Pairing-induced speedup of nuclear spontaneous fission

TL;DR

This paper investigates how nucleonic pairing correlations influence nuclear spontaneous fission pathways and lifetimes, revealing that pairing can significantly alter fission dynamics and pathway geometry.

Contribution

It introduces a self-consistent four-dimensional model incorporating shape and pairing coordinates to study fission trajectories, highlighting the dynamic role of pairing correlations.

Findings

Pairing correlations are enhanced along the minimum-action fission path.

Pairing fluctuations can restore axial symmetry in fission trajectories.

Nucleonic pairing significantly impacts the shape and dynamics of fission pathways.

Abstract

Collective inertia is strongly influenced at the level crossing at which quantum system changes diabatically its microscopic configuration. Pairing correlations tend to make the large-amplitude nuclear collective motion more adiabatic by reducing the effect of those configuration changes. Competition between pairing and level crossing is thus expected to have a profound impact on spontaneous fission lifetimes. To elucidate the role of nucleonic pairing on spontaneous fission, we study the dynamic fission trajectories of $^{264}$Fm and $^{240}$Pu using the state-of-the-art self-consistent framework. We employ the superfluid nuclear density functional theory with the Skyrme energy density functional SkM$^*$ and a density-dependent pairing interaction. Along with shape variables, proton and neutron pairing correlations are taken as collective coordinates. The collective inertia tensor is calculated within the nonperturbative cranking approximation. The fission paths are obtained by using the least action principle in a four-dimensional collective space of shape and pairing coordinates. Pairing correlations are enhanced along the minimum-action fission path. For the symmetric fission of $^{264}$Fm, where the effect of triaxiality on the fission barrier is large, the geometry of fission pathway in the space of shape degrees of freedom is weakly impacted by pairing. This is not the case for $^{240}$Pu where pairing fluctuations restore the axial symmetry of the dynamic fission trajectory. The minimum-action fission path is strongly impacted by nucleonic pairing. In some cases, the dynamical coupling between shape and pairing degrees of freedom can lead to a dramatic departure from the static picture. Consequently, in the dynamical description of nuclear fission, particle-particle correlations should be considered on the same footing as those associated with shape degrees of freedom.