Magneto-optical absorption in semiconducting spherical quantum dots: Influence of the dot-size, confining potential, and magnetic field

TL;DR

This paper provides a comprehensive theoretical analysis of magneto-optical absorption in spherical quantum dots, highlighting how magnetic field and confinement influence spectral properties and electronic behavior.

Contribution

It introduces a detailed theoretical framework using Bohm-Pines' RPA to analyze Coulomb interactions and predicts how magnetic field and dot size affect absorption spectra and electronic states.

Findings

Magnetic field and confinement similarly shift absorption spectra.

Fermi energy decreases with increasing magnetic field and dot size.

Both magneto-optical transitions persist even at extreme conditions.

Abstract

Here we embark on a thorough investigation of the magneto-optical absorption in semiconducting {\em spherical} quantum dots characterized by a confining harmonic potential and an applied magnetic field in the symmetric gauge. This is done within the framework of Bohm-Pines' random-phase approximation that enables us to derive and discuss the full Dyson equation that takes proper account of the Coulomb interactions. As an application of our theoretical strategy, we compute various single-particle and many-particle phenomena such as the Fock-Darwin spectrum; Fermi energy; magneto-optical transitions; probability distribution; and the magneto-optical absorption in the quantum dots. It is observed that the role of an applied magnetic field on the absorption spectrum is comparable to that of a confining potential. Increasing (decreasing) the strength of the magnetic field or the confining potential is found to be analogous to shrinking (expanding) the size of the quantum dots: resulting into a blue (red) shift in the absorption spectrum. The Fermi energy diminishes with both increasing magnetic-field and dot-size; and exhibits saw-tooth-like oscillations at large values of field or dot-size. Unlike laterally confined quantum dots, both (upper and lower) magneto-optical transitions survive even in the extreme instances. However, the intra-Landau level transitions are seen to be forbidden. The spherical quantum dots have an edge over the strictly two-dimensional quantum dots in that the additional (magnetic) quantum number makes the physics richer (but complex). A deeper grasp of the Coulomb blockade, quantum coherence, and entanglement can lead to a better insight into promising applications involving lasers, detectors, storage devices, and quantum computing.