Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities

TL;DR

This paper demonstrates significant enhancement of ultraviolet second-harmonic radiation at nonlinear interfaces with large disparities in second-order susceptibilities, achieved through experimental setup involving phase matching and total internal reflection.

Contribution

It introduces a novel method for enhancing UV second-harmonic generation using nonlinear interfaces with discontinuous  susceptibilities, showing up to 11.6-fold intensity increase.

Findings

Enhanced UV second-harmonic wave up to 11.6 times at the nonlinear interface.

Experimental validation of phase-matching and total internal reflection effects.

Potential for tunable UV and vacuum-UV spectral applications.

Abstract

We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparency crystal with larger second-order nonlinear coefficient \chi^{(2)}, an nonlinear interface with large disparity in \chi^{(2)} is formed and the enhancement of UV second-harmonic radiation is observed experimentally. The intensity of enhanced second harmonic wave generated at the nonlinear interface was up to 11.6 times at the crystal boundary. As a tunable phase-matching method, it may suggest potential applications in the UV, even vacuum-UV, spectral region.