Charge-Stripe Order in a Parent Compound of Iron-based Superconductors

TL;DR

This study uncovers a long-range charge-stripe order in FeTe, a parent compound of iron-based superconductors, revealing complex charge dynamics influenced by long-range Coulomb interactions and Hund's coupling.

Contribution

It demonstrates the existence of charge order in FeTe using STM, highlighting the importance of long-range Coulomb interactions in iron-based superconductors.

Findings

Discovery of charge-stripe order in FeTe

Anisotropic electronic dispersion observed

Charge order linked to long-range Coulomb interactions

Abstract

Charge ordering is one of the most intriguing and extensively studied phenomena in correlated electronic materials because of its strong impact on electron transport properties including superconductivity. Despite its ubiquitousness in correlated systems, the occurrence of charge ordering in iron-based superconductors is still unresolved. Here we use scanning tunneling microscopy to reveal a long-range charge-stripe order and a highly anisotropic dispersion of electronic states in the ground state of stoichiometric FeTe, the parent compound of the Fe(Te, Se, S) superconductor family. The formation of charge order in a strongly correlated electron system with integer nominal valence (here Fe$^{2+}$) is unexpected and suggests that the iron-based superconductors may exhibit more complex charge dynamics than originally expected. We show that the present observations can be attributed to the surpassing of the role of local Coulomb interaction by the poorly screened longer-range Coulomb interactions, facilitated by large Hund's rule coupling.