Polarization-dependent photocurrents in polar stacks of van der Waals solids

TL;DR

This paper investigates how polarization-dependent photocurrents in polar van der Waals monolayers are generated and controlled by light polarization, revealing mechanisms like asymmetric photogeneration, scattering, and Berry curvature effects.

Contribution

It introduces the concept of polarization-dependent photocurrents in polar TMD monolayers, analyzing their origins and control via light polarization and magnetic effects.

Findings

In-plane photocurrents depend on light polarization and helicity.

Ballistic and side-jump contributions influence non-helical currents.

Magneto-induced photocurrents relate to Lorentz force and Berry curvature.

Abstract

Monolayers of semiconducting van der Waals solids, such as transition metal dichalcogenides (TMDs), acquire significant electric polarization normal to the layers when placed on a substrate or in a heterogeneous stack. This causes linear coupling of electrons to electric fields normal to the layers. Irradiation at oblique incidence at frequencies above the gap causes interband transitions due to coupling to both normal and in-plane ac electric fields. The interference between the two processes leads to sizable in-plane photocurrents and valley currents. The direction and magnitude of currents is controlled by light polarization and is determined by its helical or non-helical components. The helicity-dependent ballistic current arises due to asymmetric photogeneration. The non-helical current has a ballistic contribution (dominant in sufficiently clean samples) caused by asymmetric scattering of photoexcited carriers, and a side-jump contribution. Magneto-induced photocurrent is due to the Lorentz force or due to intrinsic magnetic moment related to Berry curvature.