High-pressure study of the ground- and superconducting-state properties of CeAu$_2$Si$_2$

TL;DR

This study investigates the complex relationship between magnetism, quantum criticality, and superconductivity in CeAu$_2$Si$_2$ under high pressure, revealing new magnetic transition lines and quantum critical behavior linked to superconductivity.

Contribution

It presents the first high-pressure measurements showing a magnetic structure rearrangement and quantum critical behavior inside the magnetic phase of CeAu$_2$Si$_2$, highlighting the role of valence fluctuations.

Findings

Discovery of a new magnetic transition line at $T_{ ext{M}}^{ ext{mod}}$

Observation of non-Fermi-liquid behavior near superconductivity

Correlation between magnetic rearrangement and superconducting onset

Abstract

The pressure-temperature-phase diagram of the new heavy-fermion superconductor CeAu$_2$Si$_2$ is markedly different from those studied previously. Indeed, superconductivity emerges, not on the verge, but deep inside the magnetic phase. In this context, we have carried out ac-calorimetry, resistivity and thermoelectric power measurements on a CeAu$_2$Si$_2$-single crystal under high-pressure. The principal novelties of this experiment are the observation of a new transition line, presumably a magnetic structure rearrangement at $T_{\mathrm{M}}^{\mathrm{mod}}$ inside the antiferromagnetic phase, and the occurrence of quantum critical behavior in resistivity linked to superconductivity. Strong non-Fermi-liquid behavior is observed around the maximum of superconductivity and enhanced scattering rates are observed close to both the emergence and the maximum of superconductivity. Intriguingly, $T_{\mathrm{M}}^{\mathrm{mod}}$ almost coincides with the onset of the superconducting transition over a broad pressure range, where mysteriously Tc increases with the strengthening of magnetism. A comparison of the features in CeAu$_2$Si$_2$ and its parent compounds CeCu$_2$Si$_2$ and CeCu$_2$Ge$_2$ plotted as function of the unit-cell volume leads us to promote that critical fluctuations of a valence crossover play a crucial role in the superconducting paring mechanism. Our study reveals new intriguing features of magnetism and illustrates a complex interplay between magnetism, quantum criticality and superconductivity.