Hard-core boson approach to the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuCl$_4$ at finite temperatures in magnetic fields higher than the saturation field

TL;DR

This paper models the high-field behavior of the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuCl$_4$ using a hard-core boson approach, accurately predicting thermodynamic properties at finite temperatures.

Contribution

It introduces a self-consistent ladder approximation combined with Hartree-Fock decoupling to analyze gapped hard-core bosons in two dimensions at finite temperatures.

Findings

Calculated spectral functions match experimental data.

Accurate predictions of specific heat and magnetic susceptibility.

Validated the approach for gapped hard-core bosons in 2D.

Abstract

We study the high magnetic field regime of the antiferromagnetic insulator Cs$_2$CuCl$_4$ by expressing the spin-1/2 operators in the relevant Heisenberg model in terms of hard-core bosons and implementing the hard-core constraint via an infinite on-site interaction. We focus on the case where the external magnetic field exceeds the saturation field $B_{c}\approx8.5\;\mathrm{T}$ and is oriented along the crystallographic $a$ axis perpendicular to the lattice plane. Because in this case the excited states are separated by an energy gap from the ground state, we may use the self-consistent ladder approximation to take the strong correlations due to the hard-core constraint into account. In Cs$_2$CuCl$_4$ there are additional interactions besides the hard-core interaction which we treat in self-consistent Hartree-Fock approximation. We calculate the spectral function of the hard-core bosons from which we obtain the in-plane components of the dynamic structure factor, the magnetic susceptibility, and the specific heat. Our results for the specific heat are in good agreement with the available experimental data. We conclude that the self-consistent ladder approximation in combination with a self-consistent Hartree-Fock decoupling of the non-hard-core interactions gives an accurate description of the physical properties of gapped hard-core bosons in two dimensions at finite temperatures.