SSPALS: a tool for studying positronium
Adam Deller

TL;DR
SSPALS is a valuable technique for positronium research, and this paper analyzes its methods and limitations through simulations, especially in laser spectroscopy applications like REMPI and Rydberg Ps production.
Contribution
The paper introduces a detailed analysis of SSPALS methods and explores their effectiveness and constraints in laser spectroscopy experiments using Monte-Carlo simulations.
Findings
Identifies advantages of SSPALS in positronium studies
Highlights limitations of current analysis methods
Provides insights for optimizing laser spectroscopy experiments
Abstract
Single-shot positron annihilation lifetime spectroscopy (SSPALS) is an extremely useful tool for experiments involving the positronium atom (Ps). I examine some of the methods that are typically employed to analyze lifetime spectra, and use a Monte-Carlo simulation to explore the advantages and limitations these have in laser spectroscopy experiments, such as resonance-enhanced multiphoton ionization (REMPI) or the production of Rydberg Ps.
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