Detecting the orbital character of the spin fluctuation in the Iron-based superconductors with the resonant inelastic X-ray scattering spectroscopy

TL;DR

This paper proposes using resonant inelastic X-ray scattering (RIXS) to selectively probe the orbital distribution of spin fluctuations in iron-based superconductors, providing insights into their orbital physics and pairing mechanisms.

Contribution

It introduces a method to distinguish spin fluctuations on different Fe 3d orbitals using RIXS in specific scattering geometries, advancing orbital-resolved studies.

Findings

RIXS can selectively probe spin fluctuations on different Fe 3d orbitals.

The method enables orbital-resolved analysis of spin nematicity.

This approach enhances understanding of orbital physics in superconductivity.

Abstract

The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we propose that the resonant inelastic X-ray scattering(RIXS) technique can be used to probe selectively the spin fluctuation on different Fe $3d$ orbitals. In particular, the spin fluctuation on the three $t_{2g}$ orbitals, namely, the $3d_{xz}$, $3d_{yz}$ and the $3d_{xy}$ orbital, can be selectively probed in the $\sigma\rightarrow\pi'$ scattering geometry by aligning the direction of the outgoing photon in the $y$, $x$ and $z$ direction. Such orbital-resolved information on the spin fluctuation is invaluable for the study of the orbital-selective physics in the IBSs and can greatly advance our understanding on the relation between orbital ordering and spin nematicity in the IBSs and the orbital-selective pairing mechanism in these multi-orbital systems.