Nonlinear Spectral Singularities and Laser Output Intensity
Hamed Ghaemi-Dizicheh, Ali Mostafazadeh, and Mustafa Sarisaman

TL;DR
This paper extends the concept of spectral singularities to nonlinear wave equations in laser physics, providing a mathematical framework to determine laser output intensity and conditions for lasing in slab lasers with Kerr nonlinearity.
Contribution
It introduces a nonlinear spectral singularity framework for slab lasers with Kerr nonlinearity, deriving explicit formulas for laser output and conditions for lasing thresholds.
Findings
Output intensity $I$ depends linearly on gain coefficient $g$
Explicit analytic expression for the slope of $I$ versus $g$
Lasing in oblique TM modes is forbidden beyond Brewster's angle
Abstract
The mathematical notion of spectral singularity admits a description in terms of purely outgoing solutions of a corresponding linear wave equation. This leads to a nonlinear generalization of this notion for nonlinearities that are confined in space. We examine the nonlinear spectral singularities in arbitrary TE and TM modes of a mirrorless slab laser that involves a weak Kerr nonlinearity. This provides a computational scheme for the determination of the laser output intensity for these modes. In particular, we offer an essentially mathematical derivation of the linear-dependence of on the gain coefficient and obtain an explicit analytic expression for its slope. This shows that if the real part of the refractive index of the slab does not exceed 3, there is a lower bound on below which lasing in both its TE and TM modes requires to be shifted by a…
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Nonlinear Spectral Singularities and Laser Output Intensity
Hamed Ghaemi-Dizicheh1, Ali Mostafazadeh1,2, , and Mustafa Sarısaman1
Departments of Physics1 and Mathematics2, Koç University,
34450 Sarıyer, Istanbul, Turkey Corresponding author, Email Address: [email protected]
Abstract
The mathematical notion of spectral singularity admits a description in terms of purely outgoing solutions of a corresponding linear wave equation. This leads to a nonlinear generalization of this notion for nonlinearities that are confined in space. We examine the nonlinear spectral singularities in arbitrary TE and TM modes of a mirrorless slab laser that involves a weak Kerr nonlinearity. This provides a computational scheme for the determination of the laser output intensity for these modes. In particular, we offer an essentially mathematical derivation of the linear-dependence of on the gain coefficient and obtain an explicit analytic expression for its slope. This shows that if the real part of the refractive index of the slab does not exceed 3, there is a lower bound on below which lasing in both its TE and TM modes requires to be shifted by a small amount as surpasses the threshold gain. Our results suggest that lasing in the oblique TM modes of the slab is forbidden if the incidence (emission) angle of the TM mode exceeds the Brewster’s angle.
Keywords: Spectral singularity, Kerr nonlinearity, nonlinear Helmholtz equation, lasing in TE and TM modes, Brewster’s angle, laser output intensity
1 Introduction
A planar slab does not reflect the transverse magnetic waves with an incident angle equal to Brewster’s angle , [1]. This well-known observation suggests that it should be extremely difficult for a mirrorless slab laser to emit a TM wave at the Brewster’s angle, because the internal reflections, whose number determines the optical path of the wave inside the slab, are essentially absent for such a wave. Ref. [2] establishes the validity of this prediction by deriving explicit formulas for the laser threshold condition governing arbitrary transverse electric (TE) and transverse magnetic (TM) modes of a homogeneous slab of gain material.
A closer look at the behavior of the singular waves, i.e., those generated at the threshold gain, reveals unexpected differences between the TM waves with and . For example, the energy density of these waves turns out to take larger values outside the slab for , while the converse is the case for TM waves with and TE waves with arbitrary . This observation will have physical significance, only if it applies also for the cases that the gain coefficient of the slab exceeds its threshold value so that the slab actually emits laser light. The purpose of the present article is to address this problem by offering a comprehensive analysis of the laser output intensity for general TE and TM modes of the slab laser.
The approach of [2] is based on the observation that the laser threshold condition can be derived as the condition for the presence of a spectral singularity [3]. This is originally demonstrated for the normally incident TE modes of a homogeneous slab in [4], and subsequently used to derive the laser threshold condition for active media of various geometries [5]. The first attempt at using this method for the description of obliquely incident TE modes of a homogeneous slab is due to Aalipour [6] whose results are improved and generalized to the TM waves in [2]. For other studies of physical aspects of spectral singularities, see [7, 8, 9, 10, 11, 12, 13, 14, 15, 16].
A related recent development is the introduction of a nonlinear generalization of the concept of spectral singularity [17]. This turns out to offer a simple effective description of the linear dependence of the laser output intensity on the gain coefficient [18]. Here the idea is to postulate the existence of a weak Kerr nonlinearity in the permittivity of the medium and use the condition for the emergence of a nonlinear spectral singularity to derive an expression for the intensity of the emitted waves. For both homogeneous [19] and symmetric bilayer slabs [20], this scheme yields
[TABLE]
where is the gain coefficient of the active component of the system, is its threshold value, is the Kerr coefficient, and is a function of the geometry and other parameters of the system. For other developments related to the optical applications of nonlinear spectral singularities, see [22, 21].
In the present article, we use nonlinear spectral singularities to offer a derivation of (1) for general TE and TM modes of a homogeneous slab. In particular, we give an explicit formula for and explore its physical consequences.
2 TE modes
Consider time-harmonic electromagnetic waves, and , interacting with an infinite homogeneous and isotropic planar slab of thickness that is aligned in the - plane. The inclusion of a Kerr nonlinearity amounts to having the permittivity of the slab given by
[TABLE]
where is the permittivity of the vacuum, is the complex refractive index of the slab in the absence of the nonlinearity, and is the Kerr coefficient [23].
For the TE waves, is parallel to the faces of the slab. We choose a coordinate system in which it is aligned along the -axis. We can then write and the wavevector in the form
[TABLE]
where , , and are respectively the unit vectors pointing along the positive -, -, and -axes,
[TABLE]
is the wavenumber, is the incidence angle depicted in Fig. 1, and is a function whose form is determined by Maxwell’s equations [24]. In view of (2) – (4), these reduce to
[TABLE]
where
[TABLE]
is the relative permittivity.
Let us introduce:
[TABLE]
Then according to (6) and (7),
[TABLE]
where satisfies the nonlinear Schrödinger equation:
[TABLE]
for .
Each solution of (10) determines a TE wave interacting with the slab provided that we impose appropriate boundary condition that fix and . These follow from the standard boundary conditions fulfilled by the electric and magnetic fields [24], i.e., their tangential component must be continuous at the interfaces. In light of (3) and (5), this implies that and are continuous functions at and . Therefore, we can apply the general formalism developed in Ref. [17] to describe the scattering of TE waves. In particular, the reflection and transmission amplitudes, and , for the left-incident TE waves are given by
[TABLE]
where
[TABLE]
and is the complex amplitude of the transmitted wave, so that for . This together with (9) imply
[TABLE]
Nonlinear spectral singularities correspond to real and positive values of for which
[TABLE]
Assuming that the strength of the nonlinearity is so small that we can ignore quadratic and higher order terms in , we can attempt to solve using first-order perturbation theory. For , i.e., normally incident TE waves, this has been done in Ref. [19]. It is easy to see that setting in (10) amounts to changing to . This in turn suggests that we can determine both the linear and nonlinear spectral singularities in arbitrary TE modes of our slab by replacing by in the analysis of the normally incident TE waves that is offered in Refs. [4, 19].
Using and to identify the values of and that yield a linear spectral singularity, introducing
[TABLE]
and substituting for in Eq. (8) of Ref. [4], we find
[TABLE]
Next, we denote the real and imaginary parts of (respectively ) by and (respectively and ), so that
[TABLE]
and recall that the gain coefficient of the slab is given by [18]:
[TABLE]
The threshold gain is the value of for and . We can determine and by equating the absolute-value and the phase of the left- and right-hand sides of (16), respectively, [2]. This gives the following expressions for the threshold gain and the wavenumber of the emitted wave:
[TABLE]
where is a positive integer (mode number) and is the phase angle (principal argument) of , [25].
Suppose that our slab is made of a typical high-gain (nongaseous) active material and that its thickness is much larger than the wavelength of the emitted wave, so that
[TABLE]
[TABLE]
where ‘’ labels approximate equalities in which we neglect the first and higher order terms in and the quadratic and higher order terms in powers of . Fig. 2 shows a plot of as a function of for and . For the wavelength , which is possible for , the approximate expression (22) for yields values that agree with the exact (numerical) values obtained directly using (16) to 6 significant figures.
Following a similar approach we can characterize the nonlinear spectral singularities in the oblique TE modes of the slab from those in its normally incident TE mode. To do this we express the values of and that give rise to a nonlinear spectral singularities in the form
[TABLE]
where and are respectively complex and real parameters. For a sufficiently weak nonlinearity, the -dependence of and is negligible. This suggests that we treat as a perturbation parameter and use first-order perturbation theory to compute and , and solve (14). This is done in Ref. [19] for . We can treat (14) for the case by setting and
[TABLE]
in Eq. (31) of [19]. This gives the following relation for the existence of a nonlinear spectral singularity.
[TABLE]
where is the time-averaged intensity of the emitted wave from the right, and
[TABLE]
Next, we introduce
[TABLE]
where ‘’ and ‘’ stand for the real and imaginary part of their argument, respectively. Then,
[TABLE]
and (26) is equivalent to
[TABLE]
These relations describe the nonlinear spectral singularities associated with a weak Kerr nonlinearity in the TE modes of our slab. In order to see how we can use them to relate the laser output intensity to the gain coefficient, we first recall that to the first order in the gain coefficient is given by [19]:
[TABLE]
This is a simple consequence of (18).
If we assume that the presence of the nonlinearity does not change the value of the refractive index , we have , and (32) and (33) reduce to
[TABLE]
Substituting these relations in (34) and making use of (8), we obtain (1) with given by
[TABLE]
Next, we expand the right-hand side of this relation in a power series in . Then using , (22), (21), and (36), we find
[TABLE]
For this relation reduces to
[TABLE]
Figure 2 shows the graph of the normalized threshold gain and as a function of for . We have checked that the graphs obtained using the exact and approximate expression for and are indistinguishable. As one increases , both and decrease monotonically. For , tends to zero while approaches .
Equations (37) and (38) reveal a surprising behavior; for , the intensity factor blows up at , where
[TABLE]
Furthermore, if and only if . These observations are easily validated using exact (numerical) treatments of (36) that do not rely on the condition (21).
The singular behavior of at shows that our first-order perturbative derivation of (1) with given by (36) is inapplicable for . The problem with negative values of is more serious. We can interpret it in either of the following alternative ways.
- •
It is a sign of the inapplicability of our derivation of (1) in terms of nonlinear spectral singularities.
- •
It suggests that a mirrorless slab made of gain material with does not actually lase in its TE modes with .
- •
It shows that making the gain coefficient exceed its threshold value does change the value of , i.e., the assumption that is false.
The latter interpretation calls for a generalization of (36) that does not rely on the condition: . Inserting (32) and (33) in (34) and making use of (8), we have
[TABLE]
where stands for the right-hand side of (36), i.e.,
[TABLE]
and
[TABLE]
To proceed further we need more information about the behavior of . Given that the refractive index is in principle a function of the frequency and therefore the wavenumber, we expect that the change in the value of , i.e., , is responsible for the change in , i.e., . Because , this suggests that
[TABLE]
where is a real parameter. Substituting this equation in (32) and solving for gives
[TABLE]
In view of (40) and (41), (39) coincides with (1) provided that we take
[TABLE]
A closer examination of this relation shows that for , there is a positive number such that the right-hand side of (42) becomes positive for all if and only if . For a sample with , , and , we have . Figure 3 shows a plot of as a function of . It reveals the fact that is a monotonically decreasing function of .
3 TM modes
3.1 Nonlinear Helmholtz Equation
For TM waves, we can write in terms of a scalar function according to
[TABLE]
Substituting this relation in Maxwell’s equations, we find
[TABLE]
where and are respectively the impedance and permeability of the vacuum. Equation (45) is to be solved subject to the following matching conditions [24].
[TABLE]
where stands for the left/right limit of as . Notice that because the relative permittivity depends on , there is a nonlinear coupling between Eqs. (44) and (43) and the matching conditions (46) and (47). This makes the the study of the TM modes much more complicated than that of the TE modes.
For , Eqs. (44), (43), (46), and (47) decouple and we have plane wave solutions. For , we can decouple the first of these equations from the rest. To do this we use (44) to compute and use (7) to show that is a root of the cubic polynomial:
[TABLE]
where
[TABLE]
Among the three roots of , only one vanishes for . Identifying with this root, we have
[TABLE]
where
[TABLE]
With the help of (7) and (49), we can express and the matching conditions (47) solely in terms of and .
We can also determine the relevant root of using perturbation theory. This yields the following expansion of the right-hand side of (49) in powers of .
[TABLE]
where stands for terms of order and higher in powers of .
In terms of the variables (8) we can express the solution of the Helmholtz equation (45) in the form
[TABLE]
where satisfies
[TABLE]
is given by
[TABLE]
and we have employed Eqs. (48) – (50).
In view of (46), (47), and (51), fulfills the boundary conditions:
[TABLE]
The and appearing in these equations are to be determined using (7), (49), and (54). These give
[TABLE]
In particular, with the help of (48) – (51) and (60), we can express and in terms of , and . Substituting these relations together with (56) and (58) in (57) and (59), we obtain a pair of decoupled nonlinear equations for and that we can, in principle, solve to express and in terms of and , respectively.
3.2 Spectral Singularities and Laser Output Intensity
According to (51), for a left-incident TM wave with outgoing complex amplitude ,
[TABLE]
and the reflection and transmission amplitudes are given by
[TABLE]
Using these relations to express and in terms of , , and , substituting the result together with (61) in (56) and (57), and solving them for and , we recover (11) with
[TABLE]
In particular, nonlinear spectral singularities for left-incident TM waves are again given by . Following the approach of Sec. 2 we seek a first-order perturbative solution of this equation where plays the role of the perturbation parameter. This requires expressing and in terms of . To do this we treat as the initial value of and use first-order perturbation theory to solve the initial-value problem defined by Helmholtz equation (52) and the boundary conditions (58) and (59), which in this context play the role of initial conditions. In view of (55), (60), and (61), they take the form:
[TABLE]
where
[TABLE]
Next, we apply first-order perturbation theory to determine the solution of the nonlinear Helmholtz equation (52) that satisfies (64) and (65). First, we note that this solution satisfies
[TABLE]
where is the solution of the linear Helmholtz equation, , that fulfils (64) and (65). It is easy to show that
[TABLE]
where
[TABLE]
Using for in the expression for that appears on the right-hand side of (67) and expanding the result in powers of give
[TABLE]
where
[TABLE]
and is to be computed by substituting for in (55).
Next, we use (63) and (73) to expand in powers of . In view of (60), this gives
[TABLE]
where
[TABLE]
We can use (69), (77), and (78) to show that
[TABLE]
where
[TABLE]
The linear spectral singularities correspond to the values of that fulfill , equivalently , where . For the typical gain media, which satisfy (21), reduces to
[TABLE]
In analogy with the TE modes, we can use this relation to determine the threshold gain for the TM modes. This is done in Ref. [2]. Here we quote the result:
[TABLE]
The wavenumber of the emitted radiation turns out to be given by (20) provided that we identify with the phase angle of .
Again, we can obtain more explicit expressions for and , if the gain medium fulfils (21). In this case, takes the form (20) and reads
[TABLE]
It is important to note that this relation holds only for the values of that are not too close to the Brewster’s angle, . In the vicinity of , the right-hand side of (83) takes arbitrarily large values. This violates (21) because, according to (18), is proportional to . Therefore, the approximation scheme leading to (83) fails [2].
To characterize nonlinear spectral singularities to the first order in , we suppose that
[TABLE]
where and are respectively -independent real and complex parameters. Inserting (84) in (76), expanding the result in powers of , neglecting the quadratic and higher order terms, enforcing , and making use of (77) – (81), we arrive at (26) with
[TABLE]
It is not difficult to see that and are independent of . In particular, if we assume that the presence of the nonlinearity does not affect the real part of the refractive index, i.e., set , we find that its intensity has the form (1) with given by (36). The only difference is that we must now use (85) and (86) to compute the right-hand side of (36).
Next, we try to obtain more explicit expressions for and . To determine , we insert (79) in (85) and make use of (81) and the definition of and to write the result in the form:
[TABLE]
The calculation of involves the use of a series of tricks that we outline in the appendix. The result is
[TABLE]
where is a function of , , and . We give its explicit expression in terms of , , and in the appendix. See Eq. (105) below.
Having determined the parameters and for the TM modes we can obtain the laser output intensity in these modes using (1) and (36), where and are respectively given by (87) and (88). In order to elucidate the physical meaning of the result, we confine our attention to gain material that satisfies (21). This allows us to neglect terms of order and , but not of , and provides the following approximate expression that is reliable for values of that are not in a close vicinity of Brewster’s angle .
[TABLE]
where
[TABLE]
For a sample with , we have compared the exact (numerical) values of with those given by (89) and found that the difference is smaller than .
Figure 4 shows the plots of the threshold gain and the normalized intensity factor (89) as a function of for this sample.
It reveals the curious fact that for , takes negative values. This observation suggests that a mirrorless slab cannot emit TM-polarized laser light having even if one fulfills the laser threshold condition (). Therefore the counterintuitive behavior of the singular TM waves with that is reported in [2], do not seem to have any physical implications.
For , (89) gives , where is the intensity factor for the normally-incident TE mode that is given by (38). The fact that for , this quantity diverges for some is a sign that the assumption, , is not valid. The situation is similar to the case of TE waves. Postulating the linear relation (40) between and resolves the difficulty with the divergence and negative values of for . It does not however affect the negativity of for .
4 Concluding Remarks
The output intensity of a homogeneous slab laser is known to be a linear function of the gain coefficient. In this article we offer a derivation of this relation and obtain the explicit form of the slope of the intensity for arbitrary TE and TM modes of a mirrorless slab laser. Our approach relies on two basic postulates:
- (i)
The emitted laser light is purely outgoing.
- (ii)
The interaction of the wave with the slab is described in terms of a weak Kerr nonlinearity.
Mathematically, these correspond to the emergence of a nonlinear spectral singularities [3, 17]. Imposing (i) in the absence of nonlinearity gives the laser threshold condition for the system. Demanding that it holds in the presence of a weak Kerr nonlinearity, i.e., enforcing (i) and (ii), allows for an analytic calculation of the laser output intensity . The effective description of the emission of the laser light that is provided by (i) and (ii) encodes all the underlying microscopic physical phenomena in a single small free parameter, namely the Kerr coefficient.
The linear dependence of on the gain coefficient follows from the observation that a first-order perturbation of the wavenumber, , induces a change in the real part of the refractive that is proportional to or equivalently . If the proportionality constant is smaller than a critical value , our analysis leads to a negative output intensity for sufficiently small emission angles . Furthermore, has the same sign as . For a mirrorless slab, we can fulfill the laser threshold condition provided that we use high-gain material which have a typically large refractive index. For , turns out to be at most of the order of . Therefore a very mild -dependence of the real part of the refractive index ensures a consistent application of our effective description of laser emission in both the TE and TM modes of the slab.
Our investigation reveals a drastic difference between the TE and TM modes. For the TM modes the laser output intensity vanishes at the Brewster’s angle and becomes negative for . This suggest that lasing in the TM modes of a mirrorless homogeneous slab is forbidden for . This is an experimentally checkable theoretical prediction that follows as a logical consequence of the postulates (i) and (ii).
Acknowledgments
This work has been supported by the Scientific and Technological Research Council of Turkey (TÜBİTAK) in the framework of the project no: 114F357, and by the Turkish Academy of Sciences (TÜBA).
Appendix: Calculation of for the TM modes
According to (86), the calculation of for the TM modes requires the computation of , , and . To achieve this, first we compute for , , and . For these values of and , we can use (69) and (81) to show that
[TABLE]
where
[TABLE]
If we set in (55) and use (90) and (91) to simplify the resulting expression for , we find
[TABLE]
where
[TABLE]
The following relations are straightforward consequences of (90) – (94).
[TABLE]
where is defined by (66). Now, we substitute (95) – (97) in (78) to obtain
[TABLE]
The computation of is much more complicated. First, we use (69), (74), and (77) to show that
[TABLE]
In view of (75), the integrand in (99) involves terms of the form and . By virtue of (81), these take the following simple form.
[TABLE]
where in the definition of and , i.e., (71) and (72), we set .
Next, we substitute (75) in (99), make use of (93), (100), and (101), and perform an integration by parts to obtain
[TABLE]
where
[TABLE]
In the derivation of (102) we have also made use of (97), (99), and the identities and , which follow from (81).
Equation (102) reduces the calculation of to that of . To do this, first we note that for ,
[TABLE]
Inserting (94) and (104) in (103), evaluating the resulting integral, and making extensive use of (81), we find
[TABLE]
where
[TABLE]
The final step of the computation of is the determination of . With the help of (79) – (81), we can easily show that . Substituting this relation together with (102) in (86) yields (88).
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