Demonstrating an absolute quantum advantage in direct absorption measurement

TL;DR

This paper experimentally demonstrates a quantum advantage in optical direct absorption measurement, surpassing classical limits per photon probe, with potential for significant reductions in photon usage.

Contribution

The study provides the first experimental proof of absolute quantum advantage in direct absorption measurement using correlated photon pairs and a novel data analysis method.

Findings

Achieved up to 1.46 times improvement over classical limits.

Demonstrated reduction of approximately 32% in photon number for absorption measurements.

Validated quantum advantage with practical, commercially available components.

Abstract

Engineering apparatus that harness quantum theory offers practical advantages over current technology. A fundamentally more powerful prospect is the long-standing prediction that such quantum technologies could out-perform any future iteration of their classical counterparts, no matter how well the attributes of those classical strategies can be improved. Here, we experimentally demonstrate such an instance of \textit{absolute} advantage per photon probe in the precision of optical direct absorption measurement. We use correlated intensity measurements of spontaneous parametric downconversion using a commercially available air-cooled CCD, a new estimator for data analysis and a high heralding efficiency photon-pair source. We show this enables improvement in the precision of measurement, per photon probe, beyond what is achievable with an ideal coherent state (a perfect laser) detected with $100\%$ efficient and noiseless detection. We see this absolute improvement for up to $50\%$ absorption, with a maximum observed factor of improvement of 1.46. This equates to around $32\%$ reduction in the total number of photons traversing an optical sample, compared to any future direct optical absorption measurement using classical light.