Advanced broad-band solid-state supermirror polarizers for cold neutrons

TL;DR

This paper introduces a novel approach to enhance solid-state supermirror neutron polarizers by using high optical potential substrates like sapphire, significantly extending their effective bandwidth and improving polarization efficiency.

Contribution

The study proposes replacing traditional substrates with high optical potential materials to overcome bandwidth limitations in neutron polarizers, validated through experimental measurements.

Findings

Extended the low-Q bandwidth of neutron polarizers

Achieved near-perfect polarization with sapphire substrates

Validated results with experimental measurements at ILL

Abstract

An ideal solid-state supermirror (SM) neutron polarizer assumes total reflection of neutrons from the SM coating for one spin-component and total absorption for the other, thus providing a perfectly polarized neutron beam at the exit. However, in practice, the substrate's neutron-nucleai optical potential does not match perfectly that for spin-down neutrons in the SM. For a positive step in the optical potential (as in a Fe/SiN(x) SM on Si substrate), this mismatch results in spin-independent total reflection for neutrons with small momentum transfer Q, limiting the useful neutron bandwidth in the low-Q region. To overcome this limitation, we propose to replace Si single-crystal substrates by media with higher optical potential than that for spin-down neutrons in the SM ferromagnetic layers. We found single-crystal sapphire and single-crystal quartz as good candidates for solid-state Fe/SiN(x) SM polarizers. To verify this idea, we coated a thick plate of single-crystal sapphire with a m=2.4 Fe/SiN(x) SM. At the T3 instrument at the ILL, we measured the spin-up and spin-down reflectivity curves with 7.5 A neutrons incident from the substrate to the interface between the substrate and the SM coating. The results of this experimental test were in excellent agreement with our expectations: the bandwidth of high polarizing power extended significantly into the low-Q region. This finding, together with the possibility to apply a strong magnetizing field, opens a new road to produce high-efficient solid-state SM polarizers with an extended neutron wavelength bandwidth and near-to-perfect polarizing power.