Strong Cavity-Pseudospin Coupling in Monolayer Transition Metal Dichalcogenides: Spontaneous Spin-Oscillations and Magnetometry

TL;DR

This paper explores the strong coupling between monolayer TMDCs and photonic cavities, revealing effects like spontaneous spin-oscillations and potential for sensitive magnetometry, advancing quantum photonics and spintronics.

Contribution

It demonstrates the realization of strong cavity-pseudospin coupling in monolayer TMDCs and uncovers novel spin-oscillation and magnetometry phenomena.

Findings

Observation of strong cavity-pseudospin coupling in TMDC monolayers.

Identification of spontaneous spin-oscillations induced by cavity coupling.

TMDC monolayers as sensitive magnetic field sensors.

Abstract

Strong coupling between the electronic states of monolayer transition metal dichalcogenides (TMDC) such as MoS$_2$, MoSe$_2$, WS$_2$, or WSe$_2$, and a two-dimensional (2D) photonic cavity gives rise to several exotic effects. The Dirac type Hamiltonian for a 2D gapped semiconductor with large spin-orbit coupling facilitates pure Jaynes-Cummings type coupling in the presence of a single mode electric field. The presence of an additional circularly polarized beam of light gives rise to valley and spin dependent cavity-QED properties. The cavity causes the TMDC monolayer to act as an on-chip coherent light source and a spontaneous spin-oscillator. In addition, a TMDC monolayer in a cavity is a sensitive magnetic field sensor for an in-plane magnetic field.