Self-Focusing Skyrmion Racetracks in Ferrimagnets
Se Kwon Kim, Kyung-Jin Lee, Yaroslav Tserkovnyak

TL;DR
This paper proposes a theoretical framework where inhomogeneous ferrimagnetic films near the angular momentum compensation point can guide skyrmions along self-focusing racetracks, enabling controlled skyrmion motion.
Contribution
It introduces the concept of using lines of zero angular momentum as self-focusing racetracks for skyrmions in ferrimagnets, with derived equations of motion and trajectory analysis.
Findings
Skyrmions can follow snake trajectories in nonuniform angular momentum density.
The equations of motion unify ferromagnetic and antiferromagnetic limits.
Self-focusing racetracks can be engineered using angular momentum profiles.
Abstract
We theoretically study the dynamics of ferrimagnetic skyrmions in inhomogeneous metallic films close to the angular momentum compensation point. In particular, it is shown that the line of the vanishing angular momentum can be utilized as a self-focusing racetrack for skyrmions. To that end, we begin by deriving the equations of motion for the dynamics of collinear ferrimagnets in the presence of a charge current. The obtained equations of motion reduce to those of ferromagnets and antiferromagnets at two special limits. In the collective coordinate approach, a skyrmion behaves as a massive charged particle moving in a viscous medium subjected to a magnetic field. Analogous to the snake orbits of electrons in a nonuniform magnetic field, we show that a ferrimagnet with the nonuniform angular momentum density can exhibit snake trajectories of skyrmions, which can be utilized as…
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Self-Focusing Skyrmion Racetracks in Ferrimagnets
Se Kwon Kim
Department of Physics and Astronomy, University of California, Los Angeles, California 90095, USA
Kyung-Jin Lee
Department of Materials Science and Engineering, Korea University, Seoul 02841, South Korea
KU-KIST Graduate School of Converging Science and Technology, Korea University, Seoul 02841, South Korea
Yaroslav Tserkovnyak
Department of Physics and Astronomy, University of California, Los Angeles, California 90095, USA
Abstract
We theoretically study the dynamics of ferrimagnetic skyrmions in inhomogeneous metallic films close to the angular momentum compensation point. In particular, it is shown that the line of the vanishing angular momentum can be utilized as a self-focusing racetrack for skyrmions. To that end, we begin by deriving the equations of motion for the dynamics of collinear ferrimagnets in the presence of a charge current. The obtained equations of motion reduce to those of ferromagnets and antiferromagnets at two special limits. In the collective coordinate approach, a skyrmion behaves as a massive charged particle moving in a viscous medium subjected to a magnetic field. Analogous to the snake orbits of electrons in a nonuniform magnetic field, we show that a ferrimagnet with the nonuniform angular momentum density can exhibit snake trajectories of skyrmions, which can be utilized as racetracks for skyrmions.
Introduction.—A free particle with the magnetic moment precesses at the frequency proportional to the applied magnetic field and its gyromagnetic ratio, which is the ratio of its magnetic moment to its angular momentum. When a magnet is composed of equivalent atoms, its net magnetization and net angular momentum density are collinear with the proportionality given by the gyromagnetic ratio of constituent atoms. Due to the linear relationship between them, the magnetization and the angular momentum density represent the same degrees of freedom, and thus are interchangeable in describing the magnetization dynamics. One-sublattice ferromagnets and two-sublattice antiferromagnets are examples of such magnets.
When a magnet consists of inequivalent atoms, however, its net magnetization and net angular momentum density can be independent degrees of freedom Wangsness (1953); *WangsnessPR1954; *WangsnessAJP1956. One class of such magnets is rare-earth transition-metal (RE-TM) ferrimagnetic alloys *[][; andreferencestherein.]KirilyukRPP2013, in which the moments of TM elements and RE elements tend to be antiparallel due to the exchange interaction. Because of different gyromagnetic ratios between RE and TM elements, one can reach the angular momentum compensation point and the magnetization compensation point, by varying the relative concentrations of the two species or changing the temperature. These compensation points are absent in the ferromagnets and antiferromagnets, which have been mainstream materials in spintronics Žutić et al. (2004); *JungwirthNN2016, and thus may bring a novel phenomenon to the field. In particular, we would like to focus on the dynamics of ferrimagnets around the angular momentum compensation point in this Letter for the following reason. Away from the compensation point, the dynamics of ferrimagnets is close to that of ferromagnets Andreev and Marchenko (1980). At the compensation point, its dynamics is antiferromagnetic Kirilyuk et al. (2013); Kim et al. . Therefore, the ideal place to look for the unique aspects of the dynamics of ferrimagnets would be close to, but not exactly at, the angular momentum compensation point.
Topological solitons in magnets *[][; andreferencestherein.]KosevichPR1990 have been serving as active units in spintronics. For example, a domain wall, which is a topological soliton in quasi-one-dimensional magnets with easy-axis anisotropy, can function as a memory unit, as demonstrated in the magnetic domain-wall racetrack memory Parkin et al. (2008). Two-dimensional magnets with certain spin-orbit coupling can also stabilize another particle-like topological soliton, which is referred to as a skyrmion. Skyrmions have been gaining attention in spintronics as information carriers, alternative to domain walls, because of fundamental interest as well as their practical advantages such as a low depinning electric current *[][; andreferencestherein.]NagaosaNN2013. Several RE-TM thin films such as GdFeCo and CoTb have been reported to possess the perpendicular magnetic anisotropy and the bulk Dzyaloshinskii-Moriya interaction Tono et al. (2015); Finley and Liu (2016), and thus are expected to be able to host skyrmions under appropriate conditions.
In this Letter, we study the dynamics of skyrmions in metallic collinear ferrimagnets, with a specific goal to understand and utilize the dynamics of skyrmions close to the angular momentum compensation point in RE-TM alloys. To that end, we first derive the equations of motion for the dynamics of general collinear magnets in the presence of an electric current. The resultant equations of motion reduce to those of ferromagnets and antiferromagnets at two limiting cases. The dynamics of a skyrmion is then derived within the collective coordinate approach Tretiakov et al. (2008); *TvetenPRL2013. Generally, it behaves as a massive charged particle in a magnetic field moving in a viscous medium. When there is a line in the sample across which the net angular momentum density reverses its direction, the emergent magnetic field acting on skyrmions also changes its sign across it. Motivated by the existence of a narrow channel in two-dimensional electron gas localized on the line across which the perpendicular magnetic field changes its direction Müller (1992); *ReijniersJPCM2000, we show that, under suitable conditions, the line of the vanishing angular momentum in RE-TM alloys can serve as a self-focusing racetrack for skyrmions Fert et al. (2013) as a result of combined effects of the effective Lorentz force and the viscous force. We envision that ferrimagnets with the tunable spin density can serve as a natural platform to engineer an inhomogeneous emergent magnetic field for skyrmions, which would provide us a useful knob to control them.
Main results.—The system of interest to us is a two-dimensional collinear ferrimagnet. Although the angular momentum can be rooted in either the spin or the orbital degrees of freedom, we will use the term, spin, as a synonym of angular momentum throughout for the sake of brevity. For temperatures much below than the magnetic ordering temperature, , the low-energy dynamics of the collinear ferrimagnet can be described by the dynamics of a single three-dimensional unit vector , which determines the collinear structure of the magnet Andreev and Marchenko (1980). Our first main result, which will be derived later within the Lagrangian formalism taken by Andreev and Marchenko (1980) for the magnetic dynamics in conjunction with the phenomenological treatment of the charge-induced torques Hals et al. (2011), is the equations of motion for the dynamics of in the presence of a charge current density and an external field to the linear order in the out-of-equilibrium deviations , , and :
[TABLE]
where is the net spin density along the direction of , and parametrize the dissipation power density and the inertia associated with the dynamics of , respectively, and is the effective field conjugate to with the potential energy 111In the supplemental material, the equations of motion for the dynamics of are derived more microscopically for two-sublattice collinear ferrimagnets, which provides us a concrete example of more general cases discussed in the main text.. Here, and are the phenomenological parameters for the adiabatic and nonadiabatic torques due to the current, respectively. It is instructive to interpret as the product of the dimensionless factor and the spin current density corresponding to the charge current density, , where is the electric charge of conducting electrons. Hereafter, the symbols with the tilde will denote the dimensionless quantities.
When the inertia vanishes, , the obtained equations of motion is reduced to the Landau-Lifshitz-Gilbert equation for ferromagnets augmented by the spin-transfer torques Slonczewski (1996); *BergerPRB1996; Zhang and Li (2004); *ThiavilleEPL2005, in which and can be identified as the Gilbert damping constant and the spin polarization rate of conducting electrons, respectively. When the net spin density vanishes, , it corresponds to the equations of motion for antiferromagnets Hals et al. (2011). The equations of motion for the dynamics of a two-sublattice ferrimagnet in the absence of an electric current and dissipation, and , has been obtained by lvanov and Sukstanskii (1983).
The low-energy dynamics of rigid magnetic solitons in two-dimensional collinear magnets can be derived from Eq. (1) within the collective coordinate approach Tretiakov et al. (2008), where the dynamics of the order parameter is encoded in the time evolution of the soliton position, . The resultant equations of motion for the position of a circularly symmetric soliton, which are obtained by integrating Eq. (1) multiplied by over the space, are our second main result:
[TABLE]
where is the soliton mass 222Relaxation of the rigidity approximation for the soliton structure will give rise to additional contributions to its mass from the internal fast modes Makhfudz et al. (2012). Therefore, understanding the dynamics of general solitons would require us to consider the mass as a parameter that can be different from the given expression., is the viscous coefficient, is the internal force, is the force due to the charge current. The first term on the right-hand side is the effective Lorentz force on the soliton, which is proportional to its topological charge
[TABLE]
which measures how many times the unit vector wraps the unit sphere as spatially varies Belavin and Polyakov (1975), and the fictitious magnetic field
[TABLE]
According to the equations of motion, a skyrmion in chiral ferrimagnets, which is characterized by its topological charge , behaves as a massive charged particle in a magnetic field moving in a viscous medium. The fictitious magnetic field is proportional to the net spin density along the direction of the order parameter , which leads us to consider collinear magnets with tunable to look for a possibly interesting dynamics of a skyrmion. The RE-TM ferrimagnetic alloys Kirilyuk et al. (2013) are such materials. For example, Co1-xTbx has been shown to exhibit the vanishing angular momentum at % at room temperature Finley and Liu (2016) by varying the chemical composition. As another example, the angular momentum compensation temperature of Gd22%Fe75%Co3% has been reported as K Stanciu et al. (2006).
A skyrmion can be driven by an electric current as can be seen in Eq. (2). In the presence of the corresponding current-induced force , the direction of which is defined as the axis, the steady state of a skyrmion is given by
[TABLE]
See Fig. 1 for illustrations of a steady-state skyrmion motion for . The skyrmion with the topological charge moves down for and up for , while moving to the right regardless of the sign of . If the ferrimagnet is prepared in such a way that for and for , the skyrmion with will move along the horizontal line after certain relaxation time because it is constantly pushed back to the line via the effective Lorentz force. Note that the skyrmion experiences no Lorentz force on the angular momentum compensation line, and thus will move as an antiferromagnetic skyrmion along it Barker and Tretiakov (2016); *ZhangSR2016.
To corroborate the qualitative prediction, we numerically solve the equations of motion [Eq. (2)] in its dimensionless form:
[TABLE]
in which time, length, and energy are measured in units of the relaxation time , the characteristic length scale for the skyrmion size 333For example, the energy density, , yields the characteristic length scale for the skyrmion radius, Bogdanov and Yablonskii (1989)., and , respectively, where is a dimensionless number determined by the skyrmion structure. Figure 2(a) shows the two trajectories of skyrmions of the charge departing from and with the zero initial velocity under the following configurations: , , and . We refer the paths as skyrmion snake trajectories due to their shapes, analogous to the electronic snake orbits in an inhomogeneous magnetic field Müller (1992). The inset shows that the skyrmion speed converges as after sufficiently long time, . Figure 2(b) depicts multiple trajectories of skyrmions when the net spin density is spatially periodic, . Skyrmions are attracted to the angular momentum compensation lines and their velocities converge to the finite value. This leads us to state our third main result: self-focusing narrow guides for skyrmions can be realized in certain ferrimagnets such as the RE-TM alloys along the lines of the angular momentum compensation points, which can be useful in using skyrmions for information processing by, e.g., providing multiple parallel skyrmion racetracks in one sample Tomasello et al. (2014).
The dynamics of collinear magnets.—The derivation of the equations of motion for the dynamics of collinear magnets in [Eq. (1)] is given below, which follows the phenomenological approach taken for antiferromagnets by Andreev and Marchenko (1980). Within the exchange approximation that the Lagrangian is assumed invariant under the global spin rotations, we can write the Lagrangian density for the dynamics of the directional order parameter in the absence of an external field as
[TABLE]
to the quadratic order in the time derivative, where is the vector potential for the magnetic monopole, Ivanov and Sukstanskii (1984); *LossPRL1992. The first term accounts for the spin Berry phase associated with the net spin density along ; The second term accounts for the inertia for the dynamics of , which can arise due to, e.g., the relative canting of the sublattice spins Note (1).
Next, the effects of an external field can be taken into account as follows. The conserved Noether charge associated with the symmetry of the Lagrangian under the global spin rotations is the net spin density, and it is given by . The magnetization in the presence of an external field can be then written as , where and are the gyromagnetic ratios for the longitudinal and transverse components of the spin density with respect to the direction , respectively, and is the magnetic susceptibility tensor. The relation, Andreev and Marchenko (1980), requires the susceptibility to be , with which the Lagrangian is extended to
[TABLE]
where includes the Zeeman term, . Finally, the dissipation can be accounted for by the Rayleigh dissipation function, , which is the half of the dissipation rate of the energy density, . The equations of motion obtained from the Lagrangian and the Rayleigh dissipation function are given by Eq. (1) without the current-induced torques.
Current-induced torques.—To derive the torque terms due to an electric current, it is convenient to begin by phenomenologically constructing the expression for the charge current density induced by the magnetic dynamics, and subsequently to invoke the Onsager’s reciprocity to obtain the torque terms as done for antiferromagnets in Ref. Hals et al. (2011). To the lowest order of the space-time gradients and to the first order in the deviations from the equilibrium, we can write two pumping terms that satisfy the appropriate spatial and spin-rotational symmetries: and . The resultant expression for the induced current density is given by
[TABLE]
where is the conductivity.
To invoke the Onsager reciprocity that is formulated in the linear order in the time derivative of the dynamic variables, we turn to the Hamiltonian formalism instead of the Lagrangian formalism. We shall restrict ourselves here to the case of a vanishing external field for simplicity, but it can be easily generalized to the case of a finite external field. The canonical conjugate momenta of is given by . The Hamiltonian density is then given by
[TABLE]
which resembles the Hamiltonian for a charged particle subjected to an external magnetic field Goldstein et al. (2002). The Hamilton equations are given by
[TABLE]
where and are conjugate fields to and , respectively. In terms of the conjugate fields, the pumped charge current is given by . By using the Onsager reciprocity and Ohm’s law for the current , we can obtain the torque terms in Eq. (1).
Discussion.—Let us discuss approximations that have been used in the Letter. First, we have developed the theory for the dynamics of collinear magnets within the exchange approximation Andreev and Marchenko (1980), in which the total energy is invariant under the simultaneous rotation of the constituent spins. The relativistic interactions including the magnetic anisotropy, which weakly break the exchange symmetry of the magnet, are added phenomenologically to the potential energy. Secondly, when studying the dynamics of skyrmions in inhomogeneous ferrimagnetic films, we have considered the nonuniform spin density , while neglecting possible spatial variations of the other parameters such as the inertia or the damping because we do not expect those variations to change the results qualitatively. As long as skyrmions are attracted to the line of vanishing angular momentum due to the combined effects of the effective Lorentz force, the viscous force, and the current-induced force, the line should be able to convey skyrmions along with it.
Ferrimagnetic RE-TM alloys have not only the angular momentum compensation point, which we have focused on in this Letter, but also the magnetic moment compensation point. Motivated by the attraction of skyrmions toward the angular momentum compensation lines that we have discussed, it would be worth looking for an interesting phenomenon that can occur on the magnetic moment compensation line. For example, since the magnetic moment governs the magnetostatic energy, there may be unusual magnetostatic spin-wave modes Damon and Eshbach (1961); *DamonJAP1965 localized at the line. In addition, we have considered the dynamics of a soliton in two-dimensional ferrimagnets driven by an electric current. In general, the dynamics of a soliton can be induced by other stimuli such as an external magnetic field Schryer and Walker (1974) and a spin-wave excitation Hinzke and Nowak (2011); *YanPRL2011; *KovalevEPL2012; Tveten et al. (2014); Kim et al. (2014), which may exhibit peculiar features of ferrimagnets that are absent in ferromagnets and antiferromagnets.
Acknowledgements.
This work was supported by the Army Research Office under Contract No. W911NF-14-1-0016 (S.K.K. and Y.T.) and by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIP) (2015M3D1A1070465) (K.-J.L.).
Appendix A Supplemental Material
In this supplemental material, we derive the equations of motion for a two-sublattice ferrimagnet by following the approach taken in Ref. Hals et al. (2011) with the explicit treatment of two sublattices.
The model system is a two-dimensional collinear magnet that consists of two inequivalent sublattices. The local spin densities of the two sublattices are denoted by and , where and are slowly varying unit vectors. We allow the two scalar spin densities, and , to be either positive and negative, which is useful to construct a general theory for collinear magnets as will be shown below. In equilibrium, the two spin densities are collinear, which we represent by . To describe the dynamics of the magnet, it is convenient to use the new vectors, and , instead of and , and the new scalars, and , instead of and . Here, serves as the order parameter, which captures the collinear structure in equilibrium; corresponds to the relative canting of the two sublattices, which vanishes in equilibrium; and are the net and the staggered spin densities in equilibrium, respectively. The cases where the two sublattices are coupled by a ferromagnetic exchange can be represented by , for which is the direction of the net spin density in equilibrium. The cases of an antiferromagnetic exchange can be represented by , for which is the direction of the staggered spin density in equilibrium. From the definitions, we obtain , and, for small deviations from the equilibrium, we can impose the constraints and Hals et al. (2011). Without loss of generality, we can assume . See Fig. S1 for illustrations of possible types of collinear structures.
Let us first derive the equations of motion in the absence of an electric current within the Lagrangian formalism. The spin Berry phase contribution to the Lagrangian density, which governs the magnetic dynamics, is given by
[TABLE]
where is a vector potential for magnetic monopoles, which satisfies . By expanding the spin Berry phase to the second order in and as done in Ref. Kim et al. (2014), we obtain
[TABLE]
The first term comes from the net spin Berry phase, which is in the Lagrangian for ferromagnets; The second term comes from the cancelation of the spin Berry phases of the two sublattices, which is in the Lagrangian for antiferromagnets; the third term shall be ignored over the first term for the slow dynamics. The total Lagrangian density is given by . The dissipation can be accounted for by the Rayleigh dissipation function, , which is the half of the dissipation rate of the energy density, . Here, we consider the dissipation associated with the dynamics of the order parameter , while neglecting the contribution from the dynamics of assuming . The equations of motion for the fields and can be obtained from the Lagrangian and the Rayleigh dissipation function Goldstein et al. (2002):
[TABLE]
where and are the effective fields conjugate to and , respectively.
By using the Onsager reciprocity as done in the main text, we can obtain the torque terms in the equations of motion:
[TABLE]
Within the exchange approximation that the energy is invariant under the global spin rotations, the free energy expanded to the second order in the gradients and the relative canting is given by , where represents the magnetic susceptibility, is the stiffness associated with the spatial change of , , , and is a static external magnetic field. Here, and are the magnetizations of the two sublattices, where and are their gyromagnetic ratios. Using , we can remove from the equations of motion, which results in Eq. (1) with .
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