Negative permittivity attests to local attractive interactions in bubble and stripe phases

TL;DR

This paper reports the direct observation of negative permittivity indicating local attractive interactions among electrons in bubble and stripe phases, using surface acoustic waves, revealing new insights into charge ordering in condensed matter.

Contribution

It provides the first unambiguous experimental evidence of attractive electron interactions in bubble and stripe phases through negative permittivity measurements.

Findings

Negative permittivity observed in bubble and stripe phases

Stripe phase confirmed as a strongly anisotropic medium

Evidence of local attractive interactions among electrons

Abstract

The physics of itinerant electrons in condensed matter is by and large governed by repulsive Coulomb forces. However, rare cases exist where local attractive interactions emerge and prevail in determining the ground state of the system despite the dominant Coulomb repulsion. The most notable example is no doubt electron pairing, which leads to superconductivity and is mediated by electron phonon coupling or more intricate mechanisms such as antiferromagnetic spin order in high-temperature superconductors. The interplay of attractive and repulsive interaction components may also instigate spontaneous symmetry lowering and clustering of charges in geometric patterns such as bubbles and stripes, provided these interactions act on different length scales. In high-temperature superconductors, for instance, fluctuating stripe or nematic ordering is intertwined with superconductivity itself. Both types of attractive interaction based physics, pairing and charge ordering, are also at play in high-quality two-dimensional electron systems exposed to a quantizing perpendicular magnetic field for electrons describing larger orbits. This has been concluded indirectly from the transport behaviour when such phases form. An unambiguous manifestation of an underlying attractive interaction between the electrons has however remained elusive. Here we report the observation of a negative permittivity as an immediate consequence of local attractive interaction rather than repulsion among the electrons when bubble and stripe phases form. The implemented technique based on surface acoustic waves offers directionality and confirms the stripe phase to be a strongly anisotropic medium.