Observation of spin Seebeck contribution to the transverse thermopower in Ni-Pt and MnBi-Au bulk nanocomposites

TL;DR

This study demonstrates that the spin Seebeck effect can be observed in bulk nanocomposites, significantly enhancing transverse thermopower and power output, which could lead to more efficient thermoelectric devices.

Contribution

It provides the first experimental evidence of SSE in bulk nanocomposites combining ferromagnets with spin-orbit nanoparticles, surpassing previous thin-film limitations.

Findings

SSE contributes to transverse thermopower in bulk composites.

Power output more than doubles in Ni-Pt nanocomposites.

SSE persists in bulk nanostructured materials.

Abstract

Transverse thermoelectric devices produce electric fields perpendicular to an incident heat flux. Classically, this process is driven by the Nernst effect in bulk solids, wherein a magnetic field generates a Lorentz force on thermally excited electrons. The spin Seebeck effect (SSE) also produces magnetization-dependent transverse electric fields. SSE is traditionally observed in thin metallic films deposited on electrically insulating ferromagnets, but the films' high resistance limits thermoelectric conversion efficiency. Combining Nernst and SSE in bulk materials would enable devices with simultaneously large transverse thermopower and low electrical resistance. Here we demonstrate experimentally this is possible in composites of conducting ferromagnets (Ni or MnBi) containing metallic nanoparticles with strong spin-orbit interactions (Pt or Au). These materials display positive shifts in transverse thermopower attributable to inverse spin Hall electric fields in the nanoparticles. This more than doubles the power output of the Ni-Pt materials, establishing proof-of-principle that SSE persists in bulk nanocomposites.