Characterization of Micro-Roughness Parameters and Optical Properties of Obliquely Deposited HfO2 Thin Films

TL;DR

This study investigates how oblique angle deposition affects the microstructure and optical properties of HfO2 thin films, revealing correlations between deposition angle, surface roughness, refractive index, and grain size.

Contribution

It provides a detailed analysis of morphological parameters and optical properties of obliquely deposited HfO2 films, highlighting the influence of deposition angle on microstructure and optical behavior.

Findings

Intrinsic roughness varies with deposition angle.

Refractive index decreases as deposition angle increases.

Grain size shows an opposite trend to refractive index.

Abstract

Oblique angle deposited oxide thin films have opened up new dimensions in fabricating optical interference devices with tailored refractive index profile along thickness by tuning its microstructure by varying angle of deposition. Microstructure of thin films strongly affects surface morphology as well as optical properties. Since surface morphology plays an important role for the qualification of thin film devices for optical or other applications, it is important to investigate morphological properties. In present work, HfO2 thin films have been deposited at several oblique angles. Morphological statistical parameters of such thin films viz., correlation length, intrinsic roughness, fractal spectral strength, etc., have been determined through suitable modelling of extended power spectral density function. Intrinsic roughness and fractal spectral strength show an interesting behaviour with deposition angle and the same has been discussed in the light of atomic shadowing, re-emission and diffusion of ad-atoms. Further refractive index and thickness of such thin films have been estimated from transmission spectra. Refractive index and grain size depict an opposite trend with deposition angle and their variation has been explained by varying column slanting angle and film porosity with deposition angle.