Quantum many-body simulation using monolayer exciton-polaritons in coupled-cavities

TL;DR

This paper proposes enhancing interparticle interactions in photon-based quantum simulators using exciton-polaritons in MoS₂ monolayer quantum dots within 2D photonic crystal microcavities, enabling more effective simulation of strongly correlated many-body systems.

Contribution

It introduces a method to significantly increase exciton-polariton interactions in coupled-cavity systems, surpassing previous limits, and demonstrates potential for advanced quantum simulations.

Findings

Optimal repulsive interaction of 1-10 meV achieved

Strong interactions occur in the crossover regime, not in blockade regimes

MoS₂ monolayer quantum dots outperform conventional materials

Abstract

Quantum simulation is a promising approach to understand complex strongly correlated many-body systems using relatively simple and tractable systems. Photon-based quantum simulators have great advantages due to the possibility of direct measurements of multi-particle correlations and ease of simulating non-equilibrium physics. However, interparticle interaction in existing photonic systems is often too weak limiting the potential of quantum simulation. Here we propose an approach to enhance the interparticle interaction using exciton-polaritons in MoS$_2$ monolayer quantum-dots embedded in 2D photonic crystal microcavities. Realistic calculation yields optimal repulsive interaction in the range of $1$-$10$~meV --- more than an order of magnitude greater than the state-of-art value. Such strong repulsive interaction is found to emerge neither in the photon-blockade regime for small quantum dot nor in the polariton-blockade regime for large quantum dot, but in the crossover between the two regimes with a moderate quantum-dot radius around 20~nm. The optimal repulsive interaction is found to be largest in MoS$_2$ among commonly used optoelectronic materials. Quantum simulation of strongly correlated many-body systems in a finite chain of coupled cavities and its experimental signature are studied via exact diagonalization of the many-body Hamiltonian. A method to simulate 1D superlattices for interacting exciton-polariton gases in serially coupled cavities is also proposed. Realistic considerations on experimental realizations reveal advantages of transition metal dichalcogenide monolayer quantum-dots over conventional semiconductor quantum-emitters.