Irreversible transformation of ferromagnetic ordered stripe domains in single-shot IR pump - resonant X-ray scattering probe experiments

TL;DR

This study investigates the ultrafast and irreversible changes in magnetic stripe domains in a CoPd alloy film after femtosecond IR laser excitation, revealing complex domain evolution and stabilization mechanisms.

Contribution

It demonstrates the first observation of irreversible magnetic domain transformations and partial reordering after ultrafast laser-induced demagnetization using time-resolved resonant X-ray scattering.

Findings

Ultrafast demagnetization occurs within hundreds of femtoseconds.

Magnetic domains evolve into a disordered labyrinth structure within nanoseconds.

A partially ordered stripe domain reemerges after about 7 nanoseconds.

Abstract

The evolution of a magnetic domain structure upon excitation by an intense, femtosecond Infra-Red (IR) laser pulse has been investigated using single-shot based time-resolved resonant X-ray scattering at the X-ray Free Electron laser LCLS. A well-ordered stripe domain pattern as present in a thin CoPd alloy film has been used as prototype magnetic domain structure for this study. The fluence of the IR laser pump pulse was sufficient to lead to an almost complete quenching of the magnetization within the ultrafast demagnetization process taking place within the first few hundreds of femtoseconds following the IR laser pump pulse excitation. On longer time scales this excitation gave rise to subsequent irreversible transformations of the magnetic domain structure. Under our specific experimental conditions, it took about 2 nanoseconds before the magnetization started to recover. After about 5 nanoseconds the previously ordered stripe domain structure had evolved into a disordered labyrinth domain structure. Surprisingly, we observe after about 7 nanoseconds the occurrence of a partially ordered stripe domain structure reoriented into a novel direction. It is this domain structure in which the sample's magnetization stabilizes as revealed by scattering patterns recorded long after the initial pump-probe cycle. Using micro-magnetic simulations we can explain this observation based on changes of the magnetic anisotropy going along with heat dissipation in the film.