Thermoelectric power factor enhancement by spin-polarized currents - a nanowire case study

TL;DR

This study investigates how spin-polarized currents in Co-Ni alloy and multilayered nanowires can enhance thermoelectric power factors, showing significant improvements under magnetic fields, with potential for adjustable thermoelectric applications.

Contribution

It provides the first systematic analysis of thermoelectric power factor enhancement via magnetic fields in Co-Ni nanowires and multilayers, demonstrating notable increases in TE performance.

Findings

TE power factors up to 3.6 mWK-2m-1 measured at room temperature.

TE power factor increases by up to 13.1% in AMR nanowires under magnetic field.

TE power factor increases by up to 52% in GMR nanowires with magnetic field.

Abstract

Thermoelectric (TE) measurements have been performed on the workhorses of today's data storage devices, exhibiting either the giant or the anisotropic magnetoresistance effect (GMR and AMR). The temperature-dependent (50-300 K) and magnetic field-dependent (up to 1 T) TE power factor (PF) has been determined for several Co-Ni alloy nanowires with varying Co:Ni ratios as well as for Co-Ni/Cu multilayered nanowires with various Cu layer thicknesses, which were all synthesized via a template-assisted electrodeposition process. A systematic investigation of the resistivity, as well as the Seebeck coefficient, is performed for Co-Ni alloy nanowires and Co-Ni/Cu multilayered nanowires. At room temperature, measured values of TE PFs up to 3.6 mWK-2m-1 for AMR samples and 2.0 mWK-2m-1 for GMR nanowires are obtained. Furthermore, the TE PF is found to increase by up to 13.1 % for AMR Co-Ni alloy nanowires and by up to 52 % for GMR Co-Ni/Cu samples in an external applied magnetic field. The magnetic nanowires exhibit TE PFs that are of the same order of magnitude as TE PFs of Bi-Sb-Se-Te based thermoelectric materials and, additionally, give the opportunity to adjust the TE power output to changing loads and hotspots through external magnetic fields.