Robust spin correlations at high magnetic fields in the honeycomb iridates

TL;DR

This study uses extremely high magnetic fields to uncover persistent, strongly correlated spin states in honeycomb iridates, revealing complex magnetic behavior beyond simple antiferromagnetic order.

Contribution

It demonstrates that high magnetic fields can melt long-range magnetic order and reveal a bistable, strongly correlated spin state with minimal net magnetization.

Findings

Long-range order is suppressed at high fields.

A bistable, strongly correlated spin state persists.

No long-range order observed up to 90 T.

Abstract

The complexity of the antiferromagnetic orders observed in the honeycomb iridates is a double-edged sword in the search for a quantum spin-liquid ground state: both attesting that the magnetic interactions provide many of the necessary ingredients, but simultaneously impeding access. As a result, focus has been drawn to the unusual magnetic orders and the hints they provide to the underlying spin correlations. However, the study of any particular broken symmetry state generally provides little clue as to the possibilities of other nearby ground states \cite{Anderson}. Here we use extreme magnetic fields to reveal the extent of the spin correlations in $\gamma$-lithium iridate. We find that a magnetic field with a small component along the magnetic easy-axis melts long-range order, revealing a bistable, strongly correlated spin state. Far from the usual destruction of antiferromagnetism via spin polarization, the correlated spin state possesses only a small fraction of the total moment, without evidence for long-range order up to the highest attainable magnetic fields (>90 T).