Random Nonlinear Infinite-Level-System Model for Amorphous Solid Phonon Echo and Saturation Phenomena
Di Zhou, Anthony J. Leggett

TL;DR
This paper generalizes the tunneling-two-level-system model to an infinite-level-system with randomness and nonlinearity, demonstrating phonon echo as stimulated emission and explaining saturation phenomena in amorphous solids.
Contribution
It introduces a novel infinite-level-system model with randomness and nonlinearity, providing theoretical proofs for phonon echo as stimulated emission and the conditions for saturation.
Findings
Phonon echo is a stimulated emission process.
Quantum nonlinearity enables saturation phenomena.
Randomness and nonlinearity are essential for echo and saturation.
Abstract
The first two successful predictions for amorphous solid experiments by tunneling-two-level-system (TTLS) was phonon echo and saturation phenomena. In this paper by generalizing TTLS to infinite-level-system model with certain randomness and nonlinearity, we prove that phonon echo is a stimulated emission process. The classical infinite-level-system (taking limit) cannot find saturation effect, while quantum infinite-level-system can find it with certain nonlinearity assumed. We also prove that without randomness or nonlinearity neither phonon echo nor saturation exists in arbitrary infinite-level-system.
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Taxonomy
TopicsSpectroscopy and Quantum Chemical Studies · Quantum and electron transport phenomena · Random lasers and scattering media
