Current-induced spin polarization of a magnetized two-dimensional electron gas with Rashba spin-orbit interaction
A. Dyrdal, J. Barnas, V. K. Dugaev

TL;DR
This paper provides a theoretical analysis of how current-induced spin polarization in a magnetized 2D electron gas with Rashba spin-orbit interaction depends on temperature, including analytical and numerical results within the linear response regime.
Contribution
It introduces a formalism using Matsubara Green functions to describe temperature effects on spin polarization in magnetized Rashba systems, highlighting the role of Berry phase and relaxation time.
Findings
Spin polarization depends on temperature and relaxation time.
The spin polarization includes a Berry phase contribution.
Rashba spin-orbit torque results from exchange coupling.
Abstract
Current-induced spin polarization in a two-dimensional electron gas with Rashba spin-orbit interaction is considered theoretically in terms of the Matsubara Green functions. This formalism allows to describe temperature dependence of the induced spin polarization. The electron gas is assumed to be coupled to a magnetic substrate via exchange interaction. Analytical and numerical results on the temperature dependence of spin polarization have been obtained in the linear response regime. The spin polarization has been presented as a sum of two terms - one proportional to the relaxation time and the other related to the Berry phase corresponding to the electronic bands of the magnetized Rashba gas. The spin-orbit torque due to Rashba interaction is also discussed. Such a torque appears as a result of the exchange coupling between the non-equilibrium spin polarization and magnetic moment of…
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Current-induced spin polarization of a magnetized two-dimensional electron gas with Rashba spin-orbit interaction
A. Dyrdał1, J. Barnaś1,2 and V. K. Dugaev3
1Faculty of Physics, Adam Mickiewicz University, ul. Umultowska 85, 61-614 Poznań, Poland
2 Institute of Molecular Physics, Polish Academy of Sciences, ul. M. Smoluchowskiego 17, 60-179 Poznań, Poland
3 Department of Physics and Medical Engineering, Rzeszów University of Technology, al. Powstańców Warszawy 6, 35-959 Rzeszów, Poland
Abstract
Current-induced spin polarization in a two-dimensional electron gas with Rashba spin-orbit interaction is considered theoretically in terms of the Matsubara Green functions. This formalism allows to describe temperature dependence of the induced spin polarization. The electron gas is assumed to be coupled to a magnetic substrate via exchange interaction. Analytical and numerical results on the temperature dependence of spin polarization have been obtained in the linear response regime. The spin polarization has been presented as a sum of two terms – one proportional to the relaxation time and the other related to the Berry phase corresponding to the electronic bands of the magnetized Rashba gas. The spin-orbit torque due to Rashba interaction is also discussed. Such a torque appears as a result of the exchange coupling between the non-equilibrium spin polarization and magnetic moment of the underlayer.
pacs:
71.70.Ej, 75.76.+j, 85.75.-d, 72.25.Mk
I Introduction
Spin-orbit interaction leads, in general, to a number of interesting transport phenomena, that enable generation and control of spin currents in a pure electrical manner. Two of the most prominent examples are the spin Hall and spin Nernst effects. The former (latter) effect consists in generation of pure spin current flowing perpendicularly to an external electric field (temperature gradient) applied to the system. These effects play currently an essential role in the processes of electrical generation and detection of spin currentsSinova_RMP2015 ; SinovaZutic2012 . For instance, the spin current can be used as origin of spin torque exerted on magnetic moments of a ferromagnet in a bilayer system consisting of a magnetic layer attached to a nonmagnetic one with strong spin-orbit coupling. This torque, in turn, may induce magnetic dynamics and even can reverse magnetic moment of the magnetic layer when the spin current exceeds some critical value.
Another consequence of the spin-orbit interaction in a system with mobile electrons is the current-induced nonequilibrium spin polarization of conduction electrons. This effect was predicted theoretically in the ’70s dyakonov71 ; Ivchenko78 for a two-dimensional electron gas (2DEG) with Rashba spin-orbit interaction, and then it was studied in various systems exhibiting spin-orbit interaction edelstein90 ; aronov89 ; liu08 ; gorini08 ; wang09 ; schwab10 ; golub11 ; dyrdal13 ; dyrdal14 . The current-induced spin polarization was also observed experimentally vorobev1979 , and currently it is attracting attention of many researchers kato04 ; silov04 ; sih05 ; yang06 ; stern06 ; koehl09 ; kuhlen12 ; norman14 .
The current-induced spin polarization can also arise in a magnetic system, when it includes spin-orbit coupling. In such a case the induced non-equilibrium spin polarization interacts with the local magnetization via exchange coupling and creates a torque exerted on the magnetic moment Manchon08 ; Abiague09 ; Gambardella11 ; Garello13 ; Kurebayashi14 . Moreover, it has been also shown that not only external electric field, but also a temperature gradient may lead to spin-orbit driven spin polarization dyrdal13 ; wang10 ; XiaoMa2016 . These observations initiated a wide interest in the field- and thermally-induced spin-orbit torques and new ways of magnetization switching, that could be alternative to the switching induced by spin transfer torques Li04 ; Hatami07 ; Ansermet10 .
In this paper we present theoretical results on the current-induced spin polarization of a magnetic 2DEG with Rashba spin-orbit interaction. Such a system is a basic model of various magnetic semiconductor heterostructures. The system consists of a 2DEG deposited on a magnetic substrate and interacting with the substrate via exchange interaction (see also Fig.1). To calculate the current-induced spin polarization we use the Matsubara Green function formalism which enables description of the temperature variation of the induced spin polarization. We derive some general formulas for the polarization and also present numerical results. The induced spin polarization is shown to include generally a term due to Berry curvature of the corresponding electron bands. Similar terms also appear in the spin-orbit torques following from exchange interaction of the electrons and magnetic underlayer.
The paper is organized as follows. In section 2 we describe the model system and also present the theoretical formalism and derive general formulas for the current-induced spin polarization. In Section 3 we present analytical and numerical results in some specific situations; first, we consider the nonequilibrium spin polarization in the absence of exchange field (Section 3 A), then we present results for exchange field oriented perpendicularly to the plane of 2DEG (Section 3 B) and for exchange field oriented in plane of 2DEG and collinear (perpendicular) to the electric current, Section 3C (Section 3 D). In Section 4 we discuss the spin polarization in a general case of arbitrarily oriented exchange field. In Section 5, in turn, we consider relation of the nonequilibrium spin polarization with the Berry curvature of the corresponding electronic bands. The induced spin-orbit torque is briefly discussed in Section 6, while summary and final conclusions are in Section 7.
II Theoretical outline
We consider a magnetized 2DEG with Rashba spin-orbit interaction, as shown schematically in Fig.1. The 2DEG is assumed to be deposited on a ferromagnetic substrate which creates an effective exchange field acting on the electron gas.
II.1 Model
The single-particle Hamiltonian describing such a system can be written in the following form:
[TABLE]
where and (for ) are the unit and Pauli matrices defined in the spin space, the parameter in the second term of the Hamiltonian describes strength of the Rashba spin-orbit interaction, while and are the in-plane wavevector components. The third term of the above Hamiltonian describes the effect of exchange field due to a magnetic substrate. This exchange field can be written as , with standing for the exchange parameter ( for a ferromagnetic coupling between the 2DEG and magnetic substrate). Note, the exchange field is measured here in energy units. In spherical coordinates (see Fig.1), components of the exchange field, , can be written as
[TABLE]
where , while and are the polar and azimuthal angles, as defined in Fig. 1. In general, we take into account the temperature dependence of the magnetization , and assume it obeys the Bloch’s law , where is the Curie temperature of the magnetic substrate, and is the corresponding zero-temperature magnetization.
Eigenvalues of the Hamiltonian (1) take the form
[TABLE]
where (with ), while .
Below we present the theoretical method based on the Matsubara-Green function formalism, and also derive a general formula for the nonequilibrium spin polarization induced by an external electric field.
II.2 Method and general solution for current-induced spin polarization
To describe spin polarization induced by an external electric field we introduce a time-dependent external electromagnetic field of frequency (note, here is energy) described by the vector potential . The electric field is related to via the formula . Hamiltonian describing interaction of the system with the external field (treated as a perturbation) takes the form
[TABLE]
Here, the operator of the electric current density is defined as ; with being the charge of electron (), and being the electron velocity operator. The and components of the velocity operator have the following explicit form:
[TABLE]
where is the angle between the wavevector and the axis , i.e. and , while the last terms in Eq. (5) and Eq. (6) represent components of the anomalous velocity that originates from the Rashba spin-orbit interaction.
Without loss of generality, we assume in this paper that the external electric field is oriented along the -axis. Thus, the -th () component of the quantum-mechanical average value of spin polarization induced by the external electric field can be found in the Matsubara-Green functions formalism from the following formula:
[TABLE]
where is the operator of the ’s spin component, (with and denoting the temperature and Boltzmann constant, respectively), and are the Matsubara energies, while are the Matsubara Green functions (in the matrix form). Note, the perturbation term takes now the form , with the amplitude of the vector potential determined by the amplitude of electric field through the relation .
Taking into account the explicit form of , one can rewrite Eq.(7) in the form
[TABLE]
The sum over Matsubara energies in the above expression can be calculated by the method of contour integration, abrikosov ; mahan
[TABLE]
where denotes the appropriate contour of integration and is a meromorphic function of the form , that has simple poles at the odd integers , (for details see Refs [abrikosov, ; mahan, ]).
Upon analytical continuation one obtains
[TABLE]
Here, is the Fermi-Dirac distribution function and is the impurity-averaged retarded/advanced Green function corresponding to the Hamiltonian (1). The Green functions take the following explicit form:
[TABLE]
where
[TABLE]
with and . Note, we assumed , with equal effective relaxation time in the two subbands.
Using equation (II.2) as a starting point and performing integration over we get finally the following formula for the three components of the current-induced spin polarization:
[TABLE]
[TABLE]
[TABLE]
Details on the derivation of the above equations are presented in the Appendix A. Before presenting results on the current-induced spin polarization for an arbitrary orientation of the exchange field, we consider first some special cases.
III Special cases
III.1 Zero exchange field
First, we reconsider the limit of zero exchange field, i.e. the limit of a nonmagnetized 2DEG, when only the component of spin polarization survives. The general expression for takes then the following form:
[TABLE]
where . Note that in this limit the eigenvalues have the form .
In the low-temperature regime, the above integrals can be evaluated analytically and one arrives at
[TABLE]
When both subbands are occupied (which corresponds to ), the Dirac delta functions in the above equation can be written in the form
[TABLE]
and finally one obtains
[TABLE]
with . The first term of Eq.(III.1) corresponds to the Edelstein expression for the current-induced spin polarization in the so-called bubble approximation,
[TABLE]
Note, the impurity vertex correction is neglected in our considerations. Such a correction leads to some renormalization of the spin polarization (for details see e.g. Ref. [edelstein90, ; BDDIchapt, ]). The second term in (III.1) is a correction which originates from the imaginary term in the nominator of the Green function and products of two retarded or two advanced Green’s functions (omitted in Ref. edelstein90, ). Note, the second term in Eq.(III.1) vanishes in the quasi-ballistic limit (low impurities concentration), when .
In the general case, i.e. for arbitrary and arbitrary chemical potential , one should use the general formula (16). However, one point requires some comment. It is known, that for impurities with short-range (-like) potential and , the parameter is constant, while for negative it increases and diverges when approaches the bottom of the lower energy band Brosco ; Dyrdal2016 . Thus, at a certain value of , , the Ioffe-Regel localization condition Ioffe is obeyed, and the states become localized below . Accordingly, the results are valid beyond the localization regime, i.e. for .
Now, we present some numerical results. In Fig.2(a) we show the temperature dependence of spin polarization for four different values of chemical potential . Here, we should mention that the chemical potential also depends on temperature, thus a fixed value of chemical potential means that the carrier concentration varies. If however the system is gated one can keep chemical potential constant. Apart from this, the relaxation time (and thus the parameter ) may also depend on temperature . This dependence, however, is neglected in Fig.2. The spin polarization was obtained from Eq.(16) and is normalized there to the corresponding value of (note does not depend explicitly on temperature). For the largest value of , the component remains almost constant in the temperature range shown in Fig.2(a), and is roughly equal to the corresponding value of . For smaller values of , in turn, the spin polarization becomes reduced monotonously with increasing (see the curves for eV and eV). For still lower values of , the temperature dependence is nonmonotonous - it first decreases and then slightly increases with temperature. To understand this behaviour we plot in Fig.2(c) the spin polarization as a function of chemical potential for several values of temperature and the same as in Fig.2(a). This figure clearly shows that spin polarization tends to with increasing . Such a behavior is reasonable as the second term in Eq.(19) decreases with increasing (the effective role of finite decreases with increasing ). For small values of , however, the second term in Eq.(19) plays a role and the spin polarization is reduced. The temperature dependence appears when at the Fermi level is of the order or smaller than , which takes place in the region of small values of . Moreover, this figure also shows that decreases with increasing , except a narrow region of small values of , where the temperature dependence is nonmonotonous, exactly like in Fig.2(a) The temperature dependence is also shown in Fig.2(b) for several values of . This figure also shows that the correction due to the second term in Eq.(19) increases with increasing . The latter behavior is shown explicitly in Fig.2(d) for indicated values of . The decrease of spin polarization with increasing is physically clear as the effective separation of the two Rashba bands becomes reduced with increasing . The second term in Eq.(19) plays then an important role and leads to reduction of spin polarization.
III.2 Exchange field perpendicular to plane of 2DEG
Consider now a magnetized 2DEG and let us begin with the situation when the exchange field (or equivalently substrate magnetization) is perpendicular to the plane of 2DEG, . The eigenvalues of Hamiltonian (1) reduce now to the form , with .
The general expressions describing the two nonzero components of spin polarization take the forms
[TABLE]
[TABLE]
while . Accordingly, the electric field generates now spin polarization with both in-plane components nonzero, while the component normal to the plane of 2DEG (along the exchange field) vanishes exactly. Thus, the exchange field generates spin polarization along the electric field and also modifies the spin polarization along the axis .
In the low temperature limit equations (III.2) and (III.2) lead to the following analytical expressions:
[TABLE]
[TABLE]
where represent the density of states corresponding to the subbands, respectively, , and are the Fermi wavevectors corresponding to the two subbands.
In the ballistic limit (extremely long relaxation time), Eq. (III.2) takes the form
[TABLE]
which after integration over leads to
[TABLE]
i.e. to the first term in Eq.(III.2). The above expression does not depend on the relaxation time and due to the mathematical form of Eq.(25) it may be identified as the Berry phase related contribution to the spin polarization, that in turn may be responsible for anti-damping spin-torque. For details see Section V.
Numerical results on the current-induced spin polarization of the magnetized 2DEG with the exchange field oriented perpendicularly to the plane are shown in Fig.3. The dependence of and on the exchange field is presented in Figs 3(a) and 3(b), respectively. Figure 3(a) clearly shows that vanishes in the limit of zero exchange field and then its magnitude grows rather fast with increasing . Then, it decreases to zero for large exchange fields. Magnitude of , in turn, is nozero for zero exchange field, and increases with increasing . It reaches a maximum at some value of , and then decreases with a further increase in . Such a behavior with can be understood since the relative role of Rashba coupling decreases with increasing . Note, that the component is antisymmetrical with respect to sign reversal of , while the component is then symmetrical. Figures 3(c) and 3(d) present the and components of spin polarization as a function of temperature for fixed values of chemical potential and . In numerical calculations we have assumed K and therefore the component vanishes for K. In turn, the components is remarkably enhanced below and drops to a weakly temperature dependent value (for fixed chemical potential and the parameter ) when K.
Variation of spin polarization with the chemical potential is presented in Figs 3(e) and 3(f) for different magnitudes of the exchange field . Magnitudes of both components increase monotonously with when is inside the energy region between the bottom edges of the two subbands. For in the vicinity of the bottom of higher energy band, these components reach maximum values and for larger they decrease with increasing . Note, the component is roughly three orders of magnitude smaller than the component.
In Fig. 3(g) and 3(h) we show the and components of the spin polarization as a function of the Rashba coupling constant. These figures clearly show that the absolute values of both components increase roughly linearly with . However, some deviations from this linear dependence appear above certain values of , where the increase is smaller.
III.3 Exchange field in plane of 2DEG and perpendicular to electric field
In this section we consider the current-induced spin polarization for the magnetization vector (exchange field) oriented along the axis, i.e. when the exchange field is in the plane of two-dimensional electron gas and perpendicular to the current. In such a case the and components of the current-induced spin polarization vanish exactly, and the only nonzero component is - like in the case of zero exchange field. This component, however, is modified by the exchange field.
Numerical results for are shown in Fig.4, where variation of with the exchange field , Fig.4(a), clearly shows that the spin polarization decreases relatively fast with increasing absolute value of and is suppressed when the Zeeman-like term (due to exchange coupling to the substrate) dominates over the Rashba term. The suppression to zero of spin polarization at large appears due to strong modification of electronic states by the Zeeman like term, and takes place for all values of chemical potential.
Temperature dependence of is shown in Fig.4(b) for two values of chemical potential and two values of . For the larger value of , the spin polarization vanishes in a broad temperature region and then increases when approaches the Curie temperature, reaching the magnitude of in the limit of a nonmagnetized 2DEG. This behavior is consistent with that in Fig.4a
In Fig.4(c) we show as a function of chemical potential. As follows from this figure, increases monotonously with the chemical potential increasing from the minimum of the lower subband, and then becomes saturated for large values of . The rate of this increase as well as the chemical potential at which the saturation appears depend on . Spin polarization as a function of the Rashba parameter is shown in Fig.4 (d) for indicated values of the exchange field. In general, the component of spin polarization increases now nonlinearly with the Rashba constant.
III.4 Exchange field in plane of 2DEG and collinear with electric field
When the exchange field is oriented along the axis, i.e. it is collinear with the external electric field, the component of spin polarization vanishes, whereas the and components are non-zero. In general, the component of spin polarization is roughly three orders of magnitude smaller than the component. Variation of both components with the exchange field , temperature, chemical potential, and Rashba constant is presented in Figs5 (a-d).
Behavior of the and components with , , and is qualitatively similar to the corresponding behavior of the components and in the case with the exchange field normal to the plane of 2DEG, see Fig.3. There are some differences of rather quantitative character, which follow from different electronic bands in these two situations. For instance, the component varies with the chemical potential in a slightly different manner than the component in Fig.3. Weak difference also appear in the variation of the component with temperature for below the Curie temperature . Similarly as in Fig. 3, both components behave almost linearly with the Rashba parameter .
IV Numerical results for arbitrarily oriented exchange field
Up to now we have discussed only some specific situations, when the exchange field is oriented along the three main directions: (i) along the electric field, (ii) normal to the electric field and to the plane of 2DEG, and (iii) normal to the electric field and oriented in the plane of 2DEG. Now let us consider a general case, when the exchange field is oriented arbitrarily. This orientation is described by the polar and azimuthal angles, as shown in Fig.1. Generally, all three components of spin polarization (i.e. , and ) can be nonzero. In Fig. 6 we present these components as a function of both and angles, see left panel in this figure. The right panel, in turn, presents several vertical cross-sections of the corresponding density plots from the left panel. In the specific configurations considered in the preceding section, the results shown in Fig. 6 reduce to the corresponding ones discussed in Sec.3. This figure shows the regions in the () plane, where particular components of the spin polarization are large and where are small or suppressed to zero .
The results in a general case, like those presented in Fig. 6 are required when considering magnetic dynamics induced by spin torque due to spin polarization. Magnetic moment (and thus also exchange field) precesses then in space, and this time evolution is associated with time evolution of the spin polarization. In this paper, however, we do not consider dynamical properties and focus rather on evaluating spin polarization in static situations.
V Relation with the Berry Curvature
Recently H. Kurebayashi et al. Kurebayashi , based on experimental results, have proposed the anti-damping spin-orbit torque mediated by the Berry phase Berry . In other words, they showed that the Berry curvature gives rise to the spin-orbit torque in systems with broken inversion symmetry.
Our results given by Eqs. (II.2)-(II.2) show that when the exchange field is nonzero, the inversion symmetry is broken and the general expressions for the and components of the spin polarization contain terms that do not depend on relaxation rate, but are functions of the Fermi-Dirac distribution function instead of its derivative. Thus, taking into account the notation well known in the context of the anomalous Hall effect, we can rewrite Eqs (II.2)-(II.2) as follows:
[TABLE]
where the first term depends on the states in a close vicinity of the Fermi level: , while the second term contains information from all electronic states: . Now we show that the terms are related to the Berry curvature.
To do this let us rewrite the Hamiltonian (1) in the following form:
[TABLE]
where , and . The eigenvectors corresponding to the eigenvalues can be written as
[TABLE]
The Berry curvature of the -th () band, , is defined as the rotation of the Berry connection (for details see Refs Volovik, ; DiXiaoRevModPhys, ; NagaosaRevModPhys, ). Thus one can write
[TABLE]
Combining Eqs. (28) to (30) we find for the Berry curvature,
[TABLE]
Taking the expression above into account, the Berry phase related terms in the electrically generated spin polarization can be written as
[TABLE]
Note, these terms disappear in the absence of exchange field.
VI Spin-orbit torque
Due to exchange interaction, the current induced spin polarization exerts a torque on the magnetic moment . This torque enters the Landau-Lifshitz-Gilbert equation for magnetic dynamics,
[TABLE]
where is a unit vector along magnetic moment , is the effective magnetic field which includes external magnetic field, dipolar field, and anisotropy field, is the Gilbert damping factor, and is the giro-magnetic factor.
To find the torque we write the coupling energy of the magnetic moment and induced spin polarization as , where is defined as
[TABLE]
Taking the above into account, one can write the torque as a sum of a field-like torque \mbox{\boldmath\tau}_{f} and damping-like torque \mbox{\boldmath\tau}_{d},
[TABLE]
These components can be written in terms of the spin-orbit field as
[TABLE]
for the field-like term, and
[TABLE]
for the damping-like term. Since the spin polarization includes terms related to the Berry curvature, the resulting spin-orbit torques include terms related to the Berry curvature as well.
VII Summary and conclusions
Using the Matsubara Green function method we have calculated current-induced spin polarization in a magnetized two-dimensional electron gas with the Rashba spin-orbit interaction. The exchange field is shown to have a significant impact on the spin polarization. First, For some orientations of the exchange field, the component of spin polarization that appears in the absence of exchange field can be enhanced by the exchange field, while for other orientations this component can be suppressed. Second, exchange field also generates the components of spin polarization which are absent in the limit of vanishing exchange field. We also note, that the states at the band edges may become localized due to disorder and the results may be not valid in the localization regime.
Analytical and/or numerical results have been presented in some special cases, when exchange field is oriented along current or perpendicular to current (in-plane and perpendicular to the plane of 2DEG in the latter case). Numerical results have been also presented in a general case of arbitrary orientation of exchange field. We have found that the exchange field leads to terms in the spin polarization that can be related to the Berry curvature of the corresponding electron bands. Since the calculated spin polarization generates a torque which may induce dynamics of the magnetic moment, this torque includes terms related to the Berry curvature as well.
Acknowledgements.
This work was supported by the Polish Ministry of Science and Higher Education through a research project Iuventus Plus in years 2015-2017 (project No. 0083/IP3/2015/73). A.D. also acknowledges support from the Fundation for Polish Science (FNP). V.D. acknowledges support from the National Science Center in Poland under Grant No. DEC-2012/06/M/ST3/00042.
Appendix A Derivation of Eqs. (II.2), (II.2), (II.2)
The current induced spin polarizaton is evaluated starting from the equation (II.2) that we rewrite in the following form:
[TABLE]
where:
[TABLE]
and the following notation has been introduced:
[TABLE]
According to the above notation the component of spin polarization is described by the following expressions:
[TABLE]
[TABLE]
Inserting Eqs. (A), (A) into Eqs. (46) and (47) respectively we get:
[TABLE]
In the limit of we find component of current-induced spin polarization given by Eq.(II.2).
In turn, the component of spin polarization is expressed by the following functions:
[TABLE]
[TABLE]
After integration over in Eqs. (46) and (47) with integrands given by (A),(A) we obtain the following expression:
[TABLE]
In the limit we obtain the formula describing component of current-induced spin polarization given by Eq.(II.2).
Finally, the component of the nonequilibrium spin polarization is described by following traces:
[TABLE]
[TABLE]
These two equations combining with Eqs. (46) and (47) lead to the following expression:
[TABLE]
In the dc-limit we get Eq. (II.2).
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