Model
Guided by Fig. 1, we describe the system using a tight-binding model for an electron hopping on two chains numbered , where the sites on each chain are numbered and the lattice constant is . Hopping between the two chains occurs along adjacent links. For , sites () form the left (right) leads, while sites form the sample in which SO is active. Hopping between two sites and within the sample is encoded by SU(2) matrices , where is the dimensionless spin-orbit strength parameter, is the vector of Pauli spin matrices, and the unit vector determines the direction of the effective magnetic field acting on the electron on link (either along a chain or between chains). The representation of SO coupling in terms of SU(2) matrices, an extension of the Peierls substitution Spohn for a non-Abelian gauge, is discussed elsewhere, see e.g., Refs. Ando ; OEW . In semiconductors there are various sources of SO couplingRH , such as the Dresselhaus term (spin component parallel to the wave number ) and the Rashba term due to structural inversion asymmetry (spin component perpendicular to ), or any combination thereof. The SO interaction strength is significantly enhanced compared to its value in vacuum. Moreover, the SO strength and Fermi energy can be controlled by applying gate voltages (see Ref. Nitta , which studies an array of mesoscopic InGaAs rings controlled by Au gate electrodes).
The model Hamiltonian for the device in Fig. 1 is written in second-quantization using the annihilation operator for an electron at site with spin projection ,
[TABLE]
where = and is the (real) hopping amplitude (we take in what follows).
II.1 The scattering Problem
The Schrödinger equation with scattering boundary conditions is solved by the transfer matrix technique, see Appendix A. For definiteness, we consider scattering of an incoming electron at Fermi energy as it approaches the sample from the left in channel with spin direction . It can be reflected or transmitted into channel with spin direction . The reflection and transmission amplitudes are the 4$$\times$$4 matrices and , where the initial and final states are denoted by and respectively. Unitarity and time-reversal constraints imply band-avishai-1 ,
[TABLE]
where is the transmission matrix for scattering of incoming electrons from the right, and . Time reversal invariance implies, where .
II.2 Order of magnitude of spin order strength
Let denote the SO strength parameter defined through the Rashba Hamiltonian, , for a two-dimensional electron gas in an asymmetric quantum well, and let the lattice constant . The dimensionless spin-orbit strength parameter is where is the effective electron (or hole) massCardona . can be varied in the range, (e.g., see Ref. Nitta which studied SO effects on the conductance of a 2D network of InGaAs rings with radius ).
III Observables
We are mainly interested in the dimensionless conductanceLandauer , and the polarization of the transmitted electrons, , where is the number of transmitted electrons with spin projection . Generically, the transmitted and reflected polarizations and are vectors in spin space. Thus,
[TABLE]
where . All physical measurable observables (see Appendix D), such as and , depend on the spin-orbit strength , the wave number (equivalently on the Fermi energy ) and the number of rungs (equivalently the length of the sample). We shall see below that the behavior of these quantities as functions of for fixed or vice versa, are qualitatively similar because appears together with in the expression for the covariant wave number . This is completely analogous to the case where the vector potential (e.g., for an electron in a ring) is present in the covariant wave number , where is the dimensionless magnetic flux through the ring of radius , responsible for the Aharonov-Bohm effect. For a single square in our ladder, is directly related to the Aharonov-Casher phase, (see Appendix B). Note that is directly proportional to the strength of the U(1) vector potential, but the relation between and the coupling strength of the SU(2) vector potential is less simple,
[TABLE]
III.1 Plannar ladder
The strength of the Rashba SO coupling due to structural inversion asymmetry can be controlled by applying a gate voltage generating a perpendicular homogeneous electric field on sites , see Fig. 1. The corresponding SU(2) matrices in Fig. 1 are then, and . In Fig. 2 we plot the conductance and the transmitted polarization for links. In (a) is plotted for fixed as a function of while in (b) is plotted for fixed as function of . The pattern of the conductance is characterized by a series of peaks reflecting the mini-band structure commensurate with the number of links. As anticipated in our discussion above, the qualitative similarity of the two patterns is evident, except at the band center where resonant transmission sometimes occurs, and at the band edges where the conductance vanishes. The corresponding transmitted polarizations are shown in (c) and (d). At the peaks, the magnitude of the polarization is remarkably high. Achieving 80% polarization with such a simple structure based solely on spin-orbit coupling is a godsend for spintronics. Just like the patterns of conductance in (a) and (b), the similarity between the patterns of polarization shown in (c) and (d) is evident.
As is evident from Figs. 2(c) and 2(d), varies sharply and changes sign at (the band center) and at . Consequently, the sign of the polarization is controllable by a gate voltage, an attractive feature from the spintronics point of view. The sharp slope of near the sign reversal point occurs due to the term [that controls the spin physics within the hopping matrix ] which is maximal at .
III.2 Twisted ordered ladder
Now we modify the geometry to be closer to that of DNA by twisting the ladder so that each strand becomes a helixMatityahu . After writing the Schrödinger equation for an electron on a single 1D helical strand, we treat the dynamics of an electron on the twisted ladder within a tight-binding model. The resulting Hamiltonian is similar to that of Eq. (A), albeit with one modification: The kinetic energy term includes a constant negative energy due to the curvature of the helix. The consequences of this modification will be analyzed for ordered and disordered ladders below. We start from Eq. (9) of Ref. Gutierrez and modify it such that the SO enters as an SU(2) gauge. Using as a length coordinate along the helix, the Hamiltonian for an electron moving along a (strictly) 1D helix is,
[TABLE]
where is a local space-dependent SU(2) vector potential Gutierrez . Here is a local potential (assumed to be 0 for simplicity), and is the curvature energy, where is the curvature of the helix.
Before turning to the tight-binding formulation, it is important to point out that one should not expect polarization in a strictly 1D structure because, without a closed loop, the vector potential can be eliminated by a suitable gauge transformation (see Appendix C). Moreover, in 1D, time reversal invariance, Eq. (II.1), implies that the 22 reflection matrix so that according to Eq. (3), . Similar considerations hold for the transmitted polarization, hence .
For the ordered ladder, we assume that the electric field is also “twisted” in the sense that its action on a given link in the twisted and non-twisted ladders is the same. Consequently, the sole effect of twisting is the occurrence of the curvature energy. If the length coordinate is expressed in units of then energies are measured in units of and = -1/4 (dimensionless). Thus, the energy on sites , , and , is lowered by . The effect of curvature is expected to be significant when . Hence, the wave number is chosen close to the band center where the Fermi energy is small.
The conductance and the polarization are plotted in Fig. 3 versus , 3, (the number of links) for and for the non-twisted ladder (, as in Fig. 1) and for the twisted ladder (). The curvature has a dramatic effect on the polarization. In the absence of curvature, the polarization at the band center virtually vanishes, but when the curvature is included, the polarization saturates close 80%. This result depends on the position of the Fermi energy; far away from the band center, the polarization generally remains high, but the curvature has just a small effect.
III.3 Combination of twisting and disorder
We now turn to the case where the SO coupling on the various links are not solely determined by the Rashba SO mechanism, and where the underlying electric fields are not necessarily homogeneous. For example, in DNA Gohler_11 ; Naaman_15 , the pattern of local fields responsible for SO coupling (strengths, directions, etc.) is extremely complicated and may vary sharply as function of position. We model this by assuming that the Hamiltonian (A) is a random matrix drawn from a GSE. Similar concepts are prevalant in many branches of physics since the early days of random-matrix theory that was employed for analyzing the energy spectra of complex nuclei. To implement this in our disordered ladder, the SU(2) hopping matrices on the links are assumed to be random, independently and identically distributed. Now, the problem of generating an ensemble of these matrices must be addressed. An SU(2) matrix is determined by three Euler angles,
[TABLE]
where , , . Generating random SU(2) matrices should take into account the Haar measure, , where . We follow the method introduced in Ref. Ozols , but with a trivial modification Ozols_mod .
The calculation of the distribution is now carried out employing a large ensemble of random SU(2) matrices. Our aim here is to elucidate the distribution of the transmitted polarization and its two lowest moments for a given number of links and wave number . The transmitted polarization is expected to be finite in all three directions in spin space, i.e., , and , but here we focus for simplicity on . It is expected that , but the interesting quantity here is the variance because large variance means that there is a significant probability for detecting a high degree of polarization in a measurement of a given disorder-realization.
Fig. 4 shows the distributions for and for a ladder of 15 links with . The effect of curvature is to enhance the variance of the polarization distribution (see the figure caption for details). This augments the probability to achieve higher polarization in a measurement of a given disorder-realization. Thus, by tuning the Fermi energy close to the band center we can substantially increase the width of the polarization distribution.
IV Summary and conclusions
We have shown that SO coupling in a 2D mesoscopic device having a simple ladder geometry yields a high degree of transmitted electron polarization. Moreover, similarly to the study of conductance in InGaAs samples Nitta , applying a gate voltage allows control of the polarization either by tuning the SO strength or the electron density (equivalently, the Fermi energy). When the ladder is twisted into a helix (as in DNA), the curvature energy plays an important role by increasing the polarization, particularly for Fermi energy near the band center. For complicated systems with rapidly and randomly varying local electric fields, it is reasonable to assume that the parameters determining the local SO strength and direction are independently and identically distributed random numbers, i.e., the hopping terms appearing bin Eq. (A) are random SU(2) matrices. The resulting distribution of transmitted polarization is broad enough to expect a high degree of polarization in a measurement of a given disorder-realization. The variance of the distribution can be increased even further, as shown in Fig. 4, due to the curvature of the helix. The results reported here show that simple spintronic devices that polarize electrons can be designed without resorting to the use of magnetic materials or external magnetic fieldsHatano .
Finally, it is worth mentioning the relevance of Refs. Miron and Liu to our work. Reference Miron demonstrated that a perpendicularly magnetized cobalt quantum dot can be switched at room temperature by injecting an in-plane current. The symmetry of the switching field is consistent with the spin accumulation induced by Rashba interaction and also with the torque induced by the spin Hall effect. The relevance to our work is that the effective magnetic field that drives the switching is due to Rashba SO coupling. However, our motivation is entirely different, as we are interested in obtaining a current of polarized electrons and not in reversing the polarization of a magnetic material. Reference Liu uses the spin Hall effect to generate a strong spin current that induces efficient spin-torque switching of ferromagnets at room temperature. Here also, our motivation is very different, as explained above. In both these works, the relevance of spin-torque is stressed. Indeed, spin-torque is an important ingredient in contemporary spintronics. Using the continuity equation for spin currents, we show in Appendix D that the volume integrated spin-torque of the ladder system is directly related to the transmitted and reflected polarizations defined in Eq. (3).
Acknowledgement. This work was supported in part by grants from the Israel Science Foundation: No. 400/2012 (YA), No. 295/2011 (YBB), and DFG Grant FO 703/2-1 through the DIP program (YBB). YA thanks D. Ariad, C. de Morais Smith and Z. Ovadyahu for fruitful discussions.
Appendix A Solution of the ladder model by the Transfer Matrix Method
Here we solve the scattering problem for the model whose Hamiltonian is introduced in Eq. (1) (re-written here for self-consistency) and compute transmission and reflection amplitudes. The model Hamiltonian for the device in Fig. 1 is written in second-quantization using the annihilation operator for an electron at site with spin projection ,
[TABLE]
where = and is the (real) hopping amplitude.
Our aim is to solve the Schrödinger equation for the two component spinor , subject to scattering boundary conditions. Here is the scattering energy and is the wave number (where we have taken the lattice constant ). For definiteness, we consider a scattering problem wherein an incoming electron approaches the link at from the left () in channel with spin direction . It can be reflected or transmitted into channel with spin direction . Henceforth, the spinor wave functions and the scattering amplitudes depend on (and should carry) the initial quantum numbers . Thus, the corresponding reflection and transmission amplitudes are written as , and .
We expand the spinor in a complete set of basis functions in the [chainsitespin] space. The basis functions are denoted by ; explicitly, and . Thus,
[TABLE]
It is useful to use compact notation and define a 4$$\times$$4 wave-function matrix whose elements are the spinor components defined in Eq. (8),
[TABLE]
where the order of rows (counting from the top) or columns (counting from the left) is .
Now we define the 8$$\times$$8 transfer matrices , , and a total transfer matrix ,
[TABLE]
while the product in the square parenthesis in Eq. (A) is the 8$$\times$$8 identity matrix for . For an ordered lattice the spin-orbit (SO) potential is periodic and all the matrices forming the product inside the square parenthesis are identical, i.e., , and the product is equal to . For the random ladder, all the matrices in the square parenthesis are different. The transfer matrices act on 8$$\times$$4 wave function matrices. The above construction implies that the total transfer matrix across the ladder satisfies
[TABLE]
Knowing the 8$$\times$$8 transfer matrix , one obtains the 4$$\times$$4 transmission and reflection matrices and with elements and .
Starting from Eq. (11) we find,
[TABLE]
This enables us to express and in terms of the four 4$$\times$$4 blocks of , denoted as , with . The explicit expressions are:
[TABLE]
As a test of the correctness of these relations one can confirm the time-reversal and unitarity constraints,
[TABLE]
Here , and and are the transmission and reflection matrices for scattering of incoming electrons from the right. Note that these relations connect matrix elements of the transmission matrices on different sides of the sample, and matrix elements of the reflection matrices on the same side of the sample. These relations imply the absence of spin-flip in the reflection amplitude of the same channel, i.e., , and also that the diagonal elements of the reflection matrix are equal, for each channel. We shall see below that these relations also imply the absence of transmitted and reflected polarizations.
It remains to determine the 8$$\times$$8 local transfer matrices . A glance at Fig. 1 suggests that there are three kinds of sites: (1) For and the coordination number is 2 and the two links attached to it are bare. (2) For and the coordination number is 3, one link is bare and two links are “dressed” with SU(2) hopping matrices. (3) For the coordination number is 3, and all three links are “dressed” with SU(2) hopping matrices. This respectively requires three slightly different definitions. For this purpose it is useful to define the following 4$$\times$$4 matrices:
[TABLE]
After some algebra we find,
[TABLE]
where every entry in these matrices is a 4$$\times$$4 matrix in channelspin space.
Appendix B Aharonov–Casher Phase for a square subject to a homogeneous perpendicular elecric field
Consider a closed contour in the form of a square of side lying on the - plane subject to a constant electric field along . Within a tight-binding model an electron hops between its corners, as in Fig. 5. Upon traversing the square counterclockwise, starting and ending at (0,0), the wave function of an electron gains an SU(2) phase factor
[TABLE]
where is dimensionless. Since is an SU(2) matrix, it can be written as
[TABLE]
where is the Aharonov–Casher phase. The value of is given by,
[TABLE]
The fact that calculation of involves a trace indicates that this expression is gauge invariant. Note that the relation between and is highly non-linear, so that the definition of SU(2) flux seems problematic. In Fig. 6 is plotted as a function of the SO coupling strength (which is identical on all four links).
Appendix C Absence of polarization in systems with two 1D leads
Following Eq. (5), we pointed out that if a sample is composed of strictly 1D helix with SO coupling, it is not possible to obtain a non-vanishing polarization because in the absence of a closed loop, the SU(2) vector potential can be eliminated by a gauge transformation. This statement is based on the formulation of the SO coupling within an SU(2) gauge formalism, namely, it relies on an approximation. Here we show that due to unitarity and time reversal invariance, this statement is exact. Moreover, it holds for any system with a maximum of two strictly 1D leads, including systems with closed loops such as in a ring interferometer. To show this, let us denote by () the 22 transmission and reflection matrices for an electron scattering impinging on the sample from lead 1 (2). Then, the 44 matrix and its unitarity relation read,
[TABLE]
Let us focus our attention on a non-diagonal element of the unitarity relation (a 22 matrix),
[TABLE]
The constraints (A) imposed on the transmission and reflection matrices show that,
[TABLE]
First, it is easy to see that the reflected polarization vanishes because is proportional to the unit matrix and hence Tr. As for the transmitted polarization, we use Eq. (A) and express the elements of in terms of the element of , and then use Eq. (20) to obtain the third equation of (C). For an unpolarized incoming beam of electrons, this implies the vanishing of the transmitted polarization, i.e.,
[TABLE]
Numerical example
As a numerical example, consider a ring interferometer of radius with two 1D leads (source lead at angle and drain lead at ), subject to a perpendicular electric field leading to Rashba SO coupling, as shown in Fig. 7. The SO strength is taken to be and the wave number is . The solution of the scattering problem yields the transmission and reflection matrices.
[TABLE]
[TABLE]
The dimensionless conductance is =Tr=1.58783. Using Eq.(22) the reader can easily verify that all the transmitted (and reflected) polarizations vanish.
Appendix D Spin Density, Current and Torque
Spin density, spin current and spin-torque are three central quantities in contemporary spintronics. In this section we show that our ladder model is an appropriate theoretical framework for studying these quantities. As a byproduct, we derive a useful relation between the transmitted and reflected polarization vectors and the volume integrated spin-torque.
The spin density at site resulting from an incoming wave in state is a local vector field in spin space defined as Qian-Niu ; band-avishai-2 , . Here is the electron spin operator in the Heisenberg representation and the spinor is defined in Eq. (8). In the leads ( for the left lead and for the right lead), where SO coupling is absent, is independent of , and the spin densities on the left and right are respectively expressible in terms of the reflection and transmission amplitudes:
[TABLE]
The spin current on chain and site resulting from an incoming wave in state is a local quantity (a tensor field with Cartesian and spin components) defined as Qian-Niu ; band-avishai-2 (where is the velocity operator). For and we have,
[TABLE]
hence is independent of . The total spin current in the leads (where SO is absent) is obtained after summing on initial conditions and adding the contributions from both chains:
[TABLE]
Here (defined after Eq. (3)), and and are the transmitted and reflected spin currents. In the present case the spin current tensor field has only a single Cartesian component, namely, it is directed along (see Fig. 1), and has spin components according to . We shall sometimes denote in order to remind us that the th component of the spin current in Euclidean space is still a vector in spin space. Following Eq. (25), for we have (the transmitted spin current) while for we have (the reflected spin current). The sign of the components of the spin current depends on its directions in Euclidean and in spin spaces. Explicitly, let us denote the component (in spin space) of and by and . Then we have
[TABLE]
and note that
[TABLE]
The spin-torque is a vector in spin space:
[TABLE]
The experimentally relevant observable spin-torque is obtained after summation over all initial conditions, i.e., . Outside the SO interaction region , , and vanishes. Generically, in the region, where SO is active, because even in the static case. Of special interest is the volume integrated spin-torque (see Ref. Qian-Niu ) which, for the discrete tight-binding geometry, takes the form .
Relation between spin flux and spin-torque. Upon using the continuity equation for the spin current in the stationary case (where ) Qian-Niu , and summing over initial conditions , we obtain
[TABLE]
which is valid anywhere (i.e., for any , including inside the sample where SO is active). Summing over in Eq. (D) we obtainHyman ,
[TABLE]
Using the divergence theorem, the LHS of Eq. (30) equals the total spin flux out of the sample into the left and right leads. Note that is a vector in spin space. In Ref. Qian-Niu it is noted that under certain symmetry constraints, . In our tight-binding model, the spin currents for and for are perpendicular to the links and there is no spin current along (through the chains). Therefore, the transmitted and reflected spin fluxes through the sample borders are and where is the length of the links. Then, if , the vector field (directed along , and having spin component ) are flux-less; the same spin current that enters the sample on one side leaves it on the other side and the total spin flux vanishes. In the generic case, however, where , the total spin flux is related the transmitted and reflected currents and to the volume-integrated spin-torque as,
[TABLE]
Equation (31) gives us a direct and useful relation between the measurable current outside the interaction region (the sample), and the wave functions inside the sample which appears in the calculations of the spin-torque, Eq. (D). In addition, our calculations on similar systems indicate that is correlated also with the charge conductance , i.e., the charge conductance reflects the underlying spin physics. Although Eq. (31) is a direct consequence of the continuity conditions, we have not seen its derivation elsewhere.
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