Dephasing effects on coherent exciton-polaritons and the breaking of the strong coupling regime

TL;DR

This study investigates how excitation-induced dephasing disrupts strong exciton-photon coupling in semiconductor microcavities, revealing density-dependent spectral broadening, resonance shifts, and the underlying many-body effects.

Contribution

It identifies excitation-induced dephasing as a key mechanism breaking strong coupling and quantifies many-body effects using excitonic Bloch equations.

Findings

Density-dependent broadening of polariton resonances

Emergence of a third resonance at high excitation density

Asymmetry in energy shifts between upper and lower polaritons

Abstract

Using femtosecond pump-probe spectroscopy, we identify excitation induced dephasing as a major mechanism responsible for the breaking of the strong-coupling between excitons and photons in a semiconductor microcavity. The effects of dephasing are observed on the transmitted probe pulse spectrum as a density dependent broadening of the exciton-polariton resonances and the emergence of a third resonance at high excitation density. A striking asymmetry in the energy shift between the upper and the lower polaritons is also evidenced. Using the excitonic Bloch equations, we quantify the respective contributions to the energy shift of many-body effects associated with Fermion exchange and photon assisted exchange processes and the contribution to collisional broadening.