Ultrafast carrier localisation in the pseudogap state of cuprate superconductors from coherent quench experiments

TL;DR

This study uses coherent quench experiments to investigate the ultrafast dynamics of the pseudogap state in cuprate superconductors, revealing rapid carrier localization without long-range order, supporting a Coulomb-strain pairing mechanism.

Contribution

First coherent quench measurements of the pseudogap transition in a high-Tc superconductor, showing rapid localization and challenging the presence of incipient collective order.

Findings

Absence of long-range collective order in the pseudogap state.

Evidence for sub-picosecond carrier localization.

Support for Coulomb interaction and strain-driven pairing mechanism.

Abstract

A pseudogap (PG) was introduced by Mott to describe a state of matter which has a minimum in the density of states at the Fermi level, deep enough for states to become localized. It can arise either from Coulomb repulsion between electrons, or due to an incipient charge or spin order, or a combination of the two. These states are rapidly fluctuating in time with random phase, so they are hard to observe experimentally. Here we present the first coherent quench measurements of the dynamical transition to the pseudogap state in the prototype high temperature superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+\delta}$, revealing a marked absence of incipient collective ordering beyond a few coherence lengths on short timescales at any level of doping. Instead we find evidence for sub-picosecond carrier localization favouring a picture of pairing resulting from the competing Coulomb interaction and strain, enhanced by a Fermi surface instability.