Boundary-driven Lindblad dynamics of random quantum spin chains : strong disorder approach for the relaxation, the steady state and the current
Cecile Monthus

TL;DR
This paper investigates the non-equilibrium dynamics of a disordered quantum spin chain under boundary-driven Lindblad evolution, providing explicit calculations of the steady-state magnetization profile and current using a strong disorder renormalization approach.
Contribution
It introduces a strong disorder boundary-strong-disorder renormalization method to analyze relaxation, steady states, and currents in boundary-driven disordered quantum spin chains.
Findings
Magnetization follows a step profile in localized chains.
Explicit formulas for the magnetization step and current are derived.
The approach applies to systems with large random fields and various couplings.
Abstract
The Lindblad dynamics of the XX quantum chain with large random fields (the couplings can be either uniform or random) is considered for boundary-magnetization-drivings acting on the two end-spins. Since each boundary-reservoir tends to impose its own magnetization, we first study the relaxation spectrum in the presence of a single reservoir as a function of the system size via some boundary-strong-disorder renormalization approach. The non-equilibrium-steady-state in the presence of two reservoirs can be then analyzed from the effective renormalized Linbladians associated to the two reservoirs. The magnetization is found to follow a step profile, as found previously in other localized chains. The strong disorder approach allows to compute explicitly the location of the step of the magnetization profile and the corresponding magnetization-current for each disordered sample…
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Boundary-driven Lindblad dynamics of random quantum spin chains :
strong disorder approach for the relaxation, the steady state and the current
Cécile Monthus
Institut de Physique Théorique, Université Paris Saclay, CNRS, CEA, 91191 Gif-sur-Yvette, France
Abstract
The Lindblad dynamics of the XX quantum chain with large random fields (the couplings can be either uniform or random) is considered for boundary-magnetization-drivings acting on the two end-spins. Since each boundary-reservoir tends to impose its own magnetization, we first study the relaxation spectrum in the presence of a single reservoir as a function of the system size via some boundary-strong-disorder renormalization approach. The non-equilibrium-steady-state in the presence of two reservoirs can be then analyzed from the effective renormalized Linbladians associated to the two reservoirs. The magnetization is found to follow a step profile, as found previously in other localized chains. The strong disorder approach allows to compute explicitly the location of the step of the magnetization profile and the corresponding magnetization-current for each disordered sample in terms of the random fields and couplings.
I Introduction
In the field of random quantum spin chains, the interplay of disorder and dissipation has attracted a lot of attention recently. As a first example, the coupling to a dissipative bath of harmonic oscillators with some spectral function as in the spin-boson model [1] has been analyzed via Strong Disorder Renormalization [2, 3, 4, 5, 6, 7, 8, 9]. As a second example, the Lindblad dynamics with boundary-driving and/or dephasing has been studied for Many-Body-Localization models in various regimes [10, 11, 12, 13, 14, 15].
Among the various descriptions of open quantum systems [16], one of the most effective is indeed the Lindblad equation for the density matrix
[TABLE]
where the Lindblad operator contains the unitary evolution as if the system of Hamiltonian were isolated
[TABLE]
and the dissipative contribution defined in terms of some set of operators that describe the interaction with the reservoirs (see example in section II)
[TABLE]
so that the trace of the density matrix is conserved by the dynamics
[TABLE]
The first advantage of this formulation of the dynamics as a Quantum Markovian Master Equation is that the relaxation properties can be studied from the spectrum of the Lindblad operator [17, 18, 19] with possible metastability phenomena [20]. This spectral analysis also allows to make some link with the Random Matrix Theory of eigenvalues statistics [21]. The second advantage is that this framework is very convenient to study the non-equilibrium transport properties [23, 24, 25, 26, 27, 28, 29, 30, 31] with many exact solutions [32, 33, 34, 35, 36, 37]. In addition, many important ideas that have been developed in the context of classical non-equilibrium systems (see the review [38] and references therein) have been adapted to the Lindblad description of non-equilibrium dissipative quantum systems, in particular the large deviation formalism to access the full-counting statistics [39, 40, 41, 42, 43, 44, 45, 46], the additivity principle [47] and the fluctuation relations [48].
In the present paper, we consider the XX chain of spins with random fields and couplings (that can be either uniform or random)
[TABLE]
and analyze the Lindblad dynamics in the presence of two boundary-magnetization-drivings acting on the two end-spins. We focus on the strong disorder regime where the scale of the random fields is much bigger than the couplings . The paper is organized as follows. In section II, we introduce the notations for the boundary-magnetization-drivings and we recall the spectral analysis of the Lindbladian in the ladder formulation, as well as the notion of tilted-Lindbladian to access the full-counting statistics of the exchanges with one reservoir. In section III, we show how this formalism works in practice on the simplest case of spins. We then turn to the case of a chain of arbitrary length : in section IV, we analyze the relaxation properties of a long chain in contact with a single reservoir, while in section V, we analyze the non-equilibrium-steady-state for the chain coupled to two reservoirs : the magnetization profile and the magnetization current are computed in the strong disorder regime. Our conclusions are summarized in section VI.
II Lindblad dynamics with boundary-magnetization-driving
II.1 Boundary-magnetization-driving on the end-spins and
The standard boundary-magnetization-driving on the first spin is based on the dissipative operator of Eq. 3 with the two operators
[TABLE]
and the corresponding amplitudes
[TABLE]
leading to
[TABLE]
Using the identities
[TABLE]
Eq 8 becomes
[TABLE]
The physical meaning of this dissipative operator is that it tends to impose the magnetization on the spin 1 with a characteristic relaxation rate of order .
A simple way to generate a non-equilibrium steady-state is to consider a similar boundary-magnetization-driving on the last spin that tend to impose another magnetization with some rate , so that the corresponding dissipative operator reads
[TABLE]
II.2 Ladder Formulation of the Lindbladian
Since the Lindblad operator acts on the density matrix of the chain of spins that can be expanded in the basis
[TABLE]
in terms of the coefficients
[TABLE]
it can be technically convenient to ’vectorize’ the density *matrix * of the *spin chain * [19, 47, 49, 50, 51], i.e. to consider that these coefficients are the components of a *ket * describing the state of a *spin ladder *
[TABLE]
To translate the Lindblad operator of Eq. 1 in this ladder formulation, one needs to consider the product where and are two arbitrary matrices
[TABLE]
and to write the corresponding ket
[TABLE]
where denotes the transpose of the matrix . As a consequence, the Lindblad operator governing the evolution of the ket
[TABLE]
can be translated from Eqs 2 and 3 and reads
[TABLE]
For the chain of Eq. 5, the unitary part reads in terms of the Pauli matrices of the spin ladder
[TABLE]
while the dissipative operators of Eqs 8 and 11 become
[TABLE]
and
[TABLE]
II.3 Spectral Decomposition of the Ladder Lindbladian
The ladder formulation of the Lindbladian described above is especially useful to use the very convenient bra-ket notations to denote the Right and Left eigenvectors associated to the eigenvalues
[TABLE]
with the orthonormalization
[TABLE]
and the identity decomposition
[TABLE]
The spectral decomposition of the Lindbladian
[TABLE]
then allows to write the solution for the dynamics in terms of the initial condition at as
[TABLE]
The trace of the density matrix corresponds in the Ladder Formulation to
[TABLE]
Its conservation by the dynamics (Eq 4) means that the eigenvalue
[TABLE]
is associated to the Left eigenvector
[TABLE]
while the corresponding Right Eigenvector corresponds to the steady state towards which any initial condition will converges
[TABLE]
The other eigenvalues with negative real parts describe the relaxation towards this steady state.
II.4 Tilted-Lindbladian to measure the exchanges with the boundary-reservoir on spin 1
As mentioned in the Introduction, the method of ’tilting’ the master equation to access the full-counting statistics developed for classical non-equilibrium models (see the review [38] and references therein) has been adapted to the Lindblad framework [39, 40, 41, 42, 43, 44, 45, 46, 47] as follows. To keep the information on the global number of ’magnetization particles’ that have been exchanged with the reservoir acting on the spin 1 since the initial condition at , it is convenient to decompose the Lindbladian into three terms
[TABLE]
where
[TABLE]
describe respectively the processes corresponding to an increase () and a decrease () by an elementary ’magnetization particle’, while contains all the other terms of the Lindbladian that do not correspond to an exchange with the reservoir acting on spin 1 (). As a consequence, the eigenvalue with the largest real-part of the tilted-Lindbladian by the parameter
[TABLE]
allows to obtain the statistics of the number in the large-time regime via
[TABLE]
In particular, the expansion up to second order in
[TABLE]
gives the averaged current entering from the reservoir acting on the spin 1
[TABLE]
and the fluctuation
[TABLE]
More generally, the whole large-deviation properties of the probability distribution of the current
[TABLE]
can be obtained as the Legendre transform of the tilted eigenvalue of Eq. 34
[TABLE]
II.5 Notation
In the remaining of this paper, the ladder formulation of the Lindblad operator described above will be always used, so that the explicit mention ’Ladder’ will be dropped from now on in order to simplify the notations.
III Strong-Disorder Approach for spins
To see how the formalism recalled in the previous section works in practice, it is useful to focus first on the simplest example of spins. In addition, to motivate the Strong-Disorder approach for long chains that will be described in the following sections, we will consider that the only term of the Linbladian that couples the two spins
[TABLE]
is a perturbation with respect to all the other terms that do not couple the two spins
[TABLE]
III.1 Spectral decomposition of
The tilted Lindbladian of Eq. 31 for the spin 1
[TABLE]
has the following four eigenvalues that do not depend on the tilting parameter in contrast to some corresponding eigenvectors written in the basis :
(0) The eigenvalue is associated to
[TABLE]
(1) The eigenvalue is associated to
[TABLE]
(2) The eigenvalue is associated to
[TABLE]
(4) The eigenvalue is associated to
[TABLE]
III.2 Spectral decomposition of
The non-tilted Lindbladian for the spin
[TABLE]
has the following four eigenvalues and eigenvectors in the basis :
(0) The eigenvalue is associated to
[TABLE]
(1) The eigenvalue is associated to
[TABLE]
(2) The eigenvalue is associated to
[TABLE]
(4) The eigenvalue is associated to
[TABLE]
III.3 Second-Order perturbation theory in the coupling
The unperturbed Lindbladian of Eq. 41 is the sum of the two independent Lindbladians discussed above, so its 16 eigenvalues are simply given by the sum of eigenvalues for and
[TABLE]
while the left and right eigenvectors are given by the corresponding tensor-products
[TABLE]
Here we are interested into the eigenvalue with the largest real part of the tilted Lindbladian (Eq. 33). The corresponding unperturbed eigenvalue vanishes
[TABLE]
but it will become non-zero and depend on the parameter when the coupling between the two spins is taken into account by the second-order perturbation theory
[TABLE]
The application of the perturbation to the left unperturbed eigenvector
[TABLE]
and to the right unperturbed eigenvector
[TABLE]
shows that the formula of Eq. 53 only involves the two intermediate states and with the unperturbed complex-conjugated eigenvalues
[TABLE]
and becomes
[TABLE]
where we have introduced the notation
[TABLE]
III.4 Averaged current and fluctuations
The expansion of the eigenvalue of Eq. 57 up to second order in (Eq. 35)
[TABLE]
yields the averaged current (Eq 36)
[TABLE]
and the fluctuation (Eq 37)
[TABLE]
III.5 Large deviations
To compute the function that governs the large-deviation form of the probability distribution of the current (Eq. 38), we need the Legendre transform of Eq. 39
[TABLE]
where is the location of the maximum determined by the solution of the equation
[TABLE]
Since this is a second-order equation in the variable
[TABLE]
with the discriminant
[TABLE]
one obtains that the positive roots reads
[TABLE]
so that the large deviation function of Eq. 62 finally reads
[TABLE]
It vanishes at of Eq. 60 as it should.
III.6 Discussion
In summary, besides the magnetizations and of the boundary drivings, the important parameter in the averaged current , in the fluctuation and more generally in the whole large-deviation function is the parameter introduced in Eq. 58 that contains the difference of the two random fields in the denominator. In the remaining of the paper, we focus on the ’Strong-Disorder regime’ where the scale of the random fields is much bigger than the scale of the couplings that can be either uniform or random
[TABLE]
so that it is valid to use perturbation theory in the hoppings to evaluate various observables, as shown in this section on the example of spins.
IV Renormalization approach for the relaxation with a single reservoir
When the quantum chain of spins is subject to the single boundary-magnetization-driving (Eq 20) of parameters on the spin 1 (while there is no driving on the last spin ), the stationary state is the trivial tensor-product with the magnetization for all spins
[TABLE]
but it is nevertheless interesting to analyze the behavior of the relaxation rate as a function of the system size .
IV.1 Boundary Strong Disorder Renormalization for the relaxation rate
The idea is that in the Strong Disorder regime for the random fields (Eq. 68), there exists a strong hierarchy between the relaxation rates
[TABLE]
i.e. the first spin in contact with the reservoir is the first to equilibrate with rate , then the second spin will equilibrate with some slower rate , and so on. The aim is thus to introduce a Boundary Strong Disorder Renormalization procedure in order to compute iteratively the relaxation rates .
So we decompose the Lindbladian for the chain of spins into
[TABLE]
in order to take into account the coupling term by perturbation theory in the hopping .
IV.2 Structure of the four lowest modes of
When the strong hierarchy of Eq. 70 exists, one may restrict the Lindbladian to its four lowest modes
[TABLE]
that have the following structure for the last spin (while all the previous spins have already relaxed towards equilibrium) :
(0) The vanishing eigenvalue representing the equilibrium is associated to the left an right eigenvectors
[TABLE]
(1) The real eigenvalue is associated to
[TABLE]
(2-3) The complex eigenvalue is associated to
[TABLE]
while the complex-conjugate eigenvalue is associated to
[TABLE]
IV.3 Properties of the unperturbed Lindbladian
The lowest modes sector of the decoupled unperturbed Lindbladian reads
[TABLE]
so that its eigenstates are simply tensor-products of eigenstates of each term
[TABLE]
and the corresponding eigenvalues are simply the sums
[TABLE]
In particular, the four eigenvalues corresponding to (with and ) have no real part as a consequence of . After taking into account the perturbation of Eq. 71, these four eigenvalues will correspond to the four slowest modes of , with the structure analog to Eq. 72.
Since the perturbation has no diagonal contribution, we need to consider the second-order perturbation theory for the eigenvalues. Let us first consider the two complex-conjugate non-degenerate eigenvalues
[TABLE]
before we turn to the two-dimensional degenerate subspace
[TABLE]
IV.4 Second-Order Perturbation for
the two imaginary non-degenerate eigenvalues
In this section, we focus on the two imaginary complex-conjugate non-degenerate eigenvalues of Eq. 80. The unperturbed eigenvalue
[TABLE]
corresponding to the left and right unperturbed eigenvectors (Eq. 78)
[TABLE]
has the following second-order perturbation correction
[TABLE]
The application of the perturbation of Eq. 71 on the left and right eigenvectors yield
[TABLE]
So the sum of Eq. 84 contains only two terms corresponding to the unperturbed eigenvalues
[TABLE]
and finally reads
[TABLE]
For the other complex-conjugate unperturbed eigenvalue
[TABLE]
the second-order perturbation is similar and yields of course the complex-conjugate result of Eq. 87
[TABLE]
In summary, the identification of these two complex-conjugate eigenvalues
[TABLE]
leads to the following recurrences for the two variables
[TABLE]
and
[TABLE]
IV.5 Perturbation in the two-dimensional degenerate subspace
Within the two-dimensional degenerate subspace associated to the projector
[TABLE]
the second-order perturbation theory corresponds to the effective operator (that generalizes the non-degenerate perturbation formula of Eq. 84)
[TABLE]
The application of the perturbation of Eq. 71 on the left and right eigenvectors yield respectively
[TABLE]
and
[TABLE]
As a consequence, Eq. 94 contains only two intermediate states that are associated to the unperturbed eigenvalues
[TABLE]
and becomes
[TABLE]
In terms of the notation introduced in Eq. 91, the four corresponding matrix elements read
[TABLE]
[TABLE]
[TABLE]
[TABLE]
So the two-by-two matrix can be factorized into
[TABLE]
where
[TABLE]
represents the eigenvalue associated to the right and left eigenvectors
[TABLE]
while the vanishing eigenvalue corresponds to the right and left eigenvectors
[TABLE]
IV.6 Validity of the Strong Disorder Approach
In summary, we have obtained the recurrences of Eqs 91, 92 for the two variables that characterize the structure of the four slowest modes described in sec IV.2. The above perturbative calculation is valid in the strong disorder regime for the random fields (Eq. 68) that leads to a strong hierarchy between the relaxation rates (Eq. 70). When this is the case, the relaxation rate decays with and can be neglected with respect to the difference of random fields in the denominators of the recurrences of Eqs 91 and 92 that becomes
[TABLE]
and
[TABLE]
At leading order in the strong disorder regime for the random fields, one further obtains that can be neglected with respect to the difference of random fields in the denominators leading to the simple value for the correction to the imaginary part
[TABLE]
and to the simplified multiplication recurrence for the relaxation rates alone
[TABLE]
This result clearly shows that the hypothesis of Eq. 70 concerning the strong hierarchy between two sucessive relaxation rates is satisfied in the strong disorder regime (Eq. 68), so that the renormalization procedure described in the present section is fully consistent.
In terms of the initial relaxation rate and of the random fields and random couplings , the relaxation rate is then simply given by the product
[TABLE]
so that its logarithm corresponds to a sum of independent random variables
[TABLE]
The Central Limit Theorem then yields that the distribution of over the disordered samples is Gaussian with the average
[TABLE]
and the variance
[TABLE]
V Non-equilibrium steady states between two reservoirs
V.1 Non-equilibrium magnetization profile between two reservoirs
Although the simplest expectation for a non-equilibrium steady-state between two reservoirs would be a linear magnetization profile as in the Fourier-Fick-diffusive standard result, it should be stressed that the completely opposite situation of a step-magnetization profile with a ’shock’ has been found in various regimes [22, 29, 30] and in particular in the presence of disorder as a consequence of the localization phenomenon [15]. In the strong disorder regime that we consider, we also expect that the magnetization profile will have a step-profile : the magnetization will remain near for the spins , while it will remain near for the other spins . In this section, our goal is to determine the location of the step as a function of the random fields of the sample. This step magnetization profile means that the reservoir acting on the spin 1 is actually able to impose its magnetization on all the spins , while the other reservoir acting on the spin N is actually able to impose its magnetization on all the spins , so that we may directly use the results of the previous section concerning the relaxation in the presence of a single reservoir :
(i) For the spin , the effective Lindbladian describing the influence of the left reservoir acting on spin 1 reads in terms of the four states of the ladder formulation
[TABLE]
with the relaxation rate given by Eq. 111
[TABLE]
(ii) Similarly, for the spin , the effective Linbladian describing the influence of the right reservoir acting on spin reads
[TABLE]
with the relaxation rate given by the appropriate adaptation of Eq. 111
[TABLE]
(iii) Taking into account the random field , one finally obtain that the total effective Lindbladian acting on the spin reads
[TABLE]
So the global relaxation rate corresponds to the sum
[TABLE]
while the effective magnetization that the combination of the two reservoirs tend to impose on site can be obtained from the identification
[TABLE]
leading to the weighted average
[TABLE]
The same approach for the other spin on the other side of the step yields
[TABLE]
This step magnetization profile approximation will be valid if
[TABLE]
and the location of the step correspond to the location where there is a change of the dominant reservoir in the weighted average. For instance, for the standard example of opposite boundary magnetizations and equal boundary-rates , the location of the step corresponds to the index where there is a sign change in the difference
[TABLE]
So while the average position of the step is at the middle of the chain by symmetry, there are sample-to-sample fluctuations of order as a consequence of the statistical properties discussed after Eq. 111.
V.2 Non-equilibrium magnetization current between two reservoirs
Within the picture of the step-magnetization-profile located on the bond described above, the analysis of the current is actually similar to the two-spin problem described in detail in section III. The important parameter of Eq. 58 becomes
[TABLE]
in terms of the relaxation rates and given by Eqs. 116 and 118. Since they are small, they can be neglected in the denominator with respect to the random fields, so that the parameter reads at leading order in the strong disorder regime
[TABLE]
where the location of the step has been discussed after Eq. 124 : the two products in the parenthesis are then roughly of the same order. As a consequence, the averaged current and the fluctuation given by Eqs 60 and 61 in terms of this parameter
[TABLE]
will be typically exponentially small with respect to the system-size . The probability distribution of over the samples is expected to be log-normal as a consequence of the product-structure discussed after Eq. 111.
VI Conclusions
In this paper, we have considered the Lindblad dynamics of the XX quantum chain with large random fields , while the couplings can be either uniform or random, for boundary-magnetization-drivings acting on the two end-spins. We have first analyzed the relaxation properties in the presence of a single reservoir as a function of the system size via some boundary-strong-disorder renormalization approach. We have then studied the non-equilibrium-steady-state in the presence of two reservoirs via the effective renormalized Linbladians associated to the two reservoirs. The magnetization has been found to follow a step profile, as found previously in other localized chains [15]. The strong disorder approach has been used to compute explicitly the location of the step of the magnetization profile and the corresponding exponentially-small magnetization-current for each disordered sample in terms of the random fields and couplings.
The companion paper [52] describes how the addition of bulk-dephasing in the dissipative part of the Linbladian destroys these localization properties.
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