A tunable CW UV laser with <35 kHz absolute frequency instability for precision spectroscopy of Sr Rydberg states

TL;DR

This paper introduces a solid-state, tunable CW UV laser with sub-35 kHz frequency stability, enabling high-precision spectroscopy of strontium Rydberg states with mode-hop-free scans and Doppler-limited linewidths.

Contribution

The work presents a novel, stable, and tunable UV laser system based on fiber amplifiers and nonlinear optics, suitable for precision atomic spectroscopy.

Findings

Achieved <35 kHz long-term frequency instability.

Demonstrated mode-hop-free scans of 24 GHz.

Measured Doppler-limited linewidths of 350 kHz.

Abstract

We present a solid-state laser system that generates over 200 mW of continuous-wave, narrowband light, tunable from 316.3 nm - 317.7 nm and 318.0 nm - 319.3 nm. The laser is based on commercially available fiber amplifiers and optical frequency doubling technology, along with sum frequency generation in a periodically poled stoichiometric lithium tantalate crystal. The laser frequency is stabilized to an atomic-referenced high finesse optical transfer cavity. Using a GPS-referenced optical frequency comb we measure a long term frequency instability of $<$35 kHz for timescales between $10^{-3}$ s and $10^3$ s. As an application we perform spectroscopy of Sr Rydberg states from $n$ = 37 - 81, demonstrating mode-hop-free scans of 24 GHz. In a cold atomic sample we measure Doppler-limited linewidths of 350 kHz.