Plasmonics of opalic surface: a combined near-and far-field approach

TL;DR

This paper investigates the optical properties of an opalic plasmonic surface made of metallized silica spheres, demonstrating its potential for exciting localized and propagating surface plasmons through combined near- and far-field techniques.

Contribution

It introduces a hybrid 2D plasmonic system and explores its excitation mechanisms using both spectrometry and electron microscopy, highlighting its versatility for nanophotonics.

Findings

Demonstrates excitation of both localized and propagating plasmons

Shows the effectiveness of combined spectrometry and microscopy techniques

Highlights the potential of hybrid opalic surfaces in nanophotonics

Abstract

An opalic plasmonic sample, constituted by a hexagonal arrangement of metallized silica spheres, presents remarkable optical properties due to the mixing of periodic arrangement and singularities at the sphere touching points. It is therefore an interesting candidate for exploiting the excitation of both localized and propagating surface plasmons. Several channels of excitation based on these properties or exploiting a certain level of disorder are evidenced, opening new routes for the efficient excitation of plasmons on a wide spectral range. The versatility of such hybrid system is evidenced in the context of two complementary experiments: specular reflective spectrometry and photoemission electron microscopy. Both techniques offer different points of view on the same physical phenomenon and the link between them is discussed. Such experiments evidence the opportunities offered by these 2D hybrid materials in the context of nanophotonics.