Stochastic methods for light propagation and recurrent scattering in saturated and nonsaturated atomic ensembles

TL;DR

This paper develops a comprehensive theoretical framework for modeling light propagation in dense atomic ensembles, incorporating quantum effects, and demonstrates its application through simulations of collective atomic states in optical lattices.

Contribution

It introduces a formalism that includes arbitrary atomic level structures and extends classical stochastic electrodynamics to account for quantum fluctuations and saturation effects.

Findings

Recurrent scattering induces strong interatomic correlations.

Collective states exhibit subradiance and superradiance.

Response depends on atomic spatial confinement.

Abstract

We derive equations for the strongly coupled system of light and dense atomic ensembles. The formalism includes an arbitrary internal level structure for the atoms and is not restricted to weak excitation of atoms by light. In the low light intensity limit for atoms with a single electronic ground state, the full quantum field-theoretical representation of the model can be solved exactly by means of classical stochastic electrodynamics simulations for stationary atoms that represent cold atomic ensembles. Simulations for the optical response of atoms in a quantum degenerate regime require one to synthesize a stochastic ensemble of atomic positions that generates the corresponding quantum statistical position correlations between the atoms. In the case of multiple ground levels or at light intensities where saturation becomes important, the classical simulations require approximations that neglect quantum fluctuations between the levels. We show how the model is extended to incorporate corrections due to quantum fluctuations that result from virtual scattering processes. In the low light intensity limit we illustrate the simulations in a system of atoms in a Mott-insulator state in a 2D optical lattice, where recurrent scattering of light induces strong interatomic correlations. These correlations result in collective many-atom subradiant and superradiant states and a strong dependence of the response on the spatial confinement within the lattice sites.