Ultra-confined acoustic THz graphene plasmons revealed by photocurrent nanoscopy

TL;DR

This paper demonstrates real-space imaging of ultra-confined terahertz graphene plasmons using nanoscale photocurrent microscopy, revealing their linear dispersion and strong confinement, which could advance subwavelength THz device technology.

Contribution

It introduces a novel nanoscale-resolved THz photocurrent near-field microscopy technique for imaging strongly confined graphene plasmons in real space.

Findings

Achieved imaging of THz graphene plasmons with wavelengths reduced by a factor of 66.

Observed linear dispersion of acoustic THz plasmons due to coupling with the metal gate.

Identified Coulomb impurity scattering as the main damping mechanism at positive carrier densities.

Abstract

Terahertz (THz) fields are widely applied for sensing, communication and quality control. In future applications, they could be efficiently confined, enhanced and manipulated - well below the classical diffraction limit - through the excitation of graphene plasmons (GPs). These possibilities emerge from the strongly reduced GP wavelength, lp, compared to the photon wavelength, l0, which can be controlled by modulating the carrier density of graphene via electrical gating. Recently, GPs in a graphene-insulator-metal configuration have been predicted to exhibit a linear dispersion (thus called acoustic plasmons) and a further reduced wavelength, implying an improved field confinement, analogous to plasmons in two-dimensional electron gases (2DEGs) near conductive substrates. While infrared GPs have been visualised by scattering-type scanning near-field optical microscopy (s-SNOM), the real-space imaging of strongly confined THz plasmons in graphene and 2DEGs has been elusive so far - only GPs with nearly free-space wavelength have been observed. Here we demonstrate real-space imaging of acoustic THz plasmons in a graphene photodetector with split-gate architecture. To that end, we introduce nanoscale-resolved THz photocurrent near-field microscopy, where near-field excited GPs are detected thermoelectrically rather than optically. The on-chip GP detection simplifies GP imaging, as sophisticated s-SNOM detection schemes can be avoided. The photocurrent images reveal strongly reduced GP wavelengths (lp = l0/66), a linear dispersion resulting from the coupling of GPs with the metal gate below the graphene, and that plasmon damping at positive carrier densities is dominated by Coulomb impurity scattering. Acoustic GPs could thus strongly benefit the development of deep subwavelength-scale THz devices.