Heterophase liquid states: Thermodynamics, structure, dynamics
A.S. Bakai
TL;DR
This paper reviews theoretical and experimental insights into heterophase glass-forming liquids, focusing on thermodynamics, structure, and dynamics using the mesoscopic heterophase fluctuations model.
Contribution
It introduces the HPFM framework to analyze heterophase liquids, encompassing phenomena like Fischer clusters, glass transition, and liquid-liquid transformations.
Findings
Fischer cluster phenomenon explained by HPFM
Insights into glass transition mechanisms
Phase diagram characterization of heterophase liquids
Abstract
An overview of theoretical results and experimental data on the thermodynamics, structure and dynamics of the heterophase glass-forming liquids is presented. The theoretical approach is based on the mesoscopic heterophase fluctuations model (HPFM) developed within the framework of the bounded partition function approach. The Fischer cluster phenomenon, glass transition, liquid-liquid transformations, parametric phase diagram, cooperative dynamics and fragility of the glass-forming liquids is considered.
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