Estimation of the lifetime of small helium bubbles near tungsten surfaces -- a methodological study

TL;DR

This study develops a molecular dynamics method to estimate the lifetime of helium bubbles near tungsten surfaces, revealing their stochastic bursting behavior and dependencies on depth and size, aiding fusion reactor surface modeling.

Contribution

A novel molecular dynamics approach to quantify helium bubble lifetimes near tungsten surfaces, linking bursting behavior to activation energy and depth for the first time.

Findings

He bubble bursting follows the Arrhenius equation.

Activation energy depends linearly on bubble depth.

Pre-exponential factor follows Meyer-Nedle rule.

Abstract

Under low energy and high flux/fluence irradiation of helium (He) atoms, the formation and bursting of He bubbles on tungsten (W) surfaces play important roles in the morphological evolution of component surfaces and impurity production in fusion reactors. Microscopically, the bursting of He bubbles is a stochastic process, and He bubbles have statistically average lifetimes. In the present paper, a molecular dynamics-based method was developed to extract, for the first time, the lifetime of He bubbles near tungsten surfaces. It was found that He bubble bursting can be treated as an activated event. Its occurrence frequency or, equivalently, the average lifetime of bubbles follows the Arrhenius equation. For a given bubble size, the activation energy exhibits a good linear dependence with the depth, and the pre-exponential factor obeys the Meyer-Nedle rule. These results are useful for establishing a model in multi-scale simulations of impurity production in the fusion plasma and of the morphological evolution of component surfaces.