Strong-field physics with mid-IR fields

TL;DR

This paper introduces an advanced experimental setup combining a high-repetition-rate mid-IR source with a reaction microscope to explore strong-field physics, enabling detailed three-dimensional imaging of electron dynamics across a broad energy spectrum.

Contribution

It presents a novel methodology integrating a 160 kHz mid-IR source with a reaction microscope for comprehensive 3D imaging of strong-field interactions, including electron recollisions and double-ionization.

Findings

Demonstrated detection of electron energies spanning six orders of magnitude.

Investigated low-energy structures in strong-field ionization.

First-time measurement of correlated electron momentum in mid-IR driven double-ionization.

Abstract

Strong-field physics is currently experiencing a shift towards the use of mid-IR driving wavelengths. This is because they permit conducting experiments unambiguously in the quasi-static regime and enable exploiting the effects related to ponderomotive scaling of electron recollisions. Initial measurements taken in the mid-IR immediately led to a deeper understanding of photo-ionization and allowed a discrimination amongst different theoretical models. Ponderomotive scaling of rescattering has enabled new avenues towards time resolved probing of molecular structure. Essential for this paradigm shift was the convergence of two experimental tools: 1) intense mid-IR sources that can create high energy photons and electrons while operating within the quasi-static regime, and 2) detection systems that can detect the generated high energy particles and image the entire momentum space of the interaction in full coincidence. Here we present a unique combination of these two essential ingredients, namely a 160\~kHz mid-IR source and a reaction microscope detection system, to present an experimental methodology that provides an unprecedented three-dimensional view of strong-field interactions. The system is capable of generating and detecting electron energies that span a six order of magnitude dynamic range. We demonstrate the versatility of the system by investigating electron recollisions, the core process that drives strong-field phenomena, at both low (meV) and high (hundreds of eV) energies. The low energy region is used to investigate recently discovered low-energy structures, while the high energy electrons are used to probe atomic structure via laser-induced electron diffraction. Moreover we present, for the first time, the correlated momentum distribution of electrons from non-sequential double-ionization driven by mid-IR pulses.