Two types of all-optical magnetization switching mechanisms using femtosecond laser pulses

TL;DR

This paper identifies and distinguishes two all-optical magnetization switching mechanisms in magnetic materials using femtosecond laser pulses, supported by experimental analysis of their microscopic origins and timescales.

Contribution

It introduces a clear distinction between single pulse and cumulative switching mechanisms and explores their microscopic origins in different magnetic materials.

Findings

Two distinct switching mechanisms identified: single pulse and cumulative.

Cumulative switching involves heat-driven demagnetization followed by helicity-dependent remagnetization.

All-electrical, time-resolved measurements reveal different microscopic processes.

Abstract

Magnetization manipulation in the absence of an external magnetic field is a topic of great interest, since many novel physical phenomena need to be understood and promising new applications can be imagined. Cutting-edge experiments have shown the capability to switch the magnetization of magnetic thin films using ultrashort polarized laser pulses. In 2007, it was first observed that the magnetization switching for GdFeCo alloy thin films was helicity-dependent and later helicity-independent switching was also demonstrated on the same material. Recently, all-optical switching has also been discovered for a much larger variety of magnetic materials (ferrimagnetic, ferromagnetic films and granular nanostructures), where the theoretical models explaining the switching in GdFeCo films do not appear to apply, thus questioning the uniqueness of the microscopic origin of all-optical switching. Here, we show that two different all-optical switching mechanisms can be distinguished; a "single pulse" switching and a "cumulative" switching process whose rich microscopic origin is discussed. We demonstrate that the latter is a two-step mechanism; a heat-driven demagnetization followed by a helicity-dependent remagnetization. This is achieved by an all-electrical and time-dependent investigation of the all-optical switching in ferrimagnetic and ferromagnetic Hall crosses via the anomalous Hall effect, enabling to probe the all-optical switching on different timescales.