Strain accommodation through facet matching in La$_\text{1.85}$Sr$_\text{0.15}$CuO$_\text{4}$/Nd$_\text{1.85}$Ce$_\text{0.15}$CuO$_\text{4}$ ramp-edge junctions

TL;DR

This study investigates how strain is accommodated at the interface of superconducting cuprate junctions using advanced microscopy and diffraction techniques, revealing a new growth mode with a tilted crystal structure explained by a facet matching strain model.

Contribution

It introduces a strain accommodation model based on facet matching to explain the tilt in LaSrCuO films on ramped junctions, advancing understanding of interface structure in complex oxides.

Findings

Discovery of a 3.3° tilt in LaSrCuO at the ramp interface

Development of a facet matching strain accommodation model

Implications for artificial domain creation in morphotropic materials

Abstract

Scanning nano-focused X-ray diffraction (nXRD) and high-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) are used to investigate the crystal structure of ramp-edge junctions between superconducting electron-doped Nd$_\text{1.85}$Ce$_\text{0.15}$CuO$_\text{4}$ and superconducting hole-doped La$_\text{1.85}$Sr$_\text{0.15}$CuO$_\text{4}$ thin films, the latter being the top layer. On the ramp, a new growth mode of La$_\text{1.85}$Sr$_\text{0.15}$CuO$_\text{4}$ with a 3.3 degree tilt of the c-axis is found. We explain the tilt by developing a strain accommodation model that relies on facet matching, dictated by the ramp angle, indicating that a coherent domain boundary is formed at the interface. The possible implications of this growth mode for the creation of artificial domains in morphotropic materials are discussed.