Particle detection through the quantum counter concept in YAG:Er$^{3+}$

TL;DR

This paper introduces a new particle detection method using the infrared quantum counter concept in Er$^{3+}$-doped YAG crystals, demonstrating its feasibility with electron irradiation and optical signal detection.

Contribution

It presents a novel detection scheme based on a two-step excitation process in rare earth-doped crystals, showing experimental validation with electron-induced fluorescence.

Findings

Clear optical signals observed upon electron irradiation

Increased metastable level population detected

Feasibility demonstrated for particle detection

Abstract

We report about a novel scheme for particle detection based on the infrared quantum counter concept. Its operation consists of a two-step excitation process of a four level system, that can be realized in rare earth-doped crystals when a cw pump laser is tuned to the transition from the second to the fourth level. The incident particle raises the atoms of the active material into a low lying, metastable energy state, triggering the absorption of the pump laser to a higher level. Following a rapid non-radiative decay to a fluorescent level, an optical signal is observed with a conventional detectors. In order to demonstrate the feasibility of such a scheme, we have investigated the emission from the fluorescent level $^4$S$_{3/2}$ (540 nm band) in an Er$^{3+}$-doped YAG crystal pumped by a tunable titanium sapphire laser when it is irradiated with 60 keV electrons delivered by an electron gun. We have obtained a clear signature this excitation increases the $^{4}I_{13/2}$ metastable level population that can efficiently be exploited to generate a detectable optical signal.