Effect of magnetic anisotropy on spin-dependent thermoelectric effects in nanoscopic systems

TL;DR

This paper theoretically investigates how magnetic anisotropy influences spin-dependent thermoelectric effects in nanoscopic systems, revealing significant impacts on conductance and thermopower, especially in systems with magnetic impurities.

Contribution

It provides a detailed theoretical analysis of thermoelectric effects considering magnetic anisotropy and impurity interactions in nanoscopic systems, highlighting the role of inelastic scattering.

Findings

Magnetic anisotropy significantly affects thermoelectric responses.

Inelastic scattering leads to finite spin thermopower without charge flow.

Magnetic impurities induce angular momentum and energy exchange impacting thermoelectric properties.

Abstract

Conventional and spin-related thermoelectric effects in electronic transport through a nanoscopic system exhibiting magnetic anisotropy $-$with both uniaxial and transverse components$-$ are studied theoretically in the linear response regime. In particular, a magnetic tunnel junction with a large-spin impurity $-$either a magnetic atom or a magnetic molecule$-$ embedded in the barrier is considered as an example. Owing to magnetic interaction with the impurity, conduction electrons traversing the junction can scatter on the impurity, which effectively can lead to angular momentum and energy exchange between the electrons and the impurity. As we show, such processes have a profound effect on the thermoelectric response of the system. Specifically, we present a detailed analysis of charge, spin and thermal conductance, together with the Seebeck and spin Seebeck coefficients (thermopowers). Since the scattering mechanism also involves processes when electrons are inelastically scattered back to the same electrode, one can expect the flow of spin and energy also in the absence of charge transport through the junction. This, in turn, results in a finite spin thermopower, and the magnetic anisotropy plays a key role for this effect to occur.