Quantum theory of light emission from quantum dots coupled to structured photonic reservoirs and acoustic phonons

TL;DR

This paper develops a comprehensive quantum theoretical framework to analyze light emission from quantum dots coupled to structured photonic environments and acoustic phonons, comparing multiple models and applying them to various experimental setups.

Contribution

It introduces a unified quantum theory for emission spectra from quantum dots in structured reservoirs, including analytical solutions and comparisons of different electron-phonon coupling models.

Findings

Semiclassical linear susceptibility approach fails to capture phonon-mediated cavity feeding.

Analytical expressions for phonon-assisted scattering rates in weak excitation regime.

Quantum dot emission spectra are significantly affected by phonon interactions in structured photonic environments.

Abstract

Electron-phonon coupling in semiconductor quantum dots plays a significant role in determining the optical properties of excited excitons, especially the spectral nature of emitted photons. This paper presents a comprehensive theory and analysis of emission spectra from artificial atoms or quantum dots coupled to structured photon reservoirs and acoustic phonons, when excited with incoherent pump fields. As specific examples of structured reservoirs, we chose a Lorentzian cavity and a coupled cavity waveguide, which are of current experimental interest. For the case of optical cavities, we directly compare and contrast the spectra from three distinct theoretical approaches to treat electron-phonon coupling, including a Markovian polaron master equation, a non-Markovian phonon correlation expansion technique and a semiclassical linear susceptibility approach, and we point out the limitations of these models. For the cavity-QED polaron master equation, we give closed form analytical solutions to the phonon-assisted scattering rates in the weak excitation approximation, fully accounting for temperature, cavity-exciton detuning and cavity dot coupling. We show explicitly why the semiclassical linear susceptibility approach fails to correctly account for phonon-mediated cavity feeding. For weakly coupled cavities, we calculate the optical spectra using a more general reservoir approach and explain its differences from the above approaches in the low Q limit of a Lorentzian cavity. We subsequently use this general reservoir to calculate the emission spectra from quantum dots coupled to slow-light photonic crystal waveguides, which demonstrate a number of striking photon-phonon coupling effects. Our quantum theory can be applied to a wide range of photonic structures including photonic molecules and coupled-cavity waveguide systems.